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Our recent arXiv preprints have described the experimental evidence for the universal occurrence of short circuit photocurrents on illumination of solid state surfaces by strongly absorbed light. A likely mechanism has been proposed based…

材料科学 · 物理学 2008-05-02 Mladen Georgiev

When an atom or molecule absorbs a high-energy photon, an electron is emitted with a well-defined energy and a highly-symmetric angular distribution, ruled by energy quantization and parity conservation. These rules seemingly break down…

The model of hydrogen migration and of the reactions of hydrogen atoms with electrically active impurity, developed earlier, has been applied to simulate hydrogen diffusion and passivation process during plasma deuteration of silicon…

材料科学 · 物理学 2015-06-12 O. I. Velichko , Yu. P. Shaman , A. P. Kovaliova

This work demonstrates photon emission gain, i.e., emission of multiple photons per injected electron, through impact excitation in Er-doped silicon light-emitting diodes (LEDs). Conventional methods for exciting Er ions in silicon suffer…

The transient-absorption spectrum of a $V$-type three-level system is investigated, when this is periodically excited by a train of equally spaced, $\delta$-like pump pulses as, e.g., from an optical-frequency-comb laser. We show that, even…

原子物理 · 物理学 2019-01-30 Juliane Haug , Stefano M. Cavaletto

We present a quantum framework based on a density matrix of a dimer system to investigate the quantum dynamics of excitation energy transfer (EET) in the presence of the evanescent field from the metal and the phonon bath. Due to the…

量子物理 · 物理学 2017-08-02 Amrit Poudel , Xin Chen , Mark A. Ratner

Absorption of electromagnetic energy by a dissipative material is one of the most fundamental electromagnetic processes that underlies a plethora of applied problems, including sensing and molecular detection, radar detection, wireless…

光学 · 物理学 2020-03-31 Alexey Proskurin , Andrey Bogdanov , Denis G. Baranov

We explore stimulated photo-association in the context of attosecond pump-probe schemes of atomic matter. An attosecond pulse -- the probe -- is used to induce photo-association of an electronic wave packet which had been created before,…

原子物理 · 物理学 2009-11-13 Paula Rivière , Camilo Ruiz , Jan-Michael Rost

Many fundamental processes of structural changes at surfaces occur on a pico- or femtosecond time scale. In order to study such ultra-fast processes, we have combined modern surface science techniques with fs-laser pulses in a pump-probe…

介观与纳米尺度物理 · 物理学 2023-12-01 Michael Horn von Hoegen

Photoinduced charge-transfer processes play a key role for novel photovoltaic phenomena and devices. Thus, the development of ab initio methods that allow for an accurate and computationally inexpensive treatment of charge-transfer…

化学物理 · 物理学 2014-04-25 Iris Theophilou , M. Tassi , S. Thanos

We investigate the kinetic-energy spectrum of electrons emitted from an excited many-electron system, often called photo-electron spectrum (PES). We are particularly interested on the impact of resonant modes of the system on PES. To this…

原子与分子团簇 · 物理学 2015-06-23 P. M. Dinh , P. -G. Reinhard , E. Suraud , P. Wopperer

We theoretically study pump-photon-energy-dependent pathways of a photoinduced dimer-Mott-insulator-to-metal transition, on the basis of numerical solutions to the time-dependent Schr\"odinger equation for the exact many-body wave function…

强关联电子 · 物理学 2015-05-28 Kenji Yonemitsu , Satoshi Miyashita , Nobuya Maeshima

Battery electrode surfaces are generally coated with electronically insulating solid films of thickness 1-50 nm. Both electrons and Li+ can move at the electrode-surface film interface in response to the voltage, which adds complexity to…

材料科学 · 物理学 2015-07-10 Kevin Leung , Andrew Leenheer

The interaction between molecular (atomic) electron(s) and the vacuum field of a reflective cavity generates a significant interest thanks to the rapid developments in nanophotonics. Such interaction which lies within the realm of cavity…

化学物理 · 物理学 2019-05-22 Alexander Semenov , Abraham Nitzan

The shape of the photoluminescence line excited at an edge face of InP wafer and recorded from the broadside is used to investigate the intrinsic emission spectrum. The procedure is much less sensitive to the surface properties and the…

材料科学 · 物理学 2015-06-16 Oleg Semyonov , Arsen Subashiev , Zhichao Chen , Serge Luryi

Electron scattering and dielectronic recombination with an ion in the presence of a neighboring atom is studied. The incident electron is assumed to be captured by the ion, leading to resonant excitation of the atom which afterwards may…

原子物理 · 物理学 2018-08-01 A. Eckey , A. Jacob , A. B. Voitkiv , C. Müller

The advent of powerful laser sources has made it possible to observe a relatively large cross section of the excited state of Hydrogen atom. This is due to the effect of joint collisions of a linearly polarized $N$-photon and high-energy…

原子物理 · 物理学 2023-04-25 Behnam Nikoobakht

Photoemission experiments involve the motion of an electron near a conducting surface. This necessarily generates heat by ohmic losses from eddy currents. This inelastic scattering of the electrons will result in a downward shift in…

强关联电子 · 物理学 2007-05-23 Robert Haslinger , Robert Joynt

Ultrafast electron-photon spectroscopy in electron microscopes commonly requires ultrafast laser setups. Photoemission from an engineered electron source is used to generate pulsed electrons, interacting with a sample that is excited by the…

介观与纳米尺度物理 · 物理学 2023-06-28 Masoud Taleb , Mario Hentschel , Kai Rossnagel , Harald Giessen , Nahid Talebi

Ionization-excitation of an atom induced by the absorption of a single photon in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly…

原子物理 · 物理学 2023-09-06 S. Kim , S. Steinhäuser , A. B. Voitkiv , C. Müller