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Carrier multiplication (CM), a photo-physical process to generate multiple electron-hole pairs by exploiting excess energy of free carriers, is explored for efficient photovoltaic conversion of photons from the blue solar band,…

This work demonstrates photon emission gain, i.e., emission of multiple photons per injected electron, through impact excitation in Er-doped silicon light-emitting diodes (LEDs). Conventional methods for exciting Er ions in silicon suffer…

Using two-dimensional THz spectroscopy in combination with numerical models, we investigate the dynamics linked to carrier multiplication caused by high-field THz excitation of the low-gap semiconductor InSb. In addition to previously…

其他凝聚态物理 · 物理学 2022-12-21 Simone Biasco , Florence Burri , Sarah Houver , Elsa Abreu , Matteo Savoini , Steven L. Johnson

From electrodeless time-resolved microwave conductivity measurements, the efficiency of charge carrier generation, their mobility, and decay kinetics on photo-excitation were studied in arrays of Si nanowires grown by the vapor-liquid-solid…

Multiple exciton generation (MEG) is a widely studied phenomenon in semiconductor nanocrystals and quantum dots wherein photo-excited carriers relax by generating additional electron-hole pairs. Here, we present the first experimental…

材料科学 · 物理学 2023-10-27 S. R. Sahu , A. Tripathy , K. Dey , N. Mansuri , V. G. Sathe , D. K. Shukla

Above-threshold light emission from plasmonic tunnel junctions, when emitted photons have energies significantly higher than the energy scale of the incident electrons, has attracted much recent interest in nano-optics, while the underlying…

介观与纳米尺度物理 · 物理学 2020-12-08 Longji Cui , Yunxuan Zhu , Mahdiyeh Abbasi , Arash Ahmadivand , Burak Gerislioglu , Peter Nordlander , Douglas Natelson

The article reviews recent progress in the theoretical understanding of near-field surface electromagnetic phenomena in pristine and atomically doped carbon nanotubes. The phenomena involving strong coupling effects are outlined. They are…

介观与纳米尺度物理 · 物理学 2010-11-01 I. V. Bondarev

We present a real-time investigation of ultrafast carrier dynamics in single-wall carbon nanotube bundles using femtosecond time-resolved photoelectron spectroscopy. The experiments allow to study the processes governing the subpicosecond…

材料科学 · 物理学 2009-11-07 Tobias Hertel , Roman Fasel , Gunnar Moos

In atomically thin semiconductors based on transition metal dichalcogenides, photoexcitation can be used to generate high densities of electron-hole pairs. Due to optical nonlinearities, which originate from Pauli blocking and many-body…

介观与纳米尺度物理 · 物理学 2020-12-15 Daniel Erben , Alexander Steinhoff , Michael Lorke , Frank Jahnke

We present a study of free carrier photo-generation and multi-carrier bound states, such as biexcitons and trions (ionized excitons), in semiconducting single-walled carbon nanotubes. Pump-and-probe measurements performed with fs pulses…

We study the dynamics of photo-induced charge carriers in realistic models of LaVO3 and YTiO3 polar heterostructures. It is shown that two types of impact ionization processes contribute to the carrier multiplication in these strongly…

强关联电子 · 物理学 2019-09-04 Francesco Petocchi , Sophie Beck , Claude Ederer , Philipp Werner

Electrons and holes in a semiconductor form hydrogen-atom-like bound states, called excitons. At high electron-hole densities the attractive Coulomb force becomes screened and excitons can no longer exist. Bardeen-Cooper-Schrieffer theory…

超导电性 · 物理学 2012-05-16 Marijn A. M. Versteegh , A. J. van Lange , H. T. C. Stoof , Jaap I. Dijkhuis

It is shown that semiconductor nanoscale resonators with extreme dielectric confinement accelerate the diffusion of electron-hole pairs excited by nonlinear absorption. These novel cavity designs may lead to optical switches with superior…

In semiconductors, photoexcited electrons and holes (carriers) initially occupy high-energy states, but quickly lose energy to phonons and relax to the band edge within a picosecond [1]. Increasing the lifetime of carriers in…

材料科学 · 物理学 2015-04-15 Jonathan Trinastic , Iek-Heng Chu , Hai-Ping Cheng

Optically generated electron-hole pairs can probe strongly correlated electronic matter, or, by forming exciton-polaritons within an optical cavity, give rise to photonic nonlinearities. The present paper theoretically studies the…

强关联电子 · 物理学 2020-04-29 Tobias Graß , Ovidiu Cotlet , Atac İmamoğlu , Mohammad Hafezi

Theory predicts peculiar features for excited-state dynamics in one dimension (1D) that are difficult to be observed experimentally. Single-walled carbon nanotubes (SWNTs) are an excellent approximation to 1D quantum confinement, due to…

介观与纳米尺度物理 · 物理学 2015-05-13 Giancarlo Soavi , Francesco Scotognella , Daniele Viola , Timo Hefner , Tobias Hertel , Giulio Cerullo , Guglielmo Lanzani

We report here an assessment of carrier multiplication (CM) yields in PbSe and PbS nanocrystals (NCs) by a quantitative analysis of biexciton and exciton dynamics in transient photoluminescence decays. Interest in CM, the generation of more…

材料科学 · 物理学 2009-11-13 Gautham Nair , Scott M Geyer , Liang-Yi Chang , Moungi G Bawendi

Surface plasmon enhanced processes and hot-carrier dynamics in plasmonic nanostructures are of great fundamental interest to reveal light-matter interactions at the nanoscale. Using plasmonic tunnel junctions as a platform supporting both…

The recently reported experimental optical spectra of double-walled carbon nanotubes exhibit more peaks than it could be expected based on the layers alone. The appearance of excess peaks has been attributed to the interlayer interaction.…

介观与纳米尺度物理 · 物理学 2020-08-12 Valentin N. Popov

By using Boltzmann formalism, we show that carrier multiplication by impact ionization can take place at relatively low electric fields during electronic transport in graphene. Because of the absence of energy gap, this effect is not…

介观与纳米尺度物理 · 物理学 2015-05-27 Anuj Girdhar , Jean-Pierre Leburton