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Shapes and energies of icosahedral fullerenes are studied on an atomically detailed level. The numerical results based on the effective binary carbon-carbon potential are related to the theory of elasticity of crystalline membranes with…

其他凝聚态物理 · 物理学 2007-05-23 A. Siber

We study the photonic interactions between two distant atoms which are coupled by an optical element (a lens or an optical fiber) focussing part of their emitted radiation onto each other. Two regimes are distinguished depending on the…

量子物理 · 物理学 2008-07-15 Stefan Rist , Jürgen Eschner , Markus Hennrich , Giovanna Morigi

It is demonstrated that outer and inner electron shells, including that formed by collectivized electrons of the fullerene C60, affects dramatically the cross section of the subvalent ns-subshells of the noble gas endohedral atoms A@C60.…

原子物理 · 物理学 2007-05-23 M. Ya. Amusia , A. S. Baltenkov , A. Z. Msezane , S. T. Manson

We show here that the photonic states emitted by ensembles of multilevel atoms via a superradiance process exhibit entanglement in the modal (frequency) degree of freedom, making this collective emission process a favorable candidate for a…

量子物理 · 物理学 2025-07-01 Amir Sivan , Meir Orenstein

Major advances in state-of-the-art theoretical methods coupled with advances in computational architectures have opened the doorway to large-scale computations on elements across the periodic table, allowing the inclusion of fully…

高能天体物理现象 · 物理学 2012-08-17 Brendan M. McLaughlin , Connor P. Ballance

Streaked photoelectron emission spectra access the correlated dynamics of photoelectrons and residual target electrons with attosecond temporal resolution. We calculated ab initio single-ionization spectra for photoemission from helium…

原子物理 · 物理学 2024-09-06 Hongyu Shi , Uwe Thumm

Multiphoton ionization of helium is investigated in the superintense field regime, with particular emphasis on the role of the electron-electron interaction in the ionization and stabilization dynamics. To accomplish this, we solve ab…

量子物理 · 物理学 2015-05-27 S. A. Sørngård , S. Askeland , R. Nepstad , M. Førre

It is demonstrated that the fullerene shell affects dramatically the radiative and Auger vacancy decay of an endohedral atom A@C60. The collectivized electrons of the C60 shell add new possibilities for radiative and non-radiative decays…

原子物理 · 物理学 2022-06-13 M. Ya. Amusia , A. S. Baltenkov

The process of ionization of a hydrogen atom by a short infrared laser pulse is studied in the regime of very large pulse intensity, in the dipole approximation. Let $A$ denote the integral of the electric field of the pulse over time at…

数学物理 · 物理学 2015-05-18 Juerg Froehlich , Alessandro Pizzo , Benjamin Schlein

We analyze using Poisson equation the spatial distributions of the positive charge of carbon atomic nuclei shell and negative charge of electron clouds forming the electrostatic potential of the C60 fullerene shell as a whole. We consider…

原子与分子团簇 · 物理学 2019-05-01 M. Ya. Amusia , A. S. Baltenkov

Photoionization of a Xe atom confined inside C$_{60}$ has been studied using the random phase approximation with exchange (RPAE) method. The C$_{60}$ fullerene has been descr ibed by an attractive short range spherical well with potential…

原子物理 · 物理学 2009-11-13 Zhifan Chen , Alfred Z. Msezane

We demonstrate that the structure of confinement resonances in the photoionization cross section of an endohedral atom is very sensitive to the mean displacement <a> of the atom from the cage center. The resonances are strongly suppressed…

原子与分子团簇 · 物理学 2015-05-14 A. V. Korol , A. V. Solov'yov

Photoionized and electronically excited ethylene \ce{C2H4+} can undergo \ce{H}-loss, \ce{H2}-loss, and ethylene-ethylidene isomerization, where the latter entails a hydrogen migration. Recent pioneering experiments with few-femtosecond…

化学物理 · 物理学 2024-05-28 Lina Fransén , Thierry Tran , Saikat Nandi , Morgane Vacher

Fullerene complexes may play a key role in the design of future molecular electronics and nanostructured devices with potential applications in light harvesting using organic solar cells. Charge and energy flow in these systems is mediated…

The spin polarization of photoelectrons induced by an intense linearly polarized laser field is investigated using numerical solutions of the time-dependent Schr\"odinger equation in companion with our analytic treatment via the…

原子物理 · 物理学 2024-02-20 Pei-Lun He , Zhao-Han Zhang , Karen Z. Hatsagortsyan , Christoph H. Keitel

We present a detailed formalism for the description of collective electron excitations in fullerenes in the process of the electron inelastic scattering. Considering the system as a spherical shell of a finite width, we show that the…

原子与分子团簇 · 物理学 2016-10-07 Alexey V. Verkhovtsev , Andrei V. Korol , Andrey V. Solov'yov

We theoretically investigate the ability of free electrons to yield information on the nonlinear Floquet dynamics of atomic systems subject to intense external illumination. By applying a quantum-mechanical formalism to describe the…

量子物理 · 物理学 2022-09-12 Eduardo Arqué López , Valerio Di Giulio , F. Javier García de Abajo

We show that if the laser is intense enough, it may always ionize an atom or induce transitions between discrete energy levels of the atom, no matter what is its frequency. It means in the quantum transition of an atom interacting with an…

量子物理 · 物理学 2007-05-23 Qi-Ren Zhang

The initial insight into electron elastic scattering off endohedral fullerenes A@C60 is gained in the framework of a theoretical approach where the C60 cage is modelled by a rectangular (in the radial coordinate) potential well, as in many…

原子物理 · 物理学 2014-03-20 V K Dolmatov , M B Cooper , M E Hunter

Inelastic interactions of nuclei accelerated to a momentum of 4.5 GeV/$c$ per projectile nucleon with photoemulsion nuclei have been investigated. The main features of these interactions - mean ranges of $^6$Li nuclei, mean multiplicities…