中文

Polymer translocation through a nanopore under a pulling force

软凝聚态物质 2007-06-27 v3 统计力学

摘要

We investigate polymer translocation through a nanopore under a pulling force using Langevin dynamics simulations. We concentrate on the influence of the chain length NN and the pulling force FF on the translocation time τ\tau. The distribution of τ\tau is symmetric and narrow for strong FF. We find that τN2\tau\sim N^{2} and translocation velocity vN1v\sim N^{-1} for both moderate and strong FF. For infinitely wide pores, three regimes are observed for τ\tau as a function of FF. With increasing FF, τ\tau is independent of FF for weak FF, and then τF2+ν1\tau\sim F^{-2+\nu^{-1}} for moderate FF, where ν\nu is the Flory exponent, which finally crosses over to τF1\tau\sim F^{-1} for strong force. For narrow pores, even for moderate force τF1\tau\sim F^{-1}. Finally, the waiting time, for monomer ss and monomer s+1s+1 to exit the pore, has a maximum for ss close to the end of the chain, in contrast to the case where polymer is driven by an external force within the pore.

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引用

@article{arxiv.cond-mat/0608499,
  title  = {Polymer translocation through a nanopore under a pulling force},
  author = {Ilkka Huopaniemi and Kaifu luo and Tapio Ala-Nissila and See-Chen Ying},
  journal= {arXiv preprint arXiv:cond-mat/0608499},
  year   = {2007}
}

备注

submitted, 7 pages with 5 figures. To appear in PRE