相关论文: Monolayer Solid Helium-4 Clusters on Graphite
Experiments have confirmed that double monolayer graphene cannot generate finite temperature electron-hole superfluidity. This has been shown to be due to very strong screening of the electron-hole pairing attraction. The linear dispersing…
We made heat-capacity measurements of two dimensional (2D) $^3$He adsorbed on graphite preplated with monolayer $^4$He in a wide temperature range (0.1 $\leq T \leq$ 80 mK) at densities higher than that for the 4/7 phase (= 6.8 nm$^{-2}$).…
We study by Quantum Monte Carlo simulations the local superfluid response of small (up to 27 molecules) parahydrogen clusters, down to temperatures as low as 0.05 K. We show that at low temperature superfluidity is not confined at the…
This article discusses the behavior of submonolayer quantum films (He and H2) on graphene and newly discovered surfaces that are derived from graphene. Among these substrates are graphane (abbreviated GH), which has an H atom bonded to each…
Insoluble surfactant monolayers at the air/water interface undergo a phase transition from a high-temperature homogeneous state to a low-temperature demixed state, where dilute and dense phases coexist. Alternatively, the transition from a…
We study different solid phases of Helium-four, by means of Path Integral Monte Carlo simulations based on a recently developed "worm" algorithm. Our study includes simulations that start off from a high-T gas phase, which is then…
Using molecular dynamics simulation, we investigate the slow dynamics of a supercooled binary mixture of soft particles interacting with a generalized Hertzian potential. At low density, it displays typical slow dynamics near its glass…
Adsorption of ortho-deuterium and para-hydrogen films on a graphite substrate, pre-plated with a single atomic layer of krypton, is studied theoretically by means of quantum Monte Carlo simulations at low temperature. Our model explicitly…
We use density functional theory and Monte Carlo lattice simulations to investigate the structure of ZrO$_{2}$ monolayers on Si(001). Recently, we have reported on the experimental growth of amorphous ZrO$_{2}$ monolayers on silicon and…
The expression of chirality in adsorption phenomena constitutes an important topic, not only relevant to asymmetric transformations involving solid surfaces, but also to the emergence of homochirality in both terrestrial and…
Recent experiments on the flow of helium-4 fluid through nanopores with tunable pore radius provide a platform for studying the quasi-one-dimensional (quasi-1D) superfluid behaviors. In the extreme 1D limit, the helium atoms are localized…
We show theoretically that the second layer of 3He adsorbed on graphite and solidified at 4/7 of the first-layer density is close to the fluid-solid boundary with substantial density fluctuations on the third layer. The solid shows a…
Phase transitions are uncommon among homogenous one-dimensional fluids of classical particles owing to a general non-existence result due to van Hove. A way to circumvent van Hove's theorem is to consider an interparticle potential that is…
We have investigated the ground state properties of solid $^4$He with the Shadow Path Integral Ground State method. This exact T=0 K projector method allows to describes quantum solids without introducing any a priori equilibrium position.…
We study by Quantum Monte Carlo simulations the phase diagram of lattice hard core bosons with nearest-neighbour repulsive interactions, in the presence of a super-lattice of adsorption sites. For a moderate adsorption strength, the system…
Experimental observation of superfluidity in a microscopic cluster, $M:(^4He)_x$, of a molecule ($M$) and $x$ number of $^4He$ atoms (with $x$ ranging from 1 to many) is qualitatively analyzed. It concludes that: (i) each $^4He$ atom in the…
We have performed quantum Monte Carlo simulations measuring the finite size and temperature superfluid response of helium-4 to the linear and rotational motion of the walls of a nanopore. Within the two-fluid model, the portion of the…
By large-scale quantum Monte Carlo simulations we show that grain boundaries in Helium-4 crystals are generically superfluid at low temperature, with a transition temperature of the order of ~0.5K at the melting pressure; insulating grain…
We carried out simulations of crystal truncation rod (CTR) scatterings, i.e., one of the surface X-ray diffraction techniques with atomic resolution, from a monolayer He film adsorbed on graphite. Our simulations reveal that the 00L rod…
We use molecular simulation to study the structural and dynamic properties of glassy nanoclusters formed both through the direct condensation of the vapor below the glass transition temperature, without the presence of a substrate, and…