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We report the existence of broad and weakly asymmetric features in the high-energy (G) Raman modes of freely suspended metallic carbon nanotubes of defined chiral index. A significant variation in peak width (from 12 cm-1 to 110 cm-1) is…

We have measured shot noise in metallic single-walled carbon nanotubes of length L=1 $\mu$m and have found strong suppression of noise with increasing voltage. We conclude that the coupling of electron and phonon baths at temperatures $T_e$…

介观与纳米尺度物理 · 物理学 2011-04-22 Fan Wu , Pauli Virtanen , Soren Andresen , Bernard Placais , Pertti Hakonen

The coupling between electrons and phonons is at the heart of many fundamental phenomena in physics. In nature, this coupling is generally predetermined for both, molecules and solids. Tremendous advances have been made in controlling…

介观与纳米尺度物理 · 物理学 2015-06-15 Avishai Benyamini , Assaf Hamo , Silvia Viola Kusminskiy , Felix von Oppen , Shahal Ilani

Using femtosecond pump-probe spectroscopy with pulse shaping techniques, one can generate and detect coherent phonons in chirality-specific semiconducting single-walled carbon nanotubes. The signals are resonantly enhanced when the pump…

介观与纳米尺度物理 · 物理学 2015-05-13 G. D. Sanders , C. J. Stanton , J. -H. Kim , K. -J. Yee , Y. -S. Lim , E. H. Haroz , L. G. Booshehri , J. Kono , R. Saito

We prove that Electron-phonon coupling (EPC) is the major source of broadening for the Raman G and G- peaks in graphite and metallic nanotubes. This allows us to directly measure the optical-phonon EPCs from the G and G- linewidths. The…

材料科学 · 物理学 2007-05-23 Michele Lazzeri , S. Piscanec , Francesco Mauri , A. C. Ferrari , J. Robertson

Motivated by recent experiments, we investigate the electron-vibron coupling in suspended carbon nanotube quantum dots, starting with the electron-phonon coupling of the underlying graphene layer. We show that the coupling strength depends…

介观与纳米尺度物理 · 物理学 2015-05-13 Eros Mariani , Felix von Oppen

We show by ab initio calculations that the electron-phonon coupling matrix element M of the radial breathing mode in single-walled carbon nanotubes depends strongly on tube chirality. For nanotubes of the same diameter the coupling strength…

材料科学 · 物理学 2009-11-10 M. Machon , S. Reich , H. Telg , J. Maultzsch , P. Ordejon , C. Thomsen

Using pre-designed trains of femtosecond optical pulses, we have selectively excited coherent phonons of the radial breathing mode of specific-chirality single-walled carbon nanotubes within an ensemble sample. By analyzing the initial…

We present direct experimental observation of exciton-phonon bound states in the photoluminescence excitation spectra of isolated single walled carbon nanotubes in aqueous suspension. The photoluminescence excitation spectra from several…

材料科学 · 物理学 2009-11-11 Flavio Plentz , Henrique B. Ribeiro , Ado Jorio , Marcos A. Pimenta , Michael S. Strano

Coupling an electromechanical resonator with carbon-nanotube quantum dots is a significant method to control both the electronic charge and the spin quantum states. By exploiting a novel micro-transfer technique, we fabricate two…

We find that the optical properties of carbon nanotubes reflect remarkably strong effects of exciton-phonon coupling. Tight-binding calculations show that a significant fraction of the spectral weight of the absorption peak is transferred…

材料科学 · 物理学 2009-11-10 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

We investigate the Fano-type line shape of the Ba mode of Y_{1-x}Ca_xBa_2Cu_3O_{6+y} films observed in Raman spectra with A_1g symmetry. The line shape is described with an extended Fano formula that allows us to obtain the bare phonon…

超导电性 · 物理学 2015-06-25 A. Bock , S. Ostertun , K. -O. Subke

Condensed-matter emitters offer enriched cavity quantum electrodynamical effects due to the coupling to external degrees of freedom. In the case of carbon nanotubes a very peculiar coupling between localized excitons and the one-dimensional…

We theoretically estimate the electron-phonon coupling constant lambda for metallic single-walled carbon nanotubes with a diameter of 1.4 nm. The partial electron-phonon coupling constant for the hardest phonon mode is estimated to be about…

超导电性 · 物理学 2007-05-23 Guo-meng Zhao

One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

材料科学 · 物理学 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

Carbon nanotubes provide a rare access point into the plasmon physics of one-dimensional electronic systems. By assembling purified nanotubes into uniformly sized arrays, we show that they support coherent plasmon resonances, that these…

The interplay between discrete vibrational and electronic degrees of freedom directly influences the chemical and physical properties of molecular systems. This coupling is typically studied through optical methods such as fluorescence,…

介观与纳米尺度物理 · 物理学 2007-05-23 B. J. LeRoy , S. G. Lemay , J. Kong , C. Dekker

We investigate the effect of electron-phonon coupling on low temperature phases in metallic single-wall carbon nanotubes. We obtain low-temperature phase diagrams of armchair and zigzag type nanotubes with screened interactions with a…

强关联电子 · 物理学 2018-11-14 Junichi Okamoto , Ludwig Mathey , Wen-Min Huang

Phonon softening phenomena of the $\Gamma$ point optical modes including the longitudinal optical mode, transverse optical mode and radial breathing mode in "metallic" single wall carbon nanotubes are reviewed from a theoretical point of…

介观与纳米尺度物理 · 物理学 2010-05-13 K. Sasaki , H. Farhat , R. Saito , M. S. Dresselhaus

High-resolution electron energy loss spectroscopy measurements have been carried out on an optimally doped cuprate Bi2Sr2CaCu2O8+{\delta}. The momentum-dependent linewidth and the dispersion of an A1 optical phonon are obtained. Based on…

强关联电子 · 物理学 2015-05-18 Huajun Qin , Junren Shi , Yanwei Cao , Kehui Wu , Jiandi Zhang , E. W. Plummer , J. Wen , Z. J. Xu , G. D. Gu , Jiandong Guo
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