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The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle

We report on terahertz spectroscopy of quantum spin dynamics in $\alpha$-RuCl$_3$, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. An extended magnetic continuum develops below the…

Strongly Correlated Electrons · Physics 2017-11-30 Zhe Wang , S. Reschke , D. Hüvonen , S. -H. Do , K. -Y. Choi , M. Gensch , U. Nage , T. Rõõm , A. Loidl

In $\alpha$-RuCl$_3$, an external magnetic field applied within the honeycomb plane can induce a transition from a magnetically ordered state to a disordered state that is potentially related to the Kitaev quantum spin liquid. In zero…

High-resolution thermal expansion and magnetostriction measurements were performed on single crystals of $\alpha$-RuCl$_3$ in magnetic fields applied parallel to the Ru-Ru bonds. The length changes were measured in the direction…

A quantum spin liquid (QSL) is a state of matter characterized by fractionalized quasiparticle excitations, quantum entanglement, and a lack of long-range magnetic order. However, QSLs have evaded definitive experimental observation.…

Strongly Correlated Electrons · Physics 2024-12-31 Sangyun Lee , Andrew J. Woods , Minseong Lee , Shengzhi Zhang , Eun Sang Choi , A. O. Scheie , D. A. Tennant , J. Xing , A. S. Sefat , R. Movshovich

Recent studies have brought $\alpha$-RuCl$_3$ to the forefront of experimental searches for materials realizing Kitaev spin-liquid physics. This material exhibits strongly anisotropic exchange interactions afforded by the spin-orbit…

Strongly Correlated Electrons · Physics 2018-02-21 Stephen M. Winter , Kira Riedl , David Kaib , Radu Coldea , Roser Valenti

Quantum spin liquids (QSL) have generated considerable excitement as phases of matter with emergent gauge structures and fractionalized excitations. In this context, phase transitions out of QSLs have been widely discussed as Higgs…

Strongly Correlated Electrons · Physics 2021-09-15 Hyeok-Jun Yang , Nic Shannon , SungBin Lee

The Kitaev model predicts that quantum spin liquids (QSLs) will form at low temperatures under certain special conditions, and materials hosting the QSL state are frequently sought. The layered honeycomb lattice material {\alpha}-RuCl3 has…

Materials Science · Physics 2022-01-24 Danrui Ni , Xin Gui , Kelly M. Powderly , R. J. Cava

{\alpha}-RuCl3 is a Kitaev material suggested to be a proximate quantum spin liquid in a certain temperature and magnetic field range. Nonequilibrium measurements of transient dynamics have been proposed to detect fractionalized particles…

Strongly Correlated Electrons · Physics 2024-08-23 Haochen Zhang , Subin Kim , Young-June Kim , Hae-Young Kee , Luyi Yang

Inspired by experiments on the magnetic field induced phases of the spin-orbit coupled $2d$ Mott insulator $\alpha$-RuCl$_3$, we study some general aspects of gapped $Z_2$ Quantum Spin Liquids (QSL) enriched by lattice translation symmetry.…

Strongly Correlated Electrons · Physics 2022-07-25 Xue-Yang Song , T. Senthil

The Kitaev model belongs to an unconventional class of two-dimensional spin systems characterized by anisotropic, bond-dependent interactions that give rise to Quantum Spin Liquid (QSL) states. These exotic phases, marked by the absence of…

Strongly Correlated Electrons · Physics 2026-01-29 A. R. Moura , L. V. Santos

The quantum spin liquid (QSL) is an exotic phase of magnetic materials where the spins continue to fluctuate without any symmetry breaking down to zero temperature. Among the handful reports of QSL with spin $S\ge$1, examples with magnetic…

Quantum spin liquids (QSLs) are topologically ordered exotic states of matter that host fractionalized excitations. Kitaev proposed a particular route towards a QSL via strongly bond-dependent interactions on the hexagonal lattice. A number…

Strongly Correlated Electrons · Physics 2022-12-06 Xinshu Zhang , Yuanyuan Xu , T. Halloran , Ruidan Zhong , R. J. Cava , C. Broholm , N. Drichko , N. P. Armitage

We found a plateau in the magnitude of the isolated magnetic moments as a function of the anisotropy of the transfer integral (t'/t) in the gapless quantum spin liquid (QSL) phase of an S=1/2 triangular lattice molecular solid X[Pd(dmit)2]2…

Strongly Correlated Electrons · Physics 2024-03-20 K. Ueda , S. Fujiyama , R. Kato

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…

Strongly Correlated Electrons · Physics 2025-05-09 Willian Natori , Yang Yang , Hui-Ke Jin , Johannes Knolle , Natalia B. Perkins

We investigate the possibility of exotic phenomena, viz. quantum spin liquid (QSL) or deconfined quantum critical point (DQCP), in the spin-$\frac{1}{2}$ Heisenberg model on the maple-leaf lattice, a geometrically frustrated system formed…

Strongly Correlated Electrons · Physics 2024-01-18 Pratyay Ghosh

Quantum spin liquids (QSLs) host a variety of fractionalized particles. In Kitaev's paradigmatic honeycomb model a spin-$\tfrac{1}{2}$ fractionalizes into $Z_2$ flux due to emergent $Z_2$ gauge field and matter Majorana fermions. Although…

Strongly Correlated Electrons · Physics 2026-01-22 Shi Feng , Nandini Trivedi

Kitaev magnets are materials with bond-dependent Ising interactions between localized spins on a honeycomb lattice. Such interactions could lead to a quantum spin-liquid (QSL) ground state at zero temperature. Recent theoretical studies…

In the class of materials called spin liquids, a magnetically ordered state cannot be attained even at milliKelvin temperatures because of conflicting constraints on each spin (for e.g. from geometric or exchange frustration). The resulting…

Excitation by light pulses enables the manipulation of phases of quantum condensed matter. Here, we photoexcite high-energy holon-doublon pairs as a way to alter the magnetic free energy landscape of the Kitaev-Heisenberg magnet…