English

Robustness of the thermal Hall effect close to half-quantization in a field-induced spin liquid state

Strongly Correlated Electrons 2022-06-01 v1

Abstract

Thermal signatures of fractionalized excitations are a fingerprint of quantum spin liquids (QSLs). In the Jeff=1/2J_{eff}=1/2 honeycomb magnet α\alpha-RuCl3_3, a QSL state emerges upon applying an in-plane magnetic field HH_{||} greater than the critical field HC2H_{C2} \approx 7 T along the a-axis, where the thermal Hall conductivity (kXY/Tk_{XY}/T) was reported to take on the half-quantized value kHQ/Tk_{HQ}/T. This finding was discussed as a signature of an emergent Majorana edge mode predicted for the Kitaev QSL. The HH_{||}- and TT-range of the half-quantized signal and its relevance to a Majorana edge mode are, however, still under debate. Here we present a comprehensive study of kXY/Tk_{XY}/T in α\alpha-RuCl3_3 with HH_{||} up to 13 T and TT down to 250 mK, which reveals the presence of an extended region of the phase diagram with kXY/TkHQ/Tk_{XY}/T \approx k_{HQ}/T above HC2H_{C2}, in particular across a plateau-like plane for HH_{||} > 10 T and TT < 6.5 K. From 7 T up to \sim10 T, kXY/Tk_{XY}/T is suppressed to zero upon cooling to lowest temperature without any plateau-like behavior and exhibits correlations with complex anomalies in the longitudinal thermal conductivity (kXXk_{XX}) and magnetization around 10 T. The results are in support of a topological state with a half-quantized kXY/Tk_{XY}/T and suggest an interplay with crossovers or weak phase transitions beyond HC2H_{C2} in RuCl3_3.

Keywords

Cite

@article{arxiv.2104.12184,
  title  = {Robustness of the thermal Hall effect close to half-quantization in a field-induced spin liquid state},
  author = {J. A. N. Bruin and R. R. Claus and Y. Matsumoto and N. Kurita and H. Tanaka and H. Takagi},
  journal= {arXiv preprint arXiv:2104.12184},
  year   = {2022}
}