相关论文: Vibrational Study of 13C-enriched C60 Crystals
We extend the Weak Crystallization theory to the case of metallic alloys. The additional ingredient -- itinerant electrons -- generates nontrivial dependence of free energy on the angles between ordering wave vectors of ionic density. That…
133Cs and 13C-NMR have been used to study the electronic properties of the polymerized phase of CsC60 at ambient and under hydrostatic pressure. The salient result of this study is the finding of fluctuations in the local field at 133Cs…
We demonstrate, using the high resolution spectra from the ESPADONS spectrograph, fed with the 3.6m CFH telescope, that the strength ratios of the strong--to--weak spectral features, attributed to C$_{60}^+$, are variable. We found that in…
The empirical spectra and $E2$ decay rates in $^{110,112,114,116}$Cd are shown to be consistent with a vibrational interpretation for low-lying normal states, coexisting with a single deformed $\gamma$-soft band of intruder states. The…
The neutral silicon--vacancy (SiV$^{0}$) center in diamond combines inversion symmetry with optical emission, making it a robust quantum emitter resilient to stray electric fields. Using first-principles density-functional theory, we…
We present a detailed NMR study of simple cubic CsC60, the only metallic cubic fullerides known so far besides A3C60. 133Cs NMR signals the presence of about 12 to 15% of ``anomalous'' C60 balls, characterized by a 15 meV gap. We present…
More than 100 excited states of the Calcium-40 nucleus, with isospin 0, are classified into rotational-vibrational bands of an intrinsic tetrahedral structure. Almost all observed states below 8 MeV can be accommodated, as well as many…
In glasses, atomic disorder combined with atomic connectivity makes understanding of the nature of the vibrations much more complex than in crystals or molecules. With a simple model, however, it is possible to show how disorder generates…
Glasses have a large excess of low-frequency vibrational modes in comparison with crystalline solids. We show that such a feature is a necessary consequence of the geometry generic to weakly connected solids. In particular, we analyze the…
We have found the complete spectrum and eigenstates for harmonic oscillations of ideal spherical and cylindrical shells, both being infinitely thin. The spectrum of the cylindrical shell has an infinite number of Goldstone modes…
The recent detection of fullerene (C$_{60}$) in space and the positive assignment of five diffuse interstellar bands to C$_{60}^+$ reinforce the notion that fullerene-related compounds can be efficiently formed in circumstellar envelopes…
Several diamond bulk crystals with a concentration of electrically neutral single substitutional nitrogen atoms of $\lesssim 80~$ppm, the so-called C- or P1-centres, were irradiated with electrons at 10 MeV energy and low fluence. The…
Strange modes can occur in radiative classical Cepheids and RR Lyrae models. These are vibrational modes that are trapped near the surface as a result of a 'potential barrier' caused by the sharp hydrogen partial ionization region.…
We experimentally demonstrate high degree of polarization of 13C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled…
We show theoretically the fingerprints of short-range spiral magnetic correlations in the photoemission spectra of the Mott insulating ground states realized in the triangular silicon surfaces K/Si(111)-B and SiC(0001). The calculated…
The robust (spin and isospin zero) $\alpha$-particle remains one of the best projectiles to probe the nuclear isoscalar excitations. In the present work, a microscopic folding model analysis of the \ac inelastic scattering to the 2$^+$…
With infrared and terahertz ellipsometry we investigated the anisotropy of the infrared active phonon modes in SrTiO3 (110) single crystals in the tetragonal state below the so-called antiferrodistortive transition at T* = 105 K. In…
Optically active solid-state spin registers have demonstrated their unique potential in quantum computing, communication and sensing. Realizing scalability and increasing application complexity requires entangling multiple individual…
The silicon-vacancy centre (SiV) in diamond has interesting vibronic features. We demonstrate that the zero phonon line position can be used to reliably identify the silicon isotope present in a single centre. This is of interest for…
Modification induced by 110 MeV Ni ion irradiated thin film samples of C60 on Si and quartz substrates were studied at various fluences. The pristine and irradiated samples were investigated using Raman spectroscopy, electrical conductivity…