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We present an ab initio study of neutral core and valence electronic excitations in {\alpha}-Al2O3 by solving the Bethe-Salpeter equation (BSE) of many-body perturbation theory within an all-electron framework. Calculated spectra at the Al…

材料科学 · 物理学 2024-01-26 M. Laura Urquiza , Matteo Gatti , Francesco Sottile

Systematic experimental data on resonant inelastic X-ray scattering (RIXS) in GaN near the N K-edge are presented for the first time. Excitation energy dependence of the spectral structures manifests the band structure effects originating…

材料科学 · 物理学 2009-11-10 V. N. Strocov , T. Schmitt , J. -E. Rubensson , P. Blaha , T. Paskova , P. O. Nilsson

Resonant inelastic X-ray scattering (RIXS) is a promising technique for obtaining electron-phonon coupling constants. However, the ability to extract these coupling constants throughout the Brillouin zone for crystalline materials remains…

材料科学 · 物理学 2018-12-19 Andrey Geondzhian , Keith Gilmore

We investigate magnetic excitations in the spin-ladder compound Sr$_{14}$Cu$_{24}$O$_{41}$ using high-resolution Cu $L_3$-edge Resonant Inelastic X-ray Scattering (RIXS). Our findings demonstrate that RIXS couples to collective spin…

We report a Cu $K$-edge resonant inelastic x-ray scattering (RIXS) study of charge-transfer excitations in the 2-8 eV range in the structurally simple compound HgBa$_2$CuO$_{4+\delta}$ at optimal doping ($T_{\rm c} = 96.5 $ K). The spectra…

强关联电子 · 物理学 2009-11-11 L. Lu , X. Zhao , G. Chabot-Couture , J. N. Hancock , N. Kaneko , O. P. Vajk , G. Yu , S. Grenier , Y. J. Kim , D. Casa , T. Gog , M. Greven

We calculate the K-edge indirect bimagnon resonant inelastic X-ray scattering (RIXS) intensity spectra of the bicollinear antiferromagnetic order known to occur in the $\alpha$-FeTe chalcogenide system. Utilizing linear spin wave theory for…

材料科学 · 物理学 2017-11-28 Zengye Huang , Sean Mongan , Trinanjan Datta , Dao-Xin Yao

Resonant inelastic X-ray scattering (RIXS) at the $L$-edge of transition metal elements is now commonly used to probe single magnon excitations. Here we show that single magnon excitations can also be measured with RIXS at the $K$-edge of…

High resolution resonant inelastic x-ray scattering (RIXS) has proven particularly effective in the determination of crystal field and spin excitations in cuprates. Its strength lies in the large Cu $L_{3}$ resonance and in the fact that…

We theoretically examine the momentum dependence of resonant inelastic x-ray scattering (RIXS) spectrum for one-dimensional and two-dimensional cuprates based on the single-band Hubbard model with realistic parameter values. The spectrum is…

强关联电子 · 物理学 2007-05-23 T. Tohyama , K. Tsutsui , S. Maekawa

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. In this work, we will investigate how RIXS can…

超导电性 · 物理学 2016-05-13 Pasquale Marra

A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…

材料科学 · 物理学 2012-06-18 Young-June Kim , J. P. Hill , H. Yamaguchi , T. Gog , D. Casa

The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge density wave order,…

Using a model Hamiltonian, we discuss how we could interpret data obtained from transition metal $K$-edge resonant inelastic x-ray scattering (RIXS) experiments. By analyzing the creation of valence excitations from the screening of the…

材料科学 · 物理学 2008-08-08 K. H. Ahn , A. J. Fedro , Michel van Veenendaal

Nonresonant inelastic x-ray scattering (NIXS) is a possible tool to detect charge excitations in electron systems. In addition, multipole transitions at high-momentum-transfer region open a new possibility to determine orbital-selective…

强关联电子 · 物理学 2015-11-11 Kenji Tsutsui , Eiji Kaneshita , Takami Tohyama

Results of resonant inelastic X-ray scattering (RIXS) measurements at Fe L-edges and electronic structure calculations of LiFeAs and NaFeAs are presented. Both experiment and theory show that in the vicinity of the Fermi energy, the density…

We study resonant inelastic x-ray scattering (RIXS) peaks corresponding to low energy particle-hole excited states of metallic FeTe and semi-metallic TiSe$_2$ for photon incident energy tuned near the $L_{3}$ absorption edge of Fe and Ti…

材料科学 · 物理学 2014-07-04 B. Barbiellini , J. N. Hancock , C. Monney , Y. Joly , G. Ghiringhelli , L. Braicovich , T. Schmitt

We have investigated the electronic structure of Sr2IrO4 within the density-functional theory using the generalized gradient approximation while taking into account strong Coulomb correlations in the framework of the fully relativistic…

强关联电子 · 物理学 2023-10-13 V. N. Antonov , D. A. Kukusta , L. V. Bekenov

Resonant inelastic x-ray scattering (RIXS) is an extremely valuable tool for the study of elementary, including magnetic, excitations in matter. Latest developments of this technique mostly aimed at improving the energy resolution and…

We present a non-perturbative, divergence-free series expansion of Green's functions using effective operators. The method is especially suited for computing correlators of complex operators as a series of correlation functions of simpler…

强关联电子 · 物理学 2017-12-25 Yi Lu , Maurits W. Haverkort

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: the elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation…