相关论文: A Sum Rule for Nonlinear Optical Susceptibilities
In this paper, structural properties of lower semi-frames in separable Hilbert spaces are explored with a focus on transformations under linear operators (may be unbounded). Also, the direct sum of lower semi-frames, providing necessary and…
Optical binding refers to the light-induced interaction between two or more objects illuminated by laser fields. The high tunability of the strength, sign, and reciprocity of this interaction renders it highly attractive for controlling…
The validity of the Luttinger sum rule is considered for finite systems of interacting electrons, where the Fermi volume is determined by location of zeroes of Green's function. It is shown that the sum rule in the paramagnetic state is…
We establish a steady-state theory for nonlinear optical conductivity in pseudo-Hermitian systems. We derive compact formulas for the first and second order conductivity tensors in both the velocity and length gauges and prove their exact…
The Kramers-Kronig relations and various oscillator strength sum rules represent strong constraints on the physical response of materials. In this work, taking inspiration from the well-established equivalence between $f-$sum rules and…
The sum rule for the moments of the spectral density is discussed for the single-band Hubbard model. It is shown that respecting the sum rule up to the order m=3 is conceptually important for a qualitatively correct description of the…
We consider the optical Hall conductivity of a general electronic medium and prove that the optical Hall angle obeys a new sum rule. This sum rule governs the response of an electronic fluid to a Lorentz electric field and can thought of as…
Based on infinite one-dimensional single-electron periodic models of trans-polyacetylene, we show analytically that the overall permutation symmetry of nonlinear optical susceptibilities is, albeit preserved in the molecular systems with…
In a photonic realization of qubits the implementation of quantum logic is rather difficult due the extremely weak interaction on the few photon level. On the other hand, in these systems interference is available to process the quantum…
We derive universal properties of nonlinear response functions of nonequilibrium steady states. In particular, sum rules and asymptotic behaviors are derived. Their consequences are illustrated for nonlinear optical materials and nonlinear…
Thermodynamic stability of statistical systems requires that susceptibilities be semipositive and finite. Susceptibilities are known to be related to the fluctuations of extensive observable quantities. This relation becomes nontrivial,…
We show that a combination of linear absorption spectroscopy, hyper-Rayleigh scattering, and a theoretical analysis using sum rules to reduce the size of the parameter space leads to a prediction of the two-photon absorption cross-section…
Coupling light to ensembles of strongly interacting particles has emerged as a promising route toward achieving few photon nonlinearities. One specific way to implement this kind of nonlinearity is to interface light with highly excited…
We review recent results obtained in the scattering theory of dissipative quantum systems representing the long-time evolution of a system $S$ interacting with another system $S'$ and susceptible of being absorbed by $S'$. The effective…
The Burkhardt--Cottingham sum rule is an exact superconvergence relation for a spin-structure function, derived from general principles of light absorption and scattering, and valid at any momentum transfer $Q^2$. I illustrate how a class…
The concept of supersymmetry in a quantum mechanical system is extended, permitting the recognition of many more supersymmetric systems, including very familiar ones such as the free particle. Its spectrum is shown to be supersymmetric,…
We examine the temperature dependence of the optical sum rule in the normal state due to interactions. To be concrete we adopt a weak coupling approach which uses an electron-boson exchange model to describe inelastic scattering of the…
Truncated sum rules have been used to calculate the fundamental limits of the nonlinear susceptibilities; and, the results have been consistent with all measured molecules. However, given that finite-state models result in inconsistencies…
The non-linear response of infinite periodic solids to homogenous electric fields and collective atomic displacements is discussed in the framework of density functional perturbation theory. The approach is based on the 2n + 1 theorem…
We study CFTs at finite temperature and derive explicit sum rules for one-point functions of operators by imposing the KMS condition. In the case of a large gap between light and heavy operators, we explicitly compute one-point functions…