Related papers: Rotational Control and Selective Isotope Alignment…
We propose a mechanism to produce a superposition of atomic and molecular states by a train of ultrashort laser pulses combined with weak control fields. By adjusting the repetition rate of the pump pulses and the intensity of the coupling…
A general method for rotational microwave spectroscopy and control of polar molecular ions via direct microwave addressing is considered. Our method makes use of spatially varying AC Stark shifts, induced by far off-resonant, focused laser…
High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…
This work theoretically investigates high-order harmonic generation in rare gas atoms driven by two temporally delayed ultrashort laser pulses. Apart from their temporal delay, the two pulses are identical. Using a single-atom model of the…
We experimentally demonstrate shaping of the two-photon wavefunction of entangled photon-pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the two-photon wavefunction exactly like a…
The impulsive limit (the "sudden approximation") has been widely employed to describe the interaction between molecules and short, far-off-resonant laser pulses. This approximation assumes that the timescale of the laser--molecule…
Accurately modeling the inspiral-merger-ringdown (IMR) signal of coalescing compact objects is essential for the test of general relativity. However, it is known that astrophysical environments can distort gravitational-wave (GW) signal…
When circularly polarized light is scattered from a rotating target, a rotational Doppler shift (RDS) emerges from an exchange of angular momentum between the spinning object and the electromagnetic field. Here, we used coherently spinning…
Excited-state vibrational dynamics in molecules can be studied by an electronically off-resonant Raman process induced by a probe pulse with variable delay with respect to an actinic pulse. We establish the connection between several…
Vibrational spectroscopy is a cornerstone technique for molecular characterization and offers an ideal target for the computational investigation of molecular materials. Building on previous comprehensive assessments of efficient methods…
We have carried out a unified microscopic study of electric monopole, quadrupole and magnetic dipole excitations in fast rotating nuclei undergoing backbending, with special attention at the magnetic excitations. We found, among other…
We experimentally demonstrate the manipulation of two-orthogonal components of a spin wave in an atomic ensemble. Based on Raman two-photon transition and Larmor spin precession induced by magnetic field pulses, the coherent rotations…
An all-optical method of ultrafast spin rotation is put forward to precisely manipulate the polarization of relativistic charged particle beams of leptons or ions. In particular, laser-driven dense ultrashort beams are manipulated via…
We present a concept for selective excitation of magnetostatic surface waves with quasi-discrete spectrum using spatially patterned femtosecond laser pulses inducing either ultrafast change of magnetic anisotropy or inverse Faraday effect.…
On the basis of optimal control theory, we numerically study how to optimally manipulate molecular vibrational dynamics by using cycle-averaged polarizability interactions induced by mildly intense non-resonant laser (NR) pulses. As the…
We derive composite pulse sequences that achieve high-fidelity excitation of two-state systems in an optically dense, inhomogeneously broadened ensemble. The composite pulses are resistant to distortions due to the back-action of the medium…
It is predicted that nuclear spin conversion in molecules can be efficiently controlled by strong laser radiation resonant to rovibrational molecular transition. The phenomenon can be used for substantial enrichment of spin isomers, or for…
The parametric optimization for the ultrasound computed tomography system is introduced. It is hypothesized that the pulse characteristic directly affects the information present in the reconstructed profile. The ultrasound excitation modes…
PulsePol is an elegantly designed pulse-sequence-based quantum control scheme that enables polarization transfer between electron and nuclear spins, for example, in nitrogen-vacancy (NV) centers. However, previous analyses of PulsePol…
Infrared vibrational spectroscopy in the gas phase has emerged as a powerful tool to determine complex molecular structures with Angstrom accuracy. Among the different approaches IRMPD (InfraRed Multiple Photon Dissociation), which requires…