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The vibrational dynamics of formic acid monomer (FAM) and dimer (FAD) is investigated from machine-learned potential energy surfaces at the MP2 (PES$_{\rm MP2}$) and transfer-learned (PES$_{\rm TL}$) to the CCSD(T) levels of theory. The…

化学物理 · 物理学 2022-03-14 Silvan Käser , Markus Meuwly

F\"orster resonance energy transfer has an important role in nature and technology, rendering its exact theoretical understanding significant. To this end, a system of two electronically decoupled quantum dots (QDs) is considered,…

介观与纳米尺度物理 · 物理学 2025-09-22 Liubov S. Sirkina , Luke M. J. Hall , Amy Morreau , Wolfgang Langbein , Egor A. Muljarov

Single molecule FRET (fluorescence resonance energy transfer) is a powerful technique for detecting real-time conformational changes and molecular interactions during biological reactions. In this review, we examine different techniques of…

生物大分子 · 定量生物学 2007-05-23 Ivan Rasnik , Sean A. McKinney , Taekjip Ha

We derive equations of motion for the reduced density matrix of a molecular system which undergoes energy transfer dynamics competing with fast internal conversion channels. Environmental degrees of freedom of such a system have no time to…

化学物理 · 物理学 2017-05-24 Joachim Seibt , Tomas Mancal

Single molecule Forster resonance energy transfer (FRET) experiments are used to infer the properties of the denatured state ensemble (DSE) of proteins. From the measured average FRET efficiency, <E>, the distance distribution P(R) is…

生物大分子 · 定量生物学 2009-05-05 E. P. O'Brien , G. Morrison , B. R. Brooks , D. Thirumalai

We propose an energy-stable parametric finite element method (ES-PFEM) to discretize the motion of a closed curve under surface diffusion with an anisotropic surface energy $\gamma(\theta)$ -- anisotropic surface diffusion -- in two…

数值分析 · 数学 2021-10-26 Yifei Li , Weizhu Bao

We analyze the resonance energy transfer (RET) rate between quantum emitters (QEs) near a phosphorene/SiC interface under the effects of uniaxial strain. Using a low-energy tight-binding model, we describe the electronic structure of…

介观与纳米尺度物理 · 物理学 2025-05-20 J. Oliveira-Cony , C. Farina , P. P. Abrantes , Tarik P. Cysne

The flame transfer function (FTF) relates acoustic perturbations and the coherent heat release rate response. This frequency-dependent function governs the thermoacoustic stability of a combustor. The FTF measurement is therefore of great…

流体动力学 · 物理学 2025-01-23 Bayu Dharmaputra , Pushkin Nagpure , Matteo Impagnatiello , Nicolas Noiray

We investigate the resonance energy transfer (RET) rate between two quantum emitters near a suspended graphene sheet in vacuum under the influence of an external magnetic field. We perform the analysis for low and room temperatures and show…

介观与纳米尺度物理 · 物理学 2021-05-26 P. P. Abrantes , G. Bastos , D. Szilard , C. Farina , F. S. S. Rosa

A numerically exact path integral treatment of the absorption and emission spectra of open quantum systems is presented that requires only the straightforward solution of a stochastic differential equation. The approach converges rapidly…

化学物理 · 物理学 2015-05-05 Jeremy Moix , Jian Ma , Jianshu Cao

Fluorescence spectroscopy and modeling provide powerful means to characterize biomacromolecular structures, dynamics, and interactions. F\"orster resonance energy transfer serves as a key technique for this due to its nanometer-scale…

生物物理 · 物理学 2026-02-26 Thomas-Otavio Peulen , Daria Maksutova , Thorben Cordes

Electronic energy transfer in the condensed phase, such as that occurring in photosynthetic complexes, frequently occurs in regimes where the energy scales of the system and environment are similar. This situation provides a challenge to…

统计力学 · 物理学 2015-06-03 Timothy C. Berkelbach , Thomas E. Markland , David R. Reichman

Foerster and modified Redfield theories play one of the central roles in the description of excitation energy transfer in molecular systems. However, in the present state, these theories describe only the dynamics of populations of local…

化学物理 · 物理学 2020-01-29 Anton Trushechkin

A simplified differential reactor model that embodies the essential physics controlling PEM fuel cell (PEM-FC) dynamics is presented. A remarkable analogy exists between water management in the differential PEM-FC and energy balance in the…

混沌动力学 · 物理学 2016-09-08 Ee-Sunn J. Chia , Jay B. Benziger , Ioannis G. Kevrekidis

We report an experimental study of the plasmon-assisted spontaneous emission and the F\"orster resonance energy transfer between organic molecules and semiconductor colloidal quantum dots. The localized plasmonic field in the nanogap…

光学 · 物理学 2018-07-25 Hassnain Asgar , Liyan Jacob , Thang Ba Hoang

A numerical modeling study based on 3D finite element method (FEM) simulation and 1D analytical solutions has been carried out to evaluate the capabilities of two ac methods for measuring in-plane thermal conductivity of thin film deposited…

应用物理 · 物理学 2020-12-22 Hanfu Wang , Yanjun Guo , Kaiwu Peng , Weiguo Chu , Guangming Chen

Multiplexed, real-time fluorescence detection at the single-molecule level is highly desirable to reveal the stoichiometry, dynamics, and interactions of individual molecular species within complex systems. However, traditionally…

Conversion of solar energy with high quantum efficiencies is a key challenge in energy technologies. Excitation energy transfer (EET) mechanisms, such as F\"orster resonance energy transfer (FRET), play a crucial role in facilitating…

We have constructed an approximate microscopic model for the neutron dynamic structure factor of solid methane in phase II. We expect our model to apply for neutron energies below 1\textit{eV} at pressures near 1 bar and temperatures below…

原子物理 · 物理学 2008-08-21 Yunchang Shin , W. Mike Snow , Chen-yu Liu , Christopher M. Lavelle , David V. Baxter

A method is presented for the sensing of water hardness by determining the concentration of calcium and magnesium in water, based on Fluorescence resonance energy transfer (FRET) process. The principle of the proposed sensor is based on the…

材料科学 · 物理学 2014-09-16 Dibyendu Dey , D. Bhattacharjee , S. Chakraborty , Syed Arshad Hussain