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Nearly thirty years after its inception, the field of DNA-programmed colloidal self-assembly has begun to realize its initial promise. In this review, we summarize recent developments in designing effective interactions and understanding…

软凝聚态物质 · 物理学 2025-05-08 William M. Jacobs , W. Benjamin Rogers

The freezing of colloidal suspensions is encountered in many natural and engineering processes such as the freezing of soils, food engineering, and cryobiology. It can also be used as a bio-inspired, versatile, and environmentally-friendly…

应用物理 · 物理学 2018-05-16 Sylvain Deville , Jérôme Adrien , Eric Maire , Mario Scheel , Marco Di Michiel

We outline a basic strategy of how self-propulsion can be used to improve the yield of a typical colloidal self-assembly process. The success of this approach is predicated on the thoughtful design of the colloidal building block as well as…

软凝聚态物质 · 物理学 2016-08-24 S. A. Mallory , A. Cacciuto

We study the assembly of colloids in a two phase water-water system that provides an environment that can sustain bacteria, providing a new structure with rich potential to confine and structure living colloids. The water-water system,…

软凝聚态物质 · 物理学 2014-12-12 Sarah D. Hann , Mark Goulian , Daeyeon Lee , Kathleen J. Stebe

Self-assembly of colloidal particles due to elastic interactions in nematic liquid crystals promises tunable composite materials and can be guided by exploiting surface functionalization, geometric shape and topology, though these means of…

软凝聚态物质 · 物理学 2017-12-29 Bohdan Senyuk , Qingkun Liu , Philip D. Nystrom , Ivan I. Smalyukh

Entropy alone can self-assemble hard particles into colloidal crystals of remarkable complexity whose structures are the same as atomic and molecular crystals, but with larger lattice spacings. Although particle-based molecular simulation…

软凝聚态物质 · 物理学 2021-07-06 Thi Vo , Sharon C. Glotzer

Colloids dispersed in nematic liquid crystals form topological composites in which colloid-associated defects mediate interactions while adhering to fundamental topological constraints. Better realising the promise of such materials…

软凝聚态物质 · 物理学 2024-04-16 Louise C. Head , Yair A. G. Fosado , Davide Marenduzzo , Tyler N. Shendruk

The macroscopic phenomenon of filtration is the separation between suspended and liquid phases and it takes place in natural environments (e.g. groundwater, soil, hyporheic zone) and industrial systems (e.g. filtration plants,…

As computers get faster, researchers -- not hardware or algorithms -- become the bottleneck in scientific discovery. Computational study of colloidal self-assembly is one area that is keenly affected: even after computers generate massive…

软凝聚态物质 · 物理学 2018-03-28 Matthew Spellings , Sharon C Glotzer

This paper reviews the current state-of-the-art in the simulation of the mechanical behavior of polycrystalline materials by means of computational homogenization. The key ingredients of this modelling strategy are presented in detail…

材料科学 · 物理学 2018-11-22 J. Segurado , R. A. Lebensohn , J. LLorca

Soft particles display highly versatile properties with respect to hard colloids, even more so at fluid-fluid interfaces. In particular, microgels, consisting of a cross-linked polymer network, are able to deform and flatten upon adsorption…

Herein, we describe new methods to produce colloidal particle chains of three stiffness regimes that can be observed on a single-particle level, that is, on the level of the monomers that make up the chain; the chains can even be observed…

When colloids flow in a narrow channel, the transport efficiency is controlled by the non-equilibrium interplay between colloid-wall interactions and hydrodynamics. In this paper, a general, unifying description of colloidal dispersion flow…

流体动力学 · 物理学 2018-06-12 Patrice Bacchin

A robust route for the biased production of single-handed chiral structures has been found in generating non-spherical, multi-component double emulsions using microfluidics. The specific type of handedness is determined by the final packing…

软凝聚态物质 · 物理学 2018-04-20 Laura L. A. Adams , Samuel A. Ocko

In microfluidic devices, inertia drives particles to focus on a finite number of inertial focusing streamlines. Particles on the same streamline interact to form one-dimensional microfluidic crystals (or "particle trains"). Here we develop…

流体动力学 · 物理学 2018-09-12 Kaitlyn Hood , Marcus Roper

From dumbbells to FCC crystals, we study the self-assembly pathway of amphiphatic, spherical colloidal particles as a function of the size of the hydrophobic region using molecular dynamics simulations. Specifically, we analyze how local…

软凝聚态物质 · 物理学 2015-05-13 William L. Miller , Angelo Cacciuto

Colloidal particles that are confined to an interface such as the air-water interface are an example of a two-dimensional fluid. Such dispersions have been observed to spontaneously form cluster and stripe morphologies in certain systems…

软凝聚态物质 · 物理学 2008-09-17 A. J. Archer

We simulate structural phase behavior of polymer-grafted colloidal particles by molecular Monte Carlo technique. Interparticle potential, which has a finite repulsive square-step outside a rigid core of the colloid, was previously confirmed…

软凝聚态物质 · 物理学 2015-03-19 Yuki Norizoe , Toshihiro Kawakatsu

Extreme deformation of soft matter is central to our understanding of the effects of shock, fracture, and phase change in a variety of systems. Yet, despite, the increasing interest in this area, far-from-equilibrium behaviours of soft…

软凝聚态物质 · 物理学 2020-07-07 Axel Huerre , Marco De Corato , Valeria Garbin

The spontaneous assembly of particles in suspension provides a strategy for inexpensive fabrication of devices with nanometer-scale control, such as single-electron transistors for memory or logic applications. A scaleable and robust method…