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Motivated by the possible triple-$\bf Q$ classical order in the Kitaev candidate material Na$_2$Co$_2$TeO$_6$, we investigate microscopic models that may stabilize the triple-$\bf Q$ order by studying an extended Kitaev honeycomb model with…

Strongly Correlated Electrons · Physics 2023-08-01 Jiucai Wang , Zheng-Xin Liu

Quantum spin liquids (QSLs) are exotic phases of matter characterized by long-range entanglement and the absence of magnetic order even at zero temperature. Here, we present a comprehensive theoretical study of the frustrated magnet…

Strongly Correlated Electrons · Physics 2026-03-20 Yanpeng Zhou , Gang Li

Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin…

Strongly Correlated Electrons · Physics 2025-12-15 Tony An , Félix Desrochers , Yong Baek Kim

Quantum materials exhibiting magnetic frustration are connected to diverse phenomena including high-Tc superconductivity, topological order and quantum spin liquids (QSLs). A QSL is a quantum phase (QP) related to a quantum-entangled…

Strongly Correlated Electrons · Physics 2021-08-03 Samuel Mañas-Valero , Benjamin Huddart , Tom Lancaster , Eugenio Coronado , Francis Pratt

A new quantum spin liquid (QSL) candidate material H$_{3}$LiIr$_{2}$O$_{6}$ was synthesized recently and was found not to show any magnetic order or phase transition down to low temperatures. In this work, we study the quantum dynamics of…

Strongly Correlated Electrons · Physics 2020-08-17 Shuai Wang , Long Zhang , Fa Wang

The Kitaev spin liquid, stabilized as the ground state of the Kitaev honeycomb model, is a paradigmatic example of a topological $\mathbb{Z}_2$ quantum spin liquid. The fate of the Kitaev spin liquid in presence of an external magnetic…

Strongly Correlated Electrons · Physics 2026-05-04 Will Holdhusen , Daniel Huerga , Gerardo Ortiz

One of the most important issues in modern condensed matter physics is the realization of fractionalized excitations, such as the Majorana excitations in the Kitaev quantum spin liquid. To this aim, the 3d-based Kitaev material Na2Co2TeO6…

A quantum spin liquid (QSL) is an exotic insulating phase with emergent gauge fields and fractionalized excitations. However, the unambiguous demonstration of the existence of a QSL in a "non-engineered" microscopic model (or in any…

Strongly Correlated Electrons · Physics 2025-10-01 Xun Cai , Zhaoyu Han , Zi-Xiang Li , Steven A. Kivelson , Hong Yao

Measurements of the magnetic Gr\"uneisen parameter ($\Gamma_B$) and specific heat on the Kitaev material candidate $\alpha$-RuCl$_3$ are used to access in-plane field- and temperature-dependence of the entropy up to 12 T and down to 1 K. No…

Strongly Correlated Electrons · Physics 2020-08-28 S. Bachus , D. A. S. Kaib , Y. Tokiwa , A. Jesche , V. Tsurkan , A. Loidl , S. M. Winter , A. A. Tsirlin , R. Valenti , P. Gegenwart

Maximizing the ratio between Kitaev and residual Heisenberg interactions is a major goal in nowadays research on Kitaev-Heisenberg quantum magnets. Here we investigate Kitaev-Heisenberg exchange in a recently discovered crystalline phase of…

Strongly Correlated Electrons · Physics 2023-12-15 Pritam Bhattacharyya , Liviu Hozoi , Quirin Stahl , Jochen Geck , Nikolay A. Bogdanov

The quasi two-dimensional Mott insulator $\alpha$-RuCl$_3$ is proximate to the sought-after Kitaev quantum spin liquid (QSL). In a layer of $\alpha$-RuCl$_3$ on graphene the dominant Kitaev exchange is further enhanced by strain. Recently,…

Strongly Correlated Electrons · Physics 2021-03-24 V. Leeb , K. Polyudov , S. Mashhadi , S. Biswas , Roser Valenti , M. Burghard , J. Knolle

In addition to the Kitaev ($K$) interaction, candidate Kitaev materials also possess Heisenberg ($J$) and off-diagonal symmetric ($\Gamma$) couplings. We investigate the quantum ($S = 1/2$) $K$-$J$-$\Gamma$ model on the honeycomb lattice by…

Strongly Correlated Electrons · Physics 2019-11-14 Jiucai Wang , B. Normand , Zheng-Xin Liu

$\alpha$-RuCl$_3$ has been studied extensively because of its proximity to the Kitaev quantum-spin-liquid (QSL) phase and the possibility of approaching it by tuning the competing interactions. Here we present the first polarized inelastic…

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

Kitaev iridates have been proposed as candidates for realizing an elusive quantum spin liquid (QSL) state, in which strong spin-orbit coupling and bond-directional exchange generate a highly frustrated and entangled ground state. However,…

The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

The pure Kitaev honeycomb model harbors a quantum spin liquid in zero magnetic fields, while applying finite magnetic fields induces a topological spin liquid with non-Abelian anyonic excitations. This latter phase has been much sought…

Strongly Correlated Electrons · Physics 2020-03-31 Dirk Wulferding , Youngsu Choi , Seung-Hwan Do , Chan Hyeon Lee , Peter Lemmens , Clement Faugeras , Yann Gallais , Kwang-Yong Choi

Motivated by the magnetic phase transition of a proximate Kitaev system $\alpha$-RuCl$_3$ in the presence of a magnetic field, we study the simplest but essential quantum spin model with the ferromagnetic nearest neighboring (NN) Kitaev…

Strongly Correlated Electrons · Physics 2020-10-14 Beom Hyun Kim , Shigetoshi Sota , Tomonori Shirakawa , Seiji Yunoki , Young-Woo Son

Using quantum chemistry calculations we shed fresh light on the electronic structure and magnetic properties of RuCl3, a proposed realization of the honeycomb Kitaev spin model. It is found that the nearest-neighbor Kitaev exchange K is…

Strongly Correlated Electrons · Physics 2017-01-19 Ravi Yadav , Nikolay A. Bogdanov , Vamshi M. Katukuri , Satoshi Nishimoto , Jeroen van den Brink , Liviu Hozoi

Quantum spin liquids have been at the forefront of correlated electron research ever since their original proposal in 1973, and the realization that they belong to the broader class of intrinsic topological orders, along with the fractional…

Strongly Correlated Electrons · Physics 2018-04-26 Ioannis Rousochatzakis , Yuriy Sizyuk , Natalia B. Perkins
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