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We develop a formalism to study indirect resonant inelastic x-ray scattering (RIXS) in systems with itinerant electrons, accounting for the attraction between valence electrons and the positively-charged core hole exactly, and apply this…

强关联电子 · 物理学 2014-07-16 David Benjamin , Israel Klich , Eugene Demler

The real-space multiple-scattering (RSMS) approach is applied to model non-resonant inelastic scattering from deep core electron levels over a broad energy spectrum. This approach is applicable to aperiodic or periodic systems alike and…

其他凝聚态物理 · 物理学 2009-11-11 J. A. Soininen , A. L. Ankudinov , J. J. Rehr

In this short note, we report on the first inelastic neutron scattering (INS) study on high-energy magnetic excitations in Sr$_3$Ir$_2$O$_7$. We observed excitations between $\sim$80 meV and $\sim$180 meV. The peak position of the…

强关联电子 · 物理学 2021-01-12 Masaki Fujita , Kazuhiko Ikeuchi , Ryoichi Kajimoto , Mitsutaka Nakamura

High-energy, local multiplet excitations of the d-electrons are revealed in our inelastic neutron scattering measurements on the prototype magnetic insulator NiO. These become allowed by the presence of both non-zero crystal field and…

强关联电子 · 物理学 2012-06-18 Young-June Kim , A. P. Sorini , C. Stock , T. G. Perring , J. van den Brink , T. P. Devereaux

We show that Resonant Inelastic X-ray scattering (RIXS) is sensitive to three-magnon excitations in cuprates. Even if it requires three electrons to simultaneously flip their spin, the RIXS tri-magnon scattering amplitude is not small. At…

强关联电子 · 物理学 2010-02-22 Luuk J. P. Ament , Jeroen van den Brink

This paper provides a brief overview of applications of advanced X-ray spectroscopic techniques that take advantage of the resonant inelastic X-ray scattering (RIXS) in the hard and tender x-ray range and have recently become available for…

材料科学 · 物理学 2014-01-08 K. O. Kvashnina , S. M. Butorin

Despite significant progress in resonant inelastic x-ray scattering (RIXS) experiments on cuprates at the Cu L-edge, a theoretical understanding of the cross-section remains incomplete in terms of elementary excitations and the connection…

强关联电子 · 物理学 2016-05-16 Chunjing Jia , Krzysztof Wohlfeld , Yao Wang , Brian Moritz , Thomas P. Devereaux

This review aims to introduce the x-ray emission spectroscopy (XES) and resonant inelastic x-ray scattering (RIXS) techniques to the materials scientist working with magnetic semiconductors (e.g. semiconductors doped with 3d transition…

材料科学 · 物理学 2014-01-20 Mauro Rovezzi , Pieter Glatzel

Results of model calculations using exact diagonalization reveal the orbital character of states associated with different Raman loss peaks in Cu $K$-edge resonant inelastic X-ray scattering (RIXS) from La$_{2}$CuO$_{4}$. The model includes…

We calculate the K-edge indirect bimagnon resonant inelastic X-ray scattering (RIXS) intensity spectra of the bicollinear antiferromagnetic order known to occur in the $\alpha$-FeTe chalcogenide system. Utilizing linear spin wave theory for…

材料科学 · 物理学 2017-11-28 Zengye Huang , Sean Mongan , Trinanjan Datta , Dao-Xin Yao

We propose a novel way to image dynamical properties of nonstationary electron systems using ultrafast resonant x-ray scattering. Employing a rigorous theoretical analysis within the framework of quantum electrodynamics, we demonstrate that…

原子物理 · 物理学 2017-11-03 Daria Popova-Gorelova , Robin Santra

We theoretically examine the orbital excitations coupled to the spin degree of freedom in the parent state of the iron-arsenide superconductor, based on the calculation in a five-band itinerant model. The calculated Fe $L_3$-edge resonant…

强关联电子 · 物理学 2011-08-04 E. Kaneshita , K. Tsutsui , T. Tohyama

Resonant elastic x-ray scattering (REXS) is an exquisite element-sensitive tool for the study of subtle charge, orbital, and spin superlattice orders driven by the valence electrons, which therefore escape detection in conventional x-ray…

We have performed resonant inelastic x-ray scattering (RIXS) near the Cu-K edge on cuprate superconductors La(2-x)Sr(x)CuO(4), La(2-x)Ba(x)CuO(4), La(2-x)Sr(x)Cu(1-y)Fe(y)O(4) and Bi(1.76)Pb(0.35)Sr(1.89)CuO(6+d), covering underdoped to…

We theoretically investigate the resonant inelastic X-ray scattering (RIXS) spectra in a quasi-1D chain of weakly coupled frustrated spin-1/2 trimers, as realized in Na$_{2}$Cu$_{3}$Ge$_{4}$O$_{12}$, with Cu $d^{9}$ 1/2 spins. We compute…

强关联电子 · 物理学 2024-10-22 Prabhakar , Subhajyoti Pal , Umesh Kumar , Manoranjan Kumar , Anamitra Mukherjee

We present X-ray absorption spectroscopy and resonant inelastic X-ray scattering (RIXS) measurements on the iron L-edge of 0.5 mM aqueous ferricyanide. These measurements demonstrate the ability of high-throughput transition-edge-sensor…

We study conditions for aberration-free imaging of inelastic x-ray scattering (IXS) spectra with x-ray echo spectrometers. Aberration-free imaging is essential for achieving instrumental functions with high resolution and high contrast.…

仪器与探测器 · 物理学 2019-05-29 Manuel Sánchez del Río , Yuri Shvyd'ko

Resonant inelastic x-ray scattering (RIXS) has become a very powerful experimental technique to probe a broad range of intrinsic elementary excitations, for example, from low energy phonons and (bi-)magnons to high energy $d$-$d$,…

强关联电子 · 物理学 2019-06-20 Y. L. Wang , G. Fabbris , M. P. M. Dean , G. Kotliar

Resonant Inelastic X-ray scattering (RIXS) is a synchrotron-based spectroscopy that has seen growing interest across a range of scientific disciplines beyond fundamental physics. The interpretation of experimental RIXS data requires…

Controlling the flow of charge neutral interlayer exciton (IX) quasiparticles can potentially lead to low loss excitonic circuits. Here, we report unidirectional transport of IXs along nanoscale electrostatically defined channels in an…