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We utilize few-level model systems to analyze the polarization and phase properties of below-threshold harmonics generated from aligned molecules. In a two-level system, we find that the phase of emitted harmonics undergoes a distinct…

量子物理 · 物理学 2026-05-06 Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

Understanding electrochemical phenomena at complex liquid solid interfaces requires linking real time structural dynamics with atomic scale interfacial chemistry. Here, we integrate operando synchrotron X-ray fluorescence and diffraction…

HfO$_2$- and ZrO$_2$-based ferroelectric thin films have emerged as promising candidates for the gate oxides of next generation electronic devices. Recent work has experimentally demonstrated that a tetragonal/orthorhombic (t/o-) phase…

介观与纳米尺度物理 · 物理学 2024-03-11 Prabhat Kumar , Michael Hoffmann , Andrew Nonaka , Sayeef Salahuddin , Zhi Yao

Charge profiles in liquid electrolytes are of crucial importance for applications, such as supercapacitors, fuel cells, batteries, or the self-assembly of particles in colloidal or biological settings. However, creating localised (screened)…

软凝聚态物质 · 物理学 2021-03-17 Jeffrey C. Everts , Miha Ravnik

Thick (~50 nm) films of Hf were evaporated onto bare and oxidized Si(001) samples, and thin (~monolayer) films of Hf were evaporated onto clean Si(001)-(2x1) surfaces. Upon annealing to 1000$^/circ$C, films of HfSi2 were formed after…

材料科学 · 物理学 2007-05-23 H. T. Johnson-Steigelman , A. V. Brinck , P. F. Lyman

Successful synthesis of the nitrogenated holey two-dimensional structures C2N (Nat. Commun. 2015, 6, 1-7) using simply wet-chemical reaction offer a cost-effective way to generate other 2D materials with novel optical and electronic…

材料科学 · 物理学 2015-05-12 Ruiqi Zhang , Bin Li , Jinlong Yang

Chemically exfoliated nanoscale few-layer thin Li$_x$CoO$_2$ samples are studied as function of annealing at various temperatures, using transmission electron microscopy (TEM) and Electron Energy Loss Spectroscopies (EELS), probing the O-K,…

Phase diagram of Na$_x$CoO$_2$ (x $\gtrsim$ 0.71) has been reinvestigated using electrochemically fine tuned single crystals. Both phase separation and staging phenomena as a result of sodium multi-vacancy cluster ordering have been found.…

强关联电子 · 物理学 2009-07-13 G. J. Shu , F. -T. Huang , M. -W. Chu , J. -Y. Lin , Patrick A. Lee , F. C. Chou

A classical variant of the two-dimensional anisotropic Heisenberg model reproducing inelastic neutron scattering experiments on La_5 Ca_9 Cu_24 O_41 [M. Matsuda et al., Phys.Rev. B 68, 060406(R) (2003)] is analysed using mostly Monte Carlo…

统计力学 · 物理学 2009-11-10 R. Leidl , W. Selke

Destruction of the vortex lattice by random point pinning is considered as a mechanism of the ``second peak'' transition observed experimentally in weakly coupled layered high temperature superconductors. The transition field separating the…

超导电性 · 物理学 2009-10-31 A. E. Koshelev , V. M. Vinokur

Magnetization processes of spin-1/2 layered triangular-lattice antiferromagnets (TLAFs) under a magnetic field H are studied by means of a numerical cluster mean-field method with a scaling scheme. We find that small antiferromagnetic…

强关联电子 · 物理学 2015-02-13 Daisuke Yamamoto , Giacomo Marmorini , Ippei Danshita

Structural disorder causes materials surface electronic properties, e.g. work function ($\phi$) to vary spatially, yet it is challenging to prove exact causal relationships to underlying ensemble disorder, e.g. roughness or granularity. For…

In the majority of magnetic systems the surface is required to order at the same temperature as the bulk. In the present study, we report a distinct and unexpected surface magnetic phase transition, uniquely at a lower temperature than the…

Systematic exploration of amorphous ABC heterostructures revealed that nanoscale morphological modifications markedly improved their artificial bulk second-order susceptibility. These amorphous birefringent heterostructures were fabricated…

Periodic nanostructures can display the dynamics of arrays of atoms while enabling the tuning of interactions in ways not normally possible in Nature. We examine one dimensional arrays of a ``synthetic atom,'' a one dimensional ring with a…

介观与纳米尺度物理 · 物理学 2008-08-16 Bahman Roostaei , Kieran Mullen

We investigate a microwave ionization of highly excited atom in a low frequency field and show that such a process may be studied on the bases of map for the electron energy change during the period of the electron motion between two…

chao-dyn · 物理学 2016-08-31 B. Kaulakys , G. Vilutis

In this conference proceeding, I discuss in detail the deconfinement to quark matter that takes place at large densities and/or temperatures. The first-order phase transition that is assumed to appear beyond a critical point gives rise to…

核理论 · 物理学 2018-01-26 Veronica Dexheimer

Electron ptychography provides highly sensitive, dose efficient phase images which can be corrected for aberrations after the data has been acquired. This is crucial when very precise quantification is required, such as with sensitivity to…

材料科学 · 物理学 2023-07-27 Christoph Hofer , Timothy J. Pennycook

Based on first-principles calculations we show that the oxidation of ultrathin films of Ca$_2$N electrides, electrenes, drives a hexagonal$\rightarrow$tetragonal structural transition. The ground state configuration of the oxidized…

材料科学 · 物理学 2020-05-06 Pedro H. Souza , José E. Padilha , Roberto H. Miwa

Precise control of surface properties including electrical characteristics, wettability, and friction is a prerequisite for manufacturing modern organic electronic devices. The successful combination of bottom up approaches for aligning and…

材料科学 · 物理学 2011-07-05 G. Hlawacek , Q. Shen , C. Teichert , A. Lex , G. Trimmel , W. Kern