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We have studied the C14 hexagonal Laves phase of YbAg$_2$ at normal conditions and under external pressure up to 19 GPa by the time-differential perturbed angular $\gamma-\gamma$ correlation spectroscopy (TDPAC) using $^{111}$Cd probe…

The nuclear quadrupole interaction of the I=5/2 state of the nuclear probes 111Cd and 181Ta in the anatase and rutile polymorphs of bulk TiO2 was studied using the time differential perturbed angular correlation (TDPAC). The fast-slow…

材料科学 · 物理学 2015-05-13 Satyendra Kumar Das , Sanjay Vishwanath Thakare , Tilman Butz

We investigate the Yb valence instabilities in the strongly correlated YbPd compound using resonant X-ray emission spectroscopy as a function of pressure across the charge-order (CO) transition. At a low temperature (T = 30 K) in the CO…

Nuclear quadrupole interactions were measured at 111In/Cd probe atoms in rare-earth palladium phases RPd3 having the L12 structure using the technique of perturbed angular correlation of gamma rays (PAC). Measurements were made for pairs of…

材料科学 · 物理学 2014-03-27 Qiaoming Wang , Gary S. Collins

We report a comprehensive structural and valence study of the intermediate valent materials YbNiGa$_{4}$ and YbNiIn$_{4}$ under pressures up to 60 GPa. YbNiGa$_{4}$ undergoes a smooth volume contraction and shows steady increase in…

We report measurements of the physical properties and electronic structure of the hexagonal compounds Yb2Ni12Pn7 (Pn = P, As) by measuring the electrical resistivity, magnetization, specific heat and partial fluorescence yield x-ray…

We present a dynamical mean field theory study of the valence transition ($f^{14} \to f^{13}$) in elemental, metallic Yb under pressure. Our calculations reproduce the observed valence transition as reflected in the volume dependence of the…

强关联电子 · 物理学 2010-05-12 E. R. Ylvisaker , J. Kuneš , A. K. McMahan , W. E. Pickett

The pressure-temperature phase diagram of an intermediate-valence compound YbPd was revealed via simultaneous ac-calorimetry and electrical resistivity measurements. Two successive structural phase transition temperatures, $T_1$ = 125 K and…

The valence orders at $T_a=125$ K and $T_b=105$ K in the cubic compound YbPd have been investigated by $^{105}$Pd-nuclear magnetic resonance (NMR) measurements. Significant decrease in the density of states at the Fermi energy below $T_a$…

强关联电子 · 物理学 2019-02-19 R. Nakanishi , T. Fujii , Y. Nakai , K. Ueda , M. Hirata , K. Oyama , A. Mitsuda , H. Wada , T. Mito

We report Resonant inelastic x-ray scattering measurements (RIXS) in YbCu$_2$Si$_2$ at the Yb L$_{3}$ edge under high pressure (up to 22 GPa) and at low temperatures (down to 7 K) with emphasis on the vicinity of the transition to a…

Unconventional quantum critical phenomena observed in Yb-based periodic crystals such as YbRh$_2$Si$_2$ and $\beta$-YbAlB$_4$ have been one of the central issues in strongly correlated electron systems. The common criticality has been…

强关联电子 · 物理学 2017-03-14 Shinji Watanabe , Kazumasa Miyake

We present magnetization, specific heat, and 27Al NMR investigations on YbFe2Al10 over a wide range in temperature and magnetic field. The magnetic susceptibility at low temperatures is strongly enhanced at weak magnetic fields, accompanied…

强关联电子 · 物理学 2014-11-24 P. Khuntia , P. Peratheepan , A. Strydom , Y. Utsumi , K. -T. Ko , K. -D. Tsuei , L. H. Tjeng , F. Steglich , M. Baenitz

The intermediate valence compound YbAl$_3$ is known to undergo a hybridization process between itinerant and localized electrons. The resulting heavy Fermi liquid remains non-magnetic and non-superconducting. A microscopic understanding of…

强关联电子 · 物理学 2014-11-27 W. K. Park , S. M. Narasiwodeyar , M. Dwyer , P. C. Canfield , L. H. Greene

Progress of theories and experiments of the quantum valence criticality is overviewed focusing on recent discoveries of direct evidence of quantum critical point of valence transitions in periodic crystal $\alpha$-YbAl$_{1-x}$Fe$_x$B$_4$ at…

强关联电子 · 物理学 2020-04-22 Shinji Watanabe , Kazumasa Miyake

We report electrical resistivity, ac magnetic susceptibility and X-ray absorption spectroscopy measurements of intermediate valence YbNi$_{3}$Ga$_{9}$ under pressure and magnetic field. We have revealed a characteristic pressure-induced Yb…

The 63Cu nuclear quadrupole resonance (NQR) frequency, nu_q, in the multi-layered cuprates is calculated in the cluster model by the exact diagonalization method. The charge imbalance between the outer CuO_2 plane (OP) with apical oxygen…

超导电性 · 物理学 2009-11-25 M. Mori , N. Afzal Shooshtary , T. Tohyama , S. Maekawa

We have synthesized new Tsai-type Yb-based intermediate-valence approximant crystals (ACs) with different degree of approximation to quasicrystal, Zn--Au--Yb 1/1 and 2/1 AC, and studied the external pressure effect on their Yb mean-valence…

An x-ray diffraction study reveals the charge ordering structure in an intermediate valence magnet YbPd with a CsCl-structure. The valence of the Yb ions forms an incommensurate structure, characterized by the wavevector (+-0.07 +-0.07 1/2)…

The mechanism of emergence of robust quantum criticality in Yb- and Ce-based heavy electron systems under pressure is analyzed theoretically. By constructing a minimal model for quasicrystal Yb15Al34Au51 and its approximant, we show that…

强关联电子 · 物理学 2013-07-08 Shinji Watanabe , Kazumasa Miyake

We performed high-magnetic-field ultrasonic experiments on YbB$_{12}$ up to 59 T to investigate the valence fluctuations in Yb ions. In zero field, the longitudinal elastic constant $C_{11}$, the transverse elastic constants $C_{44}$ and…

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