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Strong resonant enhancements of the charge-order and spin-order superstructure-diffraction intensities in La1.8Sr0.2NiO4 are observed when x-ray energies in the vicinity of the Ni L2,3 absorption edges are used. The pronounced photon-energy…

Neutron scattering has been used to study the nature of the ferromagnetic transition in a single crystal of the perovskite La0.7Ca0.3MnO3. Diffuse scattering from lattice polarons develops as the Curie temperature is approached from below,…

强关联电子 · 物理学 2009-10-31 C. P. Adams , J. W. Lynn , Y. M. Mukovskii , A. A. Arsenov , D. A. Shulyatev

The short-range organization around Ni atoms in orthorhombic $R$NiO$_{3}$ ($R$=Pr,Nd,Eu) perovskites has been studied over a wide temperature range by Ni K-edge x-ray absorption spectroscopy. Our results demonstrate that two different Ni…

Resonant soft X-ray scattering was used to determine the presence of more subtle orderings not detected in standard structural analyses. By tuning to specific Co absorption edges, arrangements particular to the electronic states of those…

强关联电子 · 物理学 2017-07-17 F. J. Rueckert , F. He , B. Poudel , B. Dabrowski , W. A. Hines , J. I. Budnick , B. O. Wells

A system of strongly-interacting electron-lattice polarons can exhibit charge and orbital order at sufficiently high polaron concentrations. In this study, the structure of short-range polaron correlations in the layered colossal…

In pursuit of rational control of orbital polarization, we present a combined experimental and theoretical study of single unit cell superlattices of the correlated metal LaNiO$_3$ and the band insulator LaAlO$_3$. Polarized x-ray…

强关联电子 · 物理学 2012-01-23 J. W. Freeland , Jian Liu , M. Kareev , B. Gray , J. W. Kim , P. Ryan , R. Pentcheva , J. Chakhalian

Charge and orbital ordering behaviors in the half doped bi-layered compound LaSr2Mn2O7 have been studied by resonant and non-resonant X-ray scattering. Three different order parameters, which correspond to the A-type antiferromagnetic, a…

Recently a growing number of experiments have provided indications of the key role of polarons (composite particles formed by a charge strongly coupled with a local lattice deformation) in doped perovskites, hosting colossal…

超导电性 · 物理学 2009-09-25 A. Lanzara , N. L. Saini , A. Bianconi , Guo-meng Zhao , K. Conder , H. Keller , K. A. Muller

By comparing the optical conductivities of La_{1.67}Sr_{0.33}NiO_{4} (LSNO), Sr_{1.5}La_{0.5}MnO_4 (SLMO), Nd_2CuO_{4-y} (NCO), and Nd_{1.96}Ce_{0.04}CuO_{4} (NCCO), we have identified a peculiar behavior of polarons in this cuprate family.…

超导电性 · 物理学 2016-08-31 P. Calvani , P. Dore , S. Lupi , A. Paolone , P. Maselli , P. Giura , B. Ruzicka , S-W. Cheong , W. Sadowski

This review will deal with several types of free charge localisation in oxides and their consequences on the effective dielectric spectra of such materials. The first one is the polaronic localisation at the unit cell scale on residual…

材料科学 · 物理学 2010-06-21 Mario Maglione

A broken translation symmetry has recently been revealed in infinite-layer nickelates, which has piqued considerable interest in its origin and relation to superconductivity, as well as in its comparison to charge order in cuprates. Here,…

Two-dimensional (2D) perovskite oxide interfaces are ideal systems where diverse emergent properties can be uncovered.The formation and modification of polaronic properties due to short-range strong charge-lattice interactions of 2D…

We report a detailed neutron scattering study of the ordering of spins and holes in oxygen-doped La(2)NiO(4.133). The single-crystal sample exhibits the same oxygen-interstitial order but better defined charge-stripe order than that studied…

强关联电子 · 物理学 2009-10-30 P. Wochner , J. M. Tranquada , D. J. Buttrey , V. Sachan

Synchrotron x-ray scattering measurements of the low-temperature structure of the single-layer manganese oxide La$_{1-x}$Sr$_{1+x}$MnO$_4$, over the doping range $0.33 \le x \le 0.67$, indicate the existence of three distinct regions: a…

强关联电子 · 物理学 2009-11-07 S. Larochelle , A. Mehta , N. Kaneko , P. K. Mang , A. F. Panchula , L. Zhou , J. Arthur , M. Greven

X-ray absorption spectroscopy and resonant soft x-ray reflectivity show a non-uniform distribution of oxygen holes in a La2NiO4 - La2CuO4 (LNO-LCO) superlattice, with excess holes concentrated in the LNO layers. Weak ferromagnetism with Tc…

强关联电子 · 物理学 2015-05-28 S. Smadici , J. C. T. Lee , J. Morales , G. Logvenov , O. Pelleg , I. Bozovic , Y. Zhu , P. Abbamonte

The in-plane oxygen vibrations in La2NiO4 are investigated for several hole-doping concentrations both theoretically and experimentally via inelastic neutron scattering. Using an inhomogeneous Hartree-Fock plus RPA numerical method in a…

强关联电子 · 物理学 2009-10-31 R. J. McQueeney , A. R. Bishop , Ya-Sha Yi , Z. G. Yu

We report an infrared reflection spectroscopy study of La$_{1/2}$Ca$_{1/2}$MnO$_3$ over a broad frequency range and temperature interval which covers the transitions from the high temperature paramagnetic to ferromagnetic and, upon further…

强关联电子 · 物理学 2009-11-10 A. P. Litvinchuk , M. N. Iliev , M. Pissas , C. W. Chu

Superstructure reflections due to the ordering of holes into stripes in La_(1.45)Nd_(0.4)Sr_(0.15)CuO_4 have been studied with high energy x-ray diffraction. These reflections have been observed clearly for the first time in a sample which…

A hypothetical layered oxide La_2NiMO_6 where NiO_2 and MO_2 planes alternate along the c-axis of ABO_3 perovskite lattice is considered theoretically. Here, M denotes a trivalent cation Al, Ga,... such that MO_2 planes are insulating and…

强关联电子 · 物理学 2010-05-11 Jiri Chaloupka , Giniyat Khaliullin

The normal state optical response of La_{2-x}Sr_xCuO_4 is found to be consistent with a simple multi-component model, based on free carriers with strong electron-phonon interaction, localized polaronic states near 0.15 eV and a mid-infrared…

超导电性 · 物理学 2016-08-31 O. V. Dolgov , H. J. Kaufmann , E. K. H. Salje , Y. Yagil
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