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We propose a new variational method for describing nuclear matter from nucleon-nucleon interaction. We use the unitary correlation operator method (UCOM) for central correlation to treat the short-range repulsion and further include the…

The main motivation for this work is the exploration of rotational-vibrational states corresponding to electronic excitations in a pre-Born-Oppenheimer quantum theory of molecules. These states are often embedded in the continuum of the…

化学物理 · 物理学 2018-10-15 Edit Mátyus

A procedure for calculation of rotation-vibration states of medium sized molecules is presented. It combines the advantages of variational calculations and perturbation theory. The vibrational problem is solved by diagonalizing a…

化学物理 · 物理学 2015-04-13 A. I. Pavlyuchko , S. N. Yurchenko , Jonathan Tennyson

We employ the Born-Oppenheimer approximation to find the effective potential in a three-body system consisting of a light particle and two heavy ones when the heavy-light short-range interaction potential has a resonance corresponding to a…

原子物理 · 物理学 2013-09-25 Maxim A. Efremov , Lev Plimak , Misha Yu. Ivanov , Wolfgang P. Schleich

We propose an alternative to the usual time--independent Born--Oppenheimer approximation that is specifically designed to describe molecules with non--symmetrical hydrogen bonds. In our approach, the masses of the hydrogen nuclei are scaled…

数学物理 · 物理学 2009-11-13 George A. Hagedorn , Alain Joye

A few per cent fraction of antiprotons stopped in helium survives for an enormous time (up to tens of microseconds) in comparison with the usual lifetime ($10^{-12}s$) of these particles in matter. The explanation is that antiprotons are…

核理论 · 物理学 2011-04-15 O. I. Kartavtsev

We present an accurate theoretical determination of rovibrational energy levels of the hydrogen molecule and its isotopologues in its electronic ground state. We consider all significant corrections to the Born-Oppenheimer approximation,…

The hydrogen atom as relativistic bound-state system of a proton and an electron in the complex-mass scheme is investigated. Interaction of a proton and an electron in the atom is described by the Lorentz-scalar Coulomb potential; the…

量子物理 · 物理学 2019-03-19 Mikhail N. Sergeenko

A numerical algorithm based on the probabilistic path integral approach for solving Schroedinger equation has been devised to treat molecular systems without Born-Oppenheimer approximation in the non relativistic limit at zero temperature…

量子物理 · 物理学 2023-02-28 Sumita Datta

This article describes a method for calculating higher order or nonadiabatic corrections in Born-Oppenheimer theory and its interaction with the translational degrees of freedom. The method uses the Wigner-Weyl correspondence to map nuclear…

化学物理 · 物理学 2023-12-21 Robert Littlejohn , Jonathan Rawlinson , Joseph Subotnik

The calculation of the hindered roton-phonon energy levels of a hydrogen molecule in a confining potential with different symmetries is systematized for the case when the rotational angular momentum $J$ is a good quantum number. One goal of…

凝聚态物理 · 物理学 2009-11-07 T. Yildirim , A. B. Harris

Potential energy curves for excited leptonic states of the helium-antihydrogen system are calculated within Ritz' variational approach. An explicitly correlated ansatz for the leptonic wave function is employed describing accurately the…

原子物理 · 物理学 2015-05-13 V. Sharipov , L. Labzowsky , G. Plunien

This report presents a new approach for treating the coupling of electrons and nuclei in quantum mechanical calculations for molecules and condensed matter. It includes the standard "Born-Oppenheimer approximation" as a special case but…

化学物理 · 物理学 2013-06-28 Gerald I. Kerley

The energy spectrum, atom-dimer scattering length, and atom-trimer scattering length for systems of three and four ultracold atoms with $\delta$-function interactions in one dimension are presented as a function of the relative mass ratio…

量子气体 · 物理学 2015-06-18 Nirav P. Mehta

We calculate the ground--state energy and other physical properties of the hydrogen atom inside a spherical box with an impenetrable wall. We apply the variational method and perturbation theory and compare both approximate results. We show…

量子物理 · 物理学 2015-05-19 Francisco M. Fernández , N. Aquino , A. Flores-Riveros

The exchange contribution to the energy of the hydrogen atom interacting with a proton is calculated from the polarization expansion of the wave function using the conventional surface-integral formula and two formulas involving volume…

量子物理 · 物理学 2016-11-02 Piotr Gniewek , Bogumił Jeziorski

Three simple $7-, (7+3)-, 10-$parametric trial functions for the ${\rm H}_3^+$ molecular ion are presented. Each of them provides subsequently the most accurate approximation for the Born-Oppenheimer ground state energy among…

量子物理 · 物理学 2015-05-28 J. C. Lopez Vieyra , A. V. Turbiner , H. Medel Cobaxin

The mass-correction functions in the second-order non-adiabatic Hamiltonian are computed for the $^4$He$^+_2$ molecular ion using the variational method, floating explicitly correlated Gaussian functions, and a general…

化学物理 · 物理学 2018-12-05 Edit Mátyus

We leverage the power of neural quantum states to describe the ground state wave function of solid and liquid atomic hydrogen, including both electronic and protonic degrees of freedom. For static protons, the resulting Born-Oppenheimer…

强关联电子 · 物理学 2026-04-27 David Linteau , Saverio Moroni , Giuseppe Carleo , Markus Holzmann

This work considers how the properties of hydrogen bonded complexes, D-H....A, are modified by the quantum motion of the shared proton. Using a simple two-diabatic state model Hamiltonian, the analysis of the symmetric case, where the donor…

化学物理 · 物理学 2014-05-09 Ross H. McKenzie , Christiaan Bekker , Bijyalaxmi Athokpam , Sai G. Ramesh
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