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Alpha-phase (a-) RuCl_3 has emerged as a prime candidate for a quantum spin liquid (QSL) that promises exotic quasiparticles relevant for fault-tolerant quantum computation. Here, we report spin sensitive transport measurements to probe…

Strongly Correlated Electrons · Physics 2026-04-27 H. Idzuchi , M. Kimata , S. Okamoto , P. Laurell , N. Mohanta , M. Cothrine , S. E. Nagler , D. Mandrus , A. Banerjee , Y. P. Chen

The exactly-solvable Kitaev model of two-dimensional honeycomb magnet leads to a quantum spin liquid (QSL) characterized by Majorana fermions, relevant for fault-tolerant topological quantum computations. In the high-field paramagnetic…

Strongly Correlated Electrons · Physics 2022-09-13 O. Tanaka , Y. Mizukami , R. Harasawa , K. Hashimoto , K. Hwang , N. Kurita , H. Tanaka , S. Fujimoto , Y. Matsuda , E. -G. Moon , T. Shibauchi

While phase transitions between magnetic analogs of three states of matter --- a long-range ordered state, paramagnet, and spin liquid --- have been extensively studied, the possibility of "liquid-liquid" transitions, namely, between…

Strongly Correlated Electrons · Physics 2017-04-05 Joji Nasu , Yasuyuki Kato , Junki Yoshitake , Yoshitomo Kamiya , Yukitoshi Motome

The layered honeycomb magnet $\alpha$-RuCl$_3$ has attracted intense scrutiny as a prime candidate for realizing the Kitaev quantum spin liquid, yet a consensus on its microscopic Hamiltonian remains elusive due to the material's extreme…

Recently, there have been increasingly hot debates on whether there exists a quantum spin liquid in the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ in high magnetic field. To investigate this issue, we perform the ultralow-temperature thermal…

Strongly Correlated Electrons · Physics 2018-02-14 Y. J. Yu , Y. Xu , K. J. Ran , J. M. Ni , Y. Y. Huang , J. H. Wang , J. S. Wen , S. Y. Li

Organic solids host various electronic phases. Especially, a milestone compound of organic solid, $\beta'$-$X$[Pd(dmit)$_2$]$_2$ with $X$=EtMe$_3$Sb shows quantum spin-liquid (QSL) properties suggesting a novel state of matter. However,…

Strongly Correlated Electrons · Physics 2022-04-29 Kota Ido , Kazuyoshi Yoshimi , Takahiro Misawa , Masatoshi Imada

Quantum spin liquid (QSL) has become an exciting topic in interacting spin systems that do not order magnetically down to the lowest experimentally accessible temperature; however, conclusive experimental evidence remains lacking. Motivated…

Strongly Correlated Electrons · Physics 2023-10-26 Saikat Banerjee , Wei Zhu , Shi-Zeng Lin

The Kitaev model, which hosts a quantum spin liquid (QSL) in the ground state, was originally defined on a two-dimensional honeycomb lattice, but can be straightforwardly extended to any tricoordinate lattices in any spatial dimensions. In…

Strongly Correlated Electrons · Physics 2023-05-29 Kiyu Fukui , Yasuyuki Kato , Yukitoshi Motome

Quantum spin liquids are long-range entangled states of matter with emergent gauge fields and fractionalized excitations. While candidate materials, such as the Kitaev honeycomb ruthenate $\alpha$-RuCl$_3$, show magnetic order at low…

Strongly Correlated Electrons · Physics 2019-07-16 I. Rousochatzakis , S. Kourtis , J. Knolle , R. Moessner , N. B. Perkins

$\alpha$-RuCl$_{3}$ is a major candidate for the realization of the Kitaev quantum spin liquid, but its zigzag antiferromagnetic order at low temperatures indicates deviations from the Kitaev model. We have quantified the spin Hamiltonian…

Quantum antiferromagnets on geometrically frustrated lattices have long attracted interest for the formation of quantum disordered states and the possible emergence of quantum spin liquid (QSL) ground states. Here we turn to the…

Strongly Correlated Electrons · Physics 2023-12-21 Lasse Gresista , Ciarán Hickey , Simon Trebst , Yasir Iqbal

Thermodynamics of the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ is studied for different directions of in-plane magnetic field using measurements of the magnetic Gr\"uneisen parameter $\Gamma_B$ and specific heat $C$. We identify two…

Strongly Correlated Electrons · Physics 2021-03-03 S. Bachus , D. A. S. Kaib , A. Jesche , V. Tsurkan , A. Loidl , S. M. Winter , A. A. Tsirlin , R. Valentí , P. Gegenwart

The honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ has recently been proposed as a candidate material for hosting field-induced quantum spin liquid (QSL) behavior. Here, we present a comprehensive thermodynamic study of its low-temperature,…

The honeycomb magnet $\alpha$-RuCl$_{3}$ has been a leading candidate for realizing the Kitaev quantum spin liquid (QSL), but its intrinsic spin dynamics have remained obscured by crystal twinning. Here we apply biaxial anisotropic strain…

Recently there has been considerable excitement surrounding the promising realization of high-spin Kitaev material, such as the quasi-2D compound CrI$_3$ and CrGeTe$_3$. However, the stability of quantum spin liquids (QSL) against single…

Strongly Correlated Electrons · Physics 2025-04-01 Gui-Xin Liu , Ting-Long Wang , Yi-Fan Jiang

Thermal signatures of fractionalized excitations are a fingerprint of quantum spin liquids (QSLs). In the $J_{eff}=1/2$ honeycomb magnet $\alpha$-RuCl$_3$, a QSL state emerges upon applying an in-plane magnetic field $H_{||}$ greater than…

Strongly Correlated Electrons · Physics 2022-06-01 J. A. N. Bruin , R. R. Claus , Y. Matsumoto , N. Kurita , H. Tanaka , H. Takagi

Recently H$_3$LiIr$_2$O$_6$ has been reported as a spin-orbital entangled quantum spin liquid (QSL) [K. Kitagawa et al., Nature {\bf 554}, 341 (2018)], albeit its connection to Kitaev QSL has not been yet identified. To unveil the related…

Strongly Correlated Electrons · Physics 2020-05-13 Shenghai Pei , Liang-Long Huang , Gaomin Li , Xiaobin Chen , Bin Xi , XinWei Wang , Youguo Shi , Dapeng Yu , Cai Liu , Le Wang , Fei Ye , Mingyuan Huang , Jia-Wei Mei

The search for quantum spin liquids (QSL) -- topological magnets with fractionalized excitations -- has been a central theme in condensed matter and materials physics. While theories are no longer in short supply, tracking down materials…

Strongly Correlated Electrons · Physics 2022-05-11 Anish Bhardwaj , Shu Zhang , Han Yan , Roderich Moessner , Andriy H. Nevidomskyy , Hitesh J. Changlani

Layered $\alpha$-RuCl3 has been discussed as a proximate Kitaev spin liquid compound. Raman and THz spectroscopy of magnetic excitations confirm that the low-temperature antiferromagnetic ordered phase features a broad Raman continuum,…

Topological spin liquids in two spatial dimensions are stable phases in the presence of a small magnetic field, but may give way to field-induced phenomena at intermediate field strengths. Sandwiched between the low-field spin liquid…

Strongly Correlated Electrons · Physics 2021-02-17 Ciarán Hickey , Matthias Gohlke , Christoph Berke , Simon Trebst