Related papers: Rotational Control and Selective Isotope Alignment…
Compact silicon integrated devices, such as micro-ring resonators, have recently been demonstrated as efficient sources of quantum correlated photon pairs. The mass production of integrated devices demands the implementation of fast and…
A comprehensive theoretical approach to describe the electron-ion radiative recombination in the presence of intense, short laser pulses, which accounts for nondipole corrections is presented. It is based on the relativistic Coulomb-Volkov…
A new and efficient method for orientation echo spectroscopy is presented and realized experimentally. The excitation scheme utilizes concerted rotational excitations by both ultrashort terahertz and near-IR pulses and its all-optical…
We propose and experimentally validate the use of rotational echo responses for obtaining the degree of molecular alignment induced in a gas. The method is independent of various parameters that are hardly accessible in most experimental…
We demonstrate direct time-domain observation of l-doubling contributions in molecular rotational dynamics using shaped femtosecond laser pulses. By imposing a tailored spectral phase on the excitation pulse, we pre-compensate centrifugal…
The lack of a direct map between control fields and desired control objectives poses a significant challenge in applying quantum control theory to quantum technologies. Here, we propose an analytical framework to precisely control a limited…
Following up on a proposal to use four-wave mixing in an underdense plasma at mildly relativistic laser intensities to produce vastly more energetic x-ray pulses [V. M. Malkin and N. J. Fisch, Phys. Rev. E, 101, 023211 (2020)], we perform…
A fundamental goal in the manipulation of quantum systems is the achievement of many coherent oscillations within the characteristic dephasing time T2*[1]. Most manipulations of electron spins in quantum dots have focused on the…
Ultrafast lasers generating high repetition rate ultrashort pulses through various mode-locking methods can benefit many important applications including communication, materials processing, astronomical observation, etc. For decades,…
A pulse shaping algorithm for a matter wave with the purpose of controlling a binary reaction has been designed. The scheme is illustrated for an Eley-Rideal reaction where an impinging matter-wave atom recombines with an adsorbed atom on a…
We employ two-dimensional (2D) coherent, nonlinear spectroscopy to investigate couplings within individual InAs quantum dots (QD) and QD molecules. Swapping pulse ordering in a two-beam sequence permits to distinguish between rephasing and…
Ultrashort laser pulses carrying orbital angular momentum (OAM) have become essential tools in Atomic, Molecular, and Optical (AMO) studies, particularly for investigating strong-field light-matter interactions. However, controlling and…
We show that the precise preparation of a quantum superposition between three rotational states of an ultracold dipolar molecule generates controllable interferences in their two-body scattering dynamics and collisional rate coefficients,…
Exploring intermixing and interplay between different frequency-mixing processes has always been one of the interesting subjects at the interface of nonlinear optics with quantum optics. Here we investigate coherent competition and control…
Intense terahertz-frequency pulses induce coherent rotational dynamics and orientation of polar molecular ensembles. Exact numerical methods for rotational dynamics are computationally not feasible for the vast majority of molecular rotors…
Four-wave mixing (FWM) in gas-filled hollow-core capillaries, a nonlinear optical process that mixes signal and pump photon frequencies to generate idler frequency photons, offers a method for precise spectral phase transfer from signal to…
The spectrum of a CW field whose phase experiences a periodic sawtooth modulation is analyzed. Two types of the sawtooth phase modulation are considered. One is created by combining many harmonics of the fundamental frequency. The second is…
We introduce a new scheme for generating short-wavelength coherent broadband radiation with well-controlled spectral characteristics. It is based on shaping long-wavelength femtosecond pulse to coherently control atomic resonance-mediated…
We demonstrate numerically a method of focusing two-photon field inside one-dimensional random media. The approach is based on coherent control of backscattering achieved by adaptive spectral pulse shaping. The spectral phases of a…
We develop energy efficient, continuous microwave schemes to couple electron and nuclear spins, using phase or amplitude modulation to bridge their frequency difference. These controls have promising applications in biological systems,…