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In this paper we present a review on our recent experimental investigations into the phase behavior of the deeply cooled water confined in a nanoporous silica material, MCM-41, with elastic neutron scattering technique. Under such strong…

软凝聚态物质 · 物理学 2016-12-13 Zhe Wang , Kanae Ito , Sow-Hsin Chen

We investigate a one-dimensional model that shows several properties of water. The model combines the long-range attraction of the van der Waals model with the nearest-neighbor interaction potential by Ben-Naim, which is a step potential…

统计力学 · 物理学 2012-09-28 Lotta Heckmann , Barbara Drossel

We study indented spherical colloids, interacting via depletion forces. These systems exhibit liquid-vapor phase transitions whose properties are determined by a combination of strong "lock-and-key" bonds and weaker non-specific…

软凝聚态物质 · 物理学 2015-06-17 Douglas J. Ashton , Robert L. Jack , Nigel B. Wilding

Liquid-liquid phase separation has recently emerged as an important topic in the context of cellular organization. Within this context, there are multiple poorly understood features; for instance hints of critical behavior in the plasma…

统计力学 · 物理学 2024-06-25 Felix Herrmann , Burkhard Dünweg , Martin Girard

We construct a phase field model including hydrodynamics and elasticity in one-component systems. It can be used to investigate solid-liquid and liquid-liquid phase transitions. Upon first-order phase transition, a velocity field is induced…

软凝聚态物质 · 物理学 2015-03-13 Kyohei Takae , Akira Onuki

We determine the phase diagram for a generalisation of two-and three-dimensional hard spheres: a classical system with three-body interactions realised as a hard cut-off on the mean-square distance for each triplet of particles. Quantum…

统计力学 · 物理学 2015-02-06 Tommaso Comparin , Sebastian C. Kapfer , Werner Krauth

We investigate the structural properties of liquid water at near ambient conditions using first-principles molecular dynamics simulations based on a semilocal density functional augmented with nonlocal van der Waals interactions. The…

软凝聚态物质 · 物理学 2016-08-01 Giacomo Miceli , Stefano de Gironcoli , Alfredo Pasquarello

The dynamics of a thin layer of liquid, between a flat solid substrate and an infinitely-thick layer of saturated vapor, is examined. The liquid and vapor are two phases of the same fluid, governed by the diffuse-interface model. The…

统计力学 · 物理学 2021-09-27 E. S. Benilov

The electrostatic interaction in ionic fluids is well-known to give rise to a characteristic phase behavior and structure. Sometimes its long range is proposed to single out the electrostatic potential over other interactions with shorter…

软凝聚态物质 · 物理学 2015-05-05 Hendrik Bartsch , Oliver Dannenmann , Markus Bier

We study a model in which particles interact through a hard-core repulsion complemented by a short-ranged attractive potential, of the kind found in colloidal suspensions. Combining theoretical and numerical work we locate the line of…

无序系统与神经网络 · 物理学 2009-11-10 Francesco Sciortino , Piero Tartaglia , Emanuela Zaccarelli

For a fluid of convex hard particles, characterized by a length scale $\sigma_\text{min}$ and an anisotropy parameter $\epsilon$, we develop a formalism allowing one to relate thermodynamic quantities to the body's shape. In a first step…

统计力学 · 物理学 2025-06-17 Thomas Franosch , Cristiano De Michele , Rolf Schilling

For one-component fluids, we predict a pre-dewetting phase transition between a thin and thick low-density layer in liquid on a wall repelling the fluid. This is the case of a hydrophobic wall for water. A pre-dewetting line starts from the…

软凝聚态物质 · 物理学 2015-05-30 Ryohei Teshigawara , Akira Onuki

A simulation model is presented, comprising elastic spheres with a short range attraction. Besides conservative forces, radial- and shear friction, and radial noise are added. The model can be used to simulate colloids, granular solids and…

软凝聚态物质 · 物理学 2008-11-19 Robert D. Groot , Simeon D. Stoyanov

Computational studies of liquid water and its phase transition into vapor have traditionally been performed using classical water models. Here we utilize the Deep Potential methodology -- a machine learning approach -- to study this…

Many physical systems, including classical fluids, present in their phase diagram the competition between two phases that are separated by a line of first-order phase transitions which terminates at a so-called critical point. Despite…

高能物理 - 理论 · 物理学 2025-04-29 Zi-Qiang Zhao , Zhang-Yu Nie , Jing-Fei Zhang , Xin Zhang , Matteo Baggioli

When non-adsorbing polymers are added to an isotropic suspension of rod-like colloids, the colloids effectively attract each other via depletion forces. We performed Monte Carlo simulations to study the phase diagram of such rod-polymer…

软凝聚态物质 · 物理学 2009-11-13 S. Jungblut , R. Tuinier , K. Binder , T. Schilling

Much attention has been devoted to water's metastable phase behavior, including polyamorphism (multiple amorphous solid phases), and the hypothesized liquid-liquid transition and associated critical point. However, the possible relationship…

软凝聚态物质 · 物理学 2021-06-09 Thomas E. Gartner , Salvatore Torquato , Roberto Car , Pablo G. Debenedetti

In this letter, we examine the virial and the potential energy correlation for the quasi-real model system. This correlation constitutes the framework of the theory of the isomorph in the liquid phase diagram commonly examined using…

软凝聚态物质 · 物理学 2020-12-29 K. Koperwas , A. Grzybowski , M. Paluch

The transition from a liquid to a glass in colloidal suspensions of particles interacting through a hard core plus an attractive square-well potential is studied within the mode-coupling-theory framework. When the width of the attractive…

软凝聚态物质 · 物理学 2007-05-23 K. Dawson , G. Foffi , M. Fuchs , W. Gotze , F. Sciortino , M. Sperl , P. Tartaglia , Th. Voigtmann , E. Zaccarelli

We study the statistical properties of two hard spheres in a two dimensional rectangular box. In this system, the relation like Van der Waals equation loop is obtained between the width of the box and the pressure working on side walls. The…

凝聚态物理 · 物理学 2009-10-31 Akinori Awazu