English

Proximate ferromagnetic state in the Kitaev model material $\alpha$-RuCl$_{3}$

Strongly Correlated Electrons 2021-09-01 v2

Abstract

α\alpha-RuCl3_{3} is a major candidate for the realization of the Kitaev quantum spin liquid, but its zigzag antiferromagnetic order at low temperatures indicates deviations from the Kitaev model. We have quantified the spin Hamiltonian of α\alpha-RuCl3_{3} by a resonant inelastic x-ray scattering study at the Ru L3L_{3} absorption edge. In the paramagnetic state, the quasi-elastic intensity of magnetic excitations has a broad maximum around the zone center without any local maxima at the zigzag magnetic Bragg wavevectors. This finding implies that the zigzag order is fragile and readily destabilized by competing ferromagnetic correlations. The classical ground state of the experimentally determined Hamiltonian is actually ferromagnetic. The zigzag state is stabilized via a quantum "order by disorder" mechanism, leaving ferromagnetism -- along with the Kitaev spin liquid -- as energetically proximate metastable states. The three closely competing states and their collective excitations hold the key to the theoretical understanding of the unusual properties of α\alpha-RuCl3_{3} in magnetic fields.

Keywords

Cite

@article{arxiv.2008.02037,
  title  = {Proximate ferromagnetic state in the Kitaev model material $\alpha$-RuCl$_{3}$},
  author = {H. Suzuki and H. Liu and J. Bertinshaw and K. Ueda and H. Kim and S. Laha and D. Weber and Z. Yang and L. Wang and H. Takahashi and K. Fürsich and M. Minola and B. V. Lotsch and B. J. Kim and H. Yavaş and M. Daghofer and J. Chaloupka and G. Khaliullin and H. Gretarsson and B. Keimer},
  journal= {arXiv preprint arXiv:2008.02037},
  year   = {2021}
}