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We present a systematic experimental study along with theoretical modeling of the energy transfer in an ensemble of closely-packed CdTe colloidal nanocrystals identified as the F\"orster resonant energy transfer (FRET). We prove that at low…

介观与纳米尺度物理 · 物理学 2015-12-22 Feng Liu , A. V. Rodina , D. R. Yakovlev , A. A. Golovatenko , A. Greilich , E. D. Vakhtin , A. Susha , A. L. Rogach , Yu. G. Kusrayev , M. Bayer

We theoretically discuss how to tune the competition between Forster transfer and spontaneous emission in a continuous and nondestructive fashion. The proposed approach is especially suitable for delicate biological systems like light…

化学物理 · 物理学 2007-06-19 Christian Blum , Willem L. Vos , Vinod Subramaniam

Long range resonance energy transfer (RET) between a donor and an acceptor molecule is increasingly being used in many areas of biological and material science. The phenomenon is used to monitor the in vivo separation between different…

材料科学 · 物理学 2007-05-23 Sangeeta Saini , Somnath Bhowmick , Vijay B. Shenoy , Biman Bagchi

We propose an energy-stable parametric finite element method (ES-PFEM) for simulating solid-state dewetting of thin films in two dimensions via a sharp-interface model, which is governed by surface diffusion and contact line (point)…

数值分析 · 数学 2020-06-08 Quan Zhao , Wei Jiang , Weizhu Bao

F\"orster resonant energy transfer (FRET) with upconverting nanoparticles (UCNPs) as donors and quantum dots (QDs) as acceptors has been regarded as a promising tool for biosensing applications. In this work, we use time-resolved…

Photonic cavities are gathering a large interest to enhance the energy transfer between two dipoles, with far-reaching consequences for applications in photovoltaics, lighting sources and molecular biosensing. However, experimental…

Single-molecule F\"{o}rster resonance energy transfer (smFRET) has become a mainstream technique for probing biomolecular structural dynamics. The rapid and wide adoption of the technique by an ever-increasing number of groups has generated…

Zero-mode waveguides (ZMWs) are confining light into attoliter volumes, enabling single molecule fluorescence experiments at physiological micromolar concentrations. Among the fluorescence spectroscopy techniques that can be enhanced by…

The paper is concerned with Forster Resonance Energy Transfer (FRET) considered as a mechanism for communication between nanodevices. Two solved issues are reported in the paper, namely: signal generation and signal storage in FRET-based…

医学物理 · 物理学 2019-12-05 Jakub Kmiecik , Krzysztof Wojcik , Pawel Kulakowski , Andrzej Jajszczyk

We calculate the rate of non-radiative, Forster-type energy transfer (ET) from an excited epitaxial quantum well (QW) to a proximal monolayer of semiconductor nanocrystal quantum dots (QDs). Different electron-hole configurations in the QW…

介观与纳米尺度物理 · 物理学 2009-11-11 S. Kos , M. Achermann , V. I. Klimov , D. L. Smith

We have developed a new model to describe FRET efficiency (E FRET) between freely-diffusing membrane probes in phase-separated bilayers (Finite Phase-separation FRET, or FP-FRET), that in principle applies to any system where phase domain…

软凝聚态物质 · 物理学 2011-06-01 Frederick A. Heberle , Gerald W. Feigenson

Applications of Fluorescence Resonance Energy Transfer (FRET) in biology have expanded tremendously in the last 25 years. This technique has become a staple technique in many biological and biophysical fields. FRET based chemical sensors…

生物物理 · 物理学 2020-05-05 Ripa Paul , Sudip Suklabaidya , Syed Arshad Hussain

We investigate theoretically the stochastic dynamics of Resonance Electronic Energy Transfer (RET), in a bi-dimensional overexcited ensemble of donor and acceptor molecules. We find that, after initial optical excitation of all the donors,…

介观与纳米尺度物理 · 物理学 2023-11-27 R. Avriller , A. Marché , G. Jonusauskas

Despite showing great promise for optoelectronics, the commercialization of halide perovskite nanostructure-based devices is hampered by inefficient electrical excitation and strong exciton binding energies. While transport of excitons in…

介观与纳米尺度物理 · 物理学 2020-10-29 Andreas Singldinger , Moritz Gramlich , Christoph Gruber , Carola Lampe , Alexander S. Urban

Interfacial adhesion is caused by intermolecular forces that only occur between surfaces at nano-scale contact (NSC) i.e., 0.1-0.4nm. To evaluate NSC and its influence on adhesion, F\"orster resonance energy transfer (FRET) spectroscopy has…

材料科学 · 物理学 2023-01-27 Mónica Gaspar Simões , Robert Schennach , Ulrich Hirn

Photo-induced excited-state energy transfer (EET) processes play an important role in the solar energy conversions. The phenylene ethynylene (PE) dendrimers display great potential in improving the efficiency of solar cells, because of…

化学物理 · 物理学 2024-01-17 Sisi Liu , Jiawei Peng , Peng Bao , Qiang Shi , Zhenggang Lan

We theoretically analyze the excitation energy transfer between two closely spaced linear molecular J-aggregates, whose excited states are Frenkel excitons. The aggregate with the higher (lower) exciton band edge energy is considered as the…

无序系统与神经网络 · 物理学 2007-05-23 C. Didraga , V. A. Malyshev , J. Knoester

We present the first time-resolved cryogenic observations of Forster energy transfer in large, monodisperse lead sulphide quantum dots with ground state transitions near 1.5 um (0.83 eV), in environments from 160 K to room temperature. The…

The question of how quantum coherence facilitates energy transfer has been intensively debated in the scientific community. Since natural and artificial light-harvesting units operate under the stationary condition, we address this question…

化学物理 · 物理学 2020-07-22 Pei-Yun Yang , Jianshu Cao

We study transfer of coherent nuclear oscillations between an excitation energy donor and an acceptor in a simple dimeric electronic system coupled to an unstructured thermodynamic bath and some pronounced vibrational intramolecular mode.…

化学物理 · 物理学 2015-01-08 Tomáš Mančal , Jakub Dostál , Jakub Pšenčík , Donatas Zigmantas