Thermal signatures of fractionalized excitations are a fingerprint of quantum spin liquids (QSLs). In the Jeff=1/2 honeycomb magnet α-RuCl3, a QSL state emerges upon applying an in-plane magnetic field H∣∣ greater than the critical field HC2≈ 7 T along the a-axis, where the thermal Hall conductivity (kXY/T) was reported to take on the half-quantized value kHQ/T. This finding was discussed as a signature of an emergent Majorana edge mode predicted for the Kitaev QSL. The H∣∣- and T-range of the half-quantized signal and its relevance to a Majorana edge mode are, however, still under debate. Here we present a comprehensive study of kXY/T in α-RuCl3 with H∣∣ up to 13 T and T down to 250 mK, which reveals the presence of an extended region of the phase diagram with kXY/T≈kHQ/T above HC2, in particular across a plateau-like plane for H∣∣ > 10 T and T < 6.5 K. From 7 T up to ∼10 T, kXY/T is suppressed to zero upon cooling to lowest temperature without any plateau-like behavior and exhibits correlations with complex anomalies in the longitudinal thermal conductivity (kXX) and magnetization around 10 T. The results are in support of a topological state with a half-quantized kXY/T and suggest an interplay with crossovers or weak phase transitions beyond HC2 in RuCl3.
@article{arxiv.2104.12184,
title = {Robustness of the thermal Hall effect close to half-quantization in a field-induced spin liquid state},
author = {J. A. N. Bruin and R. R. Claus and Y. Matsumoto and N. Kurita and H. Tanaka and H. Takagi},
journal= {arXiv preprint arXiv:2104.12184},
year = {2022}
}