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We theoretically study collisions between ultracold polar molecules that are polarized by microwave or static electric fields. We systematically study the dependence on field strength, microwave polarization, and detuning from rotational…

原子物理 · 物理学 2022-02-09 Tijs Karman , Zoe Z. Yan , Martin Zwierlein

Molecular rotation spectra, generated by the coupling of the molecular electric-dipole moments to an external time-dependent electric field, are discussed in a few particular conditions which can be of some experimental interest. First, the…

其他凝聚态物理 · 物理学 2015-12-15 M. Apostol , L. C. Cune

Quantum degenerate cold-atom gases provide a remarkable opportunity to study strongly interacting systems. Recent experimental progress in producing ultracold polar molecules with a net electric dipole moment opens up new possibilities to…

量子气体 · 物理学 2010-12-16 Roman M. Lutchyn , Enrico Rossi , S. Das Sarma

We measure and theoretically determine the effect of molecular rotational splitting on Zeeman relaxation rates in collisions of cold Triplet-Sigma molecules with helium atoms in a magnetic field. All four stable isotopomers of the imidogen…

We study polar alkali dimer scattering in a quasi-1D geometry for both reactive and non-reactive species. Elastic and reactive rates are computed as a function of the amplitude of a static electric field within a purely long-range model…

原子物理 · 物理学 2019-09-19 Romain Vexiau , Jean-Michel Launay , Andrea Simoni

We propose and analyze a technique that allows to suppress inelastic collisions and simultaneously enhance elastic interactions between cold polar molecules. The main idea is to cancel the leading dipole-dipole interaction with a suitable…

统计力学 · 物理学 2008-09-29 A. V. Gorshkov , P. Rabl , G. Pupillo , A. Micheli , P. Zoller , M. D. Lukin , H. P. Büchler

We investigate the ultracold collisions of rotationally excited dipolar molecules in free-space, taking the hetero-nuclear bi-alkali molecule of KRb as an example. We show that we can sharply tune the elastic, inelastic and reactive rate…

原子物理 · 物理学 2015-03-31 Gaoren Wang , Goulven Quéméner

We theoretically investigate the properties of highly polar diatomic molecules containing $^2S$-state transition-metal atoms. We calculate potential energy curves, permanent electric dipole moments, spectroscopic constants, and leading…

原子物理 · 物理学 2021-02-16 Michał Śmiałkowski , Michał Tomza

Exploring inelastic and reactive collisions on the quantum level is a main goal of the developing field of ultracold chemistry. We present first experimental studies of inelastic collisions of metastable ultracold triplet molecules in the…

Recent experimental developments in the loading of ultracold KRb molecules into quasi-two-dimensional traps, combined with the ability to tune the ratio between elastic and loss (inelastic/reactive) collisions through application of an…

量子物理 · 物理学 2013-12-18 Bihui Zhu , Goulven Quéméner , Ana M. Rey , Murray J. Holland

We develop a collisional formalism adapted for the dynamics of ultracold dipolar particles in a confined geometry and in fields tilted relative to the confinement axis. Using tesseral harmonics instead of the usual spherical harmonics to…

原子物理 · 物理学 2015-10-21 Goulven Quéméner , Maxence Lepers , Olivier Dulieu

We study by quantum Monte Carlo simulations the low-temperature phase diagram of dipolar bosons confined to one dimension, with dipole moments aligned along the direction of particle motion. A hard core repulsive potential of varying range…

统计力学 · 物理学 2020-02-12 Youssef Kora , Massimo Boninsegni

We show that the electric dipole-dipole interaction between a pair of polar molecules undergoes an all-out transformation when superimposed by a far-off resonant optical field. The combined interaction potential becomes tunable by variation…

原子物理 · 物理学 2015-05-30 Mikhail Lemeshko , Bretislav Friedrich

The long-range electrostatic interactions between molecules depend strongly on their relative orientation, which manifests as a rotational state dependence. Interactions between molecules in the same rotational quantum state are well-known…

原子物理 · 物理学 2024-05-16 Etienne F. Walraven , Tijs Karman

We investigate theoretically the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom taking into account its fine-structure. The interaction involves the combination…

化学物理 · 物理学 2017-09-13 Maxence Lepers , Olivier Dulieu

We present the first experimental observation of cold collisions between two different species of neutral polar molecules, each prepared in a single internal quantum state. Combining for the first time the techniques of Stark deceleration,…

We propose a one-channel, simple model to describe the dynamics of ultracold dipolar molecules around a F\"orster resonance. Slightly above a specific electric field, a collisional shielding can take place, suppressing the molecular losses…

量子气体 · 物理学 2024-06-21 Lucas Lassablière , Goulven Quéméner

We have trapped cesium atoms over many minutes in the focus of a CO$_2$-laser beam employing an extremely simple laser system. Collisional properties of the unpolarized atoms in their electronic ground state are investigated. Inelastic…

原子物理 · 物理学 2009-11-06 H. Engler , T. Weber , M. Mudrich , R. Grimm , M. Weidemueller

Collisions between cold polar molecules represent a fascinating research frontier, but have proven hard to probe experimentally. We report measurements of inelastic cross sections for collisions between NO and ND 3 molecules at energies…

Ultracold dipolar molecules hold great promise for the creation of novel quantum states of matter, but the realization of long-lived molecular bulk samples with strong dipole-dipole interactions has remained elusive. Here, we realize a…