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Accurately modeling photochemical reactions is difficult due to the presence of conical intersections and locally avoided crossings as well as the inherently multiconfigurational character of excited states. As such, one needs a multi-state…

化学物理 · 物理学 2024-04-26 Matthew R. Hennefarth , Matthew R. Hermes , Donald G. Truhlar , Laura Gagliardi

Recent microscopic studies, based on the theoretical framework of nuclear energy density functionals, have analyzed dynamic (least action) and static (minimum energy) fission paths, and it has been shown that in addition to the important…

核理论 · 物理学 2015-11-19 Jie Zhao , Bing-Nan Lu , Tamara Niksic , Dario Vretenar

Relativistic energy density functionals (REDF) provide a complete and accurate, global description of nuclear structure phenomena. A modern semi-empirical functional, adjusted to the nuclear matter equation of state and to empirical masses…

核理论 · 物理学 2015-06-05 V. Prassa , T. Niksic , G. A. Lalazissis , D. Vretenar

A systematic study of low energy nuclear structure at normal deformation is carried out using the Hartree-Fock-Bogoliubov theory extended by the Generator Coordinate Method and mapped onto a 5-dimensional collective quadrupole Hamiltonian.…

核理论 · 物理学 2010-04-06 J. P. Delaroche , M. Girod , J. Libert , H. Goutte , S. Hilaire , S. Peru , N. Pillet , G. F. Bertsch

The evolution of the nuclear shapes along the triaxial landscape is studied in the Pt isotopic chain using the selfconsistent Hartree-Fock-Bogoliubov approximation based on the Gogny interaction. In addition to the parametrization D1S, the…

核理论 · 物理学 2014-11-20 R. Rodriguez-Guzman , P. Sarriguren , L. M. Robledo , J. E. Garcia-Ramos

To further develop accurate and large-scale simulations of electrochemical interfaces, we propose a unified explicit electric potential framework to simultaneously predict atomic forces and electron density distributions. The framework…

化学物理 · 物理学 2026-04-14 Jingwen Zhou , Yawen Yu , Xuwei Liu , Chungen Liu

Neural networks (NNs) offer a path towards synthesizing and interpreting data on faster timescales than traditional physics-informed computational models. In this work we develop two neural networks relevant to equilibrium and shape control…

等离子体物理 · 物理学 2022-07-06 J. T. Wai , M. D. Boyer , E. Kolemen

Constructing accurate, high dimensional molecular potential energy surfaces (PESs) for polyatomic molecules is challenging. Reproducing Kernel Hilbert space (RKHS) interpolation is an efficient way to construct such PESs. However, the…

化学物理 · 物理学 2020-11-06 Debasish Koner , Markus Meuwly

The cranked relativistic Hartree+Bogoliubov theory has been applied for a systematic study of the nuclei around 254No, the heaviest elements for which detailed spectroscopic data are available. The deformation, rotational response, pairing…

核理论 · 物理学 2009-11-10 A. V. Afanasjev , T. L. Khoo , S. Frauendorf , G. A. Lalazissis , I. Ahmad

One of the obstacles hindering the scaling-up of the initial successes of machine learning in practical engineering applications is the dependence of the accuracy on the size of the database that "drives" the algorithms. Incorporating the…

计算工程、金融与科学 · 计算机科学 2021-06-09 Wei Li , Martin Z. Bazant , Juner Zhu

The accurate determination of electron properties is fundamental to low-temperature plasma simulations, necessitating precise solutions to the spatially inhomogeneous electron Boltzmann equation (EBE). This work explores the use of…

等离子体物理 · 物理学 2026-05-07 Ihda Chaerony Siffa , Detlef Loffhagen , Markus M. Becker , Jan Trieschmann

In the present study we generalize the self-consistent Hartree-Fock-Bogoliubov (HFB) theory formulated in the coordinate space to the case which incorporates an arbitrary mixing between protons and neutrons in the particle-hole (p-h) and…

核理论 · 物理学 2009-11-10 E. Perlinska , S. G. Rohozinski , J. Dobaczewski , W. Nazarewicz

The microscopic studies on nuclear fission require the evaluation of the potential energy surface as a function of the collective coordinates. A reasonable choice of constraints on multipole moments should be made to describe the topography…

核理论 · 物理学 2021-07-21 A. Zdeb , M. Warda , L. M. Robledo

This paper proposed a novel radial basis function neural network (RBFNN) to solve various partial differential equations (PDEs). In the proposed RBF neural networks, the physics-informed kernel functions (PIKFs), which are derived according…

数值分析 · 数学 2023-06-08 Zhuojia Fu , Wenzhi Xu , Shuainan Liu

A recently introduced analytical model for the nuclear density profile[1] is implemented in the Extended Thomas-Fermi (ETF) energy density functional. This allows to (i) shed a new light on the issue of the sign of surface symmetry energy…

核理论 · 物理学 2014-07-10 Francois Aymard , Francesca Gulminelli , Jérôme Margueron

Guiding by the relativistic local density approximation, we explore a phenomenological formula for the coupling strength of Coulomb field to take into account the Coulomb exchange term effectively in the relativistic Hartree approximation.…

核理论 · 物理学 2013-05-27 Z. M. Niu , Q. Liu , Y. F. Niu , W. H. Long , J. Y. Guo

The development of a modern and more realistic nuclear energy density functional (EDF) for accurate predictions of properties of nuclei is the subject of enhanced activity, since it is very important for the study of properties of nuclear…

核理论 · 物理学 2019-11-14 S. Shlomo , A. I. Sanzhur

We investigated the structure of the low density regions of the inner crust of neutron stars using the Hartree-Fock-Bogoliubov (HFB) model to predict the proton content $Z$ of the nuclear clusters and, together with the lattice spacing, the…

核理论 · 物理学 2017-09-13 A. Pastore , M. Shelley , S. Baroni , C. A. Diget

The potential-energy surfaces of an extended set of heavy and super-heavy even-even nuclei with $92 \le Z \le 126$ and isospins $40 \le N-Z \le 74$ are evaluated within the recently developed Fourier shape parametrization. Ground-state and…

核理论 · 物理学 2018-03-28 K. Pomorski , B. Nerlo-Pomorska , J. Bartel , C. Schmitt

Potential energy surfaces of even-even superheavy nuclei are evaluated within the macroscopic-microscopic approximation. A very rapidly converging analytical Fourier-type shape parametrization is used to describe nuclear shapes throughout…