相关论文: Experimental verification of a self-consistent the…
We rigorously apply the sum rules to the sum-over-states expression to calculate the fundamental limits of the dispersion of the two-photon absorption cross-section. A comparison of the theory with the data suggests that the truncated sum…
Quantum-inspired superresolution methods surpass the Rayleigh limit in imaging, or the analogous Fourier limit in spectroscopy. This is achieved by carefully extracting the information carried in the emitted optical field by engineered…
High-precision measurements implemented by means of light is desired in all fields of science. However, light is a wave and Rayleigh criterion gives us a diffraction limitation in classical optics which restricts to get arbitrary high…
It is proposed a few-atom Doppler-sensitive absorption spectroscopy scheme resolving the long-standing dilemma regarding the nature of an atomic quantum translational motion (superpositional or non-superpositional) and its measurement…
Rayleigh's criterion for resolving two incoherent point sources has been the most influential measure of optical imaging resolution for over a century. In the context of statistical image processing, violation of the criterion is especially…
The electronic structure of atomic quantum systems and their dynamical interaction with light is reflected in transition dipole matrix elements coupling the system's energy eigenstates. In this work, we measure phase shifts of the…
An ab initio theory is devised for the x-ray photoabsorption cross section of atoms in the field of a moderately intense optical laser (800nm, 10^13 W/cm^2). The laser dresses the core-excited atomic states, which introduces a dependence of…
Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…
The two photon exchange amplitude is investigated in frame of analytic properties of the virtual Compton scattering amplitude as a function of the invariant mass squared of the intermediate hadronic state. A sum rule is built, based on…
We present a linear-response formalism for a system of correlated electrons out of equilibrium, as relevant for the probe optical absorption in pump-probe experiments. We consider the time dependent optical conductivity $\sigma(\omega,t)$…
We apply a sum rule for the forward light-by-light scattering process within the context of the $\phi^4$ quantum field theory. As a consequence of the sum rule a stringent causality criterion is presented and the resulting constraints are…
Entangled two-photon absorption can enable a linear scaling of fluorescence emission with the excitation power. In comparison to classical two-photon absorption with a quadratic scaling, this can allow fluorescence imaging or…
We study light absorption in many-electron interacting systems beyond the linear regime by using a {\em single} broadband impulse of an electric field in the instantaneous limit. We determine non-pertubatively the absorption cross section…
Absorption and emission of light is studied theoretically for excited atoms in coherent superposition of states subjected to isolated attosecond pulses in the extreme ultraviolet range. A gauge invariant formulation of transient absorption…
Nonlinear optics is essential for many recent photonic technologies. Here, we introduce a novel multi-scale approach to simulate the nonlinear optical response of molecular nanomaterials combining ab initio quantum-chemical and classical…
We develop a linear response theory to provide a unified description of two recent spectroscopy protocols for probing one-dimensional supersolid states realized in cold-atom systems. Both protocols involve applying a periodic optical…
Optical spectroscopy provides a powerful, contact-free probe of topological quantum states, yet exact constraints on antisymmetric Hall absorption remain much less well developed than their longitudinal counterparts. Motivated by earlier…
We present a method for recovery of narrow homogeneous spectral features out of broad inhomogeneous overlapped profile based on second-derivative processing of the absorption spectra of alkali metal atomic vapor nanocells. The method is…
We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…
Two twin beams with a shared signal beam and separated idler beams are used together with the photon-number-resolving postselection in the signal beam to arrive at two coupled beams with anticorrelations in photon-number fluctuations.…