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We consider solid surface scattering of molecules that were subject to strong non-resonant ultrashort laser pulses just before hitting the surface. The pulses modify the rotational states of the molecules, causing their field free…

Chemical Physics · Physics 2015-06-12 Yuri Khodorkovsky , J. R. Manson , Ilya Sh. Averbukh

The rotation measure (RM) and dispersion measure (DM) of fast radio bursts (FRBs) serve as critical probes of the magneto-ionic environments along the line of sight. The significant temporal evolution of RM observed in some repeating FRBs…

High Energy Astrophysical Phenomena · Physics 2026-04-29 Qing Zhao , Di Xiao , Xue-Feng Wu

We investigate spontaneous four wave mixing (SFWM) in a single-channel side-coupled integrated spaced sequence of resonators (SCISSOR). Analytic expressions for the number of photon pairs generated, as well as the biphoton wave function…

Quantum Physics · Physics 2016-04-27 T. Onodera , Marco Liscidini , J. E. Sipe , L. G. Helt

We present a novel semicoherent targeted search method for continuous gravitational waves (CWs) emitted by pulsars in binary systems. The method is based on a custom optimization of the coherence time, which is tailored according to the…

We propose and computationally study a method for simultaneously orienting the angular momentum of asymmetric top molecules along: 1) a laboratory-fixed direction; 2) the molecular intermediate moment of inertia axis; 3) the laser field…

Quantum Physics · Physics 2022-11-21 Emil J. Zak

We investigate dynamics of resonantly excited excitons in single-layers of MoSe$_2$ and WS$_2$ down to 4.5 K. To this end, we measure the delay dependence of the heterodyne four-wave mixing (FWM) amplitude induced by three, short laser…

Mesoscale and Nanoscale Physics · Physics 2020-02-06 Tomasz Jakubczyk , Miroslav Bartos , Karol Nogajewski , Lorenzo Scarpelli , Wolfgang Langbein , Marek Potemski , Jacek Kasprzak

We theoretically investigate a N-type 87Rb atomic system for efficient generation and control of a non-degenerate Four wave mixing (FWM) signal in pulsed regime. The susceptibility of the atomic medium is customized as a gain profile by a…

Optics · Physics 2023-06-29 Nawaz Sarif Mallick , Sankar De

Ultrafast lasers have become one of the most powerful tools in coherent nonlinear optical spectroscopy. Short pulses enable direct observation of fast molecular dynamics, whereas broad spectral bandwidth offers ways of controlling nonlinear…

Chemical Physics · Physics 2015-05-13 X. G. Xu , S. O. Konorov , J. W. Hepburn , V. Milner

We present a simple technique for studying collisions of ultracold atoms in the presence of a magnetic field and radio-frequency radiation (rf). Resonant control of scattering properties can be achieved by using rf to couple a colliding…

Quantum Gases · Physics 2010-09-28 Thomas M. Hanna , Eite Tiesinga , Paul S. Julienne

In this work, we observe a novel resonant mechanism, namely the modulation-induced Feshbach resonance. By applying a far-detuned laser to the cesium D2 transition with intensity modulation, we periodically shake the energy levels of atomic…

Quantum Physics · Physics 2025-12-30 Tongkang Wang , Yuqi Liu , Jundong Wang , Youjia Huang , Wenlan Chen , Zhendong Zhang , Jiazhong Hu

By implementing four-wave mixing (FWM) micro-spectroscopy we measure coherence and population dynamics of the exciton transitions in monolayers of MoSe$_2$. We reveal their dephasing times T$_2$ and radiative lifetime T$_1$ in a…

We study theoretically the nonlinear four wave mixing (FWM) response of an ensemble of coupled pairs of quantum dots (quantum dot molecules). We discuss the shape of the FWM echo signal depending on the parameters of the ensemble: the…

Mesoscale and Nanoscale Physics · Physics 2007-10-24 A. Sitek , P. Machnikowski

Nonlinear wave mixing in the X-ray range can provide valuable insights into the structural and electron dynamics of atomic and molecular systems on ultrafast time scales, with state- and site-selectivity and atomic resolution. This…

We investigate the femtosecond kinetics of an optically excited 2D magneto-plasma at intermediate and high densities under a strong magnetic field perpendicular to the quantum well (QW). We assume an additional weak lateral confinement…

Condensed Matter · Physics 2009-10-31 M. W. Wu , H. Haug

Improving resolution and sensitivity will widen possible medical applications of magnetic particle imaging. Pulsed excitation promises such benefits, at the cost of more complex hardware solutions and restrictions on drive field amplitude…

We report on coherent control of excitation processes of translationally ultracold rubidium dimers in a magneto-optical trap by using shaped femtosecond laser pulses. Evolution strategies are applied in a feedback loop in order to optimize…

A quasi-classical model (QCM) of molecular dynamics in intense femtosecond laser fields has been developed, and applied to a study of the effect of an ultrashort `control' pulse on the vibrational motion of a deuterium molecular ion in its…

Quantum Physics · Physics 2010-07-22 W A Bryan , C R Calvert , R B King , G R A J Nemeth , J B Greenwood , I D Williams , W R Newell

The chemical and physical properties of molecular clusters can heavily depend on their size, which makes them very attractive for the design of new materials with tailored properties. Deriving the structure and dynamics of clusters is…

We measure molecular vibrations with femtometer precision using time-resolved x-ray absorption spectroscopy. For a demonstration, a Raman process excites the A$_{1g}$ mode in gas-phase SF$_6$ molecules with an amplitude of $\approx50$ fm,…

Recently, a method to image molecular electronic wave functions using high harmonic generation (HHG) was introduced by Itatani \textit{et al.\} [Nature {\textbf{432}}, 876 (2004)]. We show that, while the tomographic reconstruction of…

Atomic Physics · Physics 2009-11-13 Elmar V. van der Zwan , Ciprian C. Chirilă , Manfred Lein