Related papers: Rotational Control and Selective Isotope Alignment…
Four-wave mixing (FWM) is an important nonlinear optical phenomenon that underlines many of the discoveries and device applications since the laser was invented. Examples include parametric amplification, mode-locked pulses and frequency…
Coherent control with shaped ultrafast pulses is a powerful approach for steering nonlinear light-matter interactions. Previous studies in quantum control have shown that, beyond transform-limited pulses, those with antisymmetric spectral…
We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort…
The paper presents an improved mass balancing procedure for fast rotating machinery, while it is being rotated at speeds considerably slower than the "critical speeds", where dangerously high vibration amplitudes may arise. By utilizing…
Coherent control of individual two-level systems (TLSs) is at the basis of any implementation of quantum information. An impressive level of control is now achieved using nuclear, vacancies and charge spins. Manipulation of bright exciton…
We propose a method to reconstruct the vibrational quantum state of molecules excited by a general excitation laser pulse. Unlike existing methods, we do not require the molecules before excitation to be in a pure state, allowing us to…
Trains of ultrashort laser pulses separated by the time of rotational revival (typically, tens of picoseconds) have been exploited for creating ensembles of aligned molecules. In this work we introduce a chiral pulse train - a sequence of…
We use R-Matrix with Time-dependence (RMT) theory, with spin-orbit effects included, to study krypton irradiated by two time-delayed XUV ultrashort pulses. The first pulse excites the atom to 4s$^{2}$4p$^{5}$5s. The second pulse then…
An efficient technique to produce a periodic sequence of ultrashort pulses of recoilless gamma-radiation via its transmission through the optically thick vibrating resonant absorber was demonstrated recently [Nature, 508, 80 (2014)]. In…
The four-wave mixing produced with two ultrashort phase-locked w-3w laser pulses propagating coherently in a two-level system in the infrared spectral region is shown to depend on the pulses relative phase. The Maxwell-Bloch equations are…
Precise control of hyperfine matterwaves via Raman excitations is instrumental to a class of atom-based quantum technology. We investigate the Raman spinor control technique for alkaline atoms in an intermediate regime of single-photon…
The extension of nonlinear spectroscopic techniques into the x-ray domain is in its infancy but holds the promise to provide unique insight into the dynamics of charges in photoexcited processes, which are of fundamental as well as applied…
A new approach to all-optical detection and control of the coupling between electric and magnetic order on ultrafast timescales is achieved using time-resolved second harmonic generation (SHG) to study a ferroelectric (FE)/ferromagnet (FM)…
Short laser pulses are widely used for controlling molecular rotational degrees of freedom and inducing molecular alignment, orientation, unidirectional rotation and other types of coherent rotational motion. To follow the ultra-fast…
A detailed understanding of the population and coherence dynamics in optically driven individual emitters in solids and their signatures in ultrafast nonlinear-optical signals is of prime importance for their applications in future quantum…
We provide a detailed theoretical analysis of molecular rotational excitation by a chiral pulse train -- a sequence of linearly polarised pulses with the polarisation direction rotating from pulse to pulse by a controllable angle. Molecular…
We report a method for coherent control of $\gamma$-photons, enabling the shaping of $\gamma$-ray intensity in nearly arbitrary waveforms. Different intensity waveforms are created by adjusting the motion profile of a resonant absorber (an…
We present an efficient scheme for the generation and control of a degenerate four-wave mixing (FWM) signal in a N-type inhomogeneously broadened 85Rb atomic system. We observe the propagation dynamics of the generated FWM signal along with…
Fast Radio Bursts (FRBs), a class of millisecond-scale, highly energetic phenomena with unknown progenitors and radiation mechanisms, require proper statistical analysis as a key method for uncovering their mysteries. In this research, we…
Abstract We report the experimental observation of molecular unidirectional rotation (UDR) echoes, and analyze their origin and behavior both classically and quantum mechanically. The molecules are excited by two time-delayed…