Related papers: Rotational Control and Selective Isotope Alignment…
Control over various fragmentation reactions of a series of polyatomic molecules (acetylene, ethylene, 1,3-butadiene) by the optical waveform of intense few-cycle laser pulses is demonstrated experimentally. We show both experimentally and…
We propose and demonstrate localized mode coupling as a viable dispersion engineering technique for phase-matched resonant four-wave mixing (FWM). We demonstrate a dual-cavity resonant structure that employs coupling-induced frequency…
The resonant filtering method transforming frequency modulated radiation field into a train of short pulses is proposed to apply in optical domain. Effective frequency modulation can be achieved by electro-optic modulator or by resonant…
We theoretically analyze the effectiveness of multiple-pulse laser alignment methods for asymmetric-top molecules. As an example, we choose SO_2 and investigate the alignment dynamics induced by two different sequences, each consisting of…
Light travel time changes due to gravitational waves may be detected within the next decade through precision timing of millisecond pulsars. Removal of frequency-dependent interstellar medium (ISM) delays due to dispersion and scattering is…
The rotational echo response of molecules is found to strongly depend on the delay between the two ultrashort laser pulses, as opposed to two-level systems. We study this dependence experimentally and theoretically and show that by…
We demonstrate the experimental realization of impulsive alignment of carbonyl sulfide (OCS) molecules at the Low Density Matter Beamline (LDM) at the free-electron laser FERMI. OCS molecules in a molecular beam were impulsively aligned…
Recently, it was predicted theoretically and verified experimentally that a pair of delayed and cross-polarized short laser pulses can create molecular ensembles with a well defined sense of rotation (clockwise or counterclockwise). Here we…
A new carrier-based pulse-width modulation (PWM) technique to control power inverters is presented in this paper. To generate the output waveform, this technique compares a harmonic-injection modulating wave and a frequency-modulated…
We propose a laser isotope separation mechanism in which selectivity arises from nuclear spin rather than isotope shifts, enabling the use of broadband ultrafast lasers. A Ramsey pulse sequence is applied to paramagnetic molecular…
Nonlinear waveguides with two distinct domains of anomalous dispersion can support the formation of molecule-like two-color pulse compounds. They consist of two tightly bound subpulses with frequency loci separated by a vast frequency gap.…
We theoretically demonstrate the possibility to tune the temporal waveform of optical unipolar pulses upon their coherent interaction with a multi-level resonant medium. This is achieved through the coherent control of the response of a…
We employ pulse shaping to abate single-qubit gate errors arising from the weak anharmonicity of transmon superconducting qubits. By applying shaped pulses to both quadratures of rotation, a phase error induced by the presence of higher…
We show that the decays with pressure of the alignment echoes induced in N2O-He gas mixtures by two laser pulses with various delays bring detailed information on collision-induced changes of the rotational speed. Measurements and…
The possibility of achieving highly selective excitation of low metastable states of hydrogen and helium atoms by using short laser pulses with reasonable parameters is demonstrated theoretically. Interactions of atoms with the laser field…
We describe how active feedback routines can be applied at limited repetition rate (5 Hz) to optimize high-power $>10$ TW) laser interactions with clustered gases. Optimization of x-ray production from an argon cluster jet, using a genetic…
The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…
We illustrate an iterative method for retrieving the internuclear separations of N$_2$, O$_2$ and CO$_2$ molecules using the high-order harmonics generated from these molecules by intense infrared laser pulses. We show that accurate results…
Four-wave mixing (FWM) is an efficient source of light waves emitted at various frequencies, usually associated with third-order optical nonlinearities. Whereas attention has mostly been paid in the past to the generation of Stokes (e.g.,…
Many experiments in biological and medical sciences currently use multiphoton microscopy as a core imaging technique. To date, solid-state lasers are most commonly used as excitation beam sources. However, the most demanding applications…