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Computationally inexpensive approximations describing electron-phonon scattering in molecular-scale conductors are derived from the non-equilibrium Green's function method. The accuracy is demonstrated with a first principles calculation on…

介观与纳米尺度物理 · 物理学 2007-05-23 Magnus Paulsson , Thomas Frederiksen , Mads Brandbyge

We describe a first-principles method for calculating electronic structure, vibrational modes and frequencies, electron-phonon couplings, and inelastic electron transport properties of an atomic-scale device bridging two metallic contacts…

介观与纳米尺度物理 · 物理学 2007-05-23 Thomas Frederiksen , Magnus Paulsson , Mads Brandbyge , Antti-Pekka Jauho

We present a scattering theory description for the inelastic current noise in the presence of electron-vibration interactions. In this description, we specify elastic and inelastic scattering contributions to the shot noise by examining…

介观与纳米尺度物理 · 物理学 2017-09-15 Sejoong Kim

The lattice dynamics of the metallic tin {\beta} and {\gamma} polymorphs has been studied by a combination of diffuse scattering, inelastic x-ray scattering and density functional perturbation theory. The non-symmorphic space group of the…

Electron-phonon interaction is of central importance for the electrical and heat transport properties of metals, and is directly responsible for charge-density-waves or (conventional) superconducting instabilities. The direct observation of…

超导电性 · 物理学 2022-02-02 S. M. Souliou , A. Bosak , G. Garbarino , M. Le Tacon

Inelastic phonon scattering in graphene field-effect transistors (FETs) is studied by numerically solving the Boltzmann transport equation in three dimensional real and phase spaces (x, kx, ky). A kink behavior due to ambipolar transport…

介观与纳米尺度物理 · 物理学 2015-05-27 Jyotsna Chauhan , Jing Guo

We consider a model for a spin field-effect molecular transistor, where a directed pure spin current is controlled by an external electric field. Inelastic scattering effects of such molecular device are discussed within a framework of full…

介观与纳米尺度物理 · 物理学 2010-02-17 Jonas Fransson , Michael Galperin

We have measured the differential resistance of mesoscopic gold wires of different lengths connected to an aluminum superconductor as a function of temperature and voltage. Our experimental results differ substantially from theoretical…

介观与纳米尺度物理 · 物理学 2009-10-31 M. J. Black , V. Chandrasekhar

Our objective is to study resonant tunneling of an electron in the presence of inelastic scattering by optical phonons. Using a recently developed technique, based on exact mapping of a many-body problem onto a one-body problem, we compute…

介观与纳米尺度物理 · 物理学 2009-10-31 K. Haule , J. Bonca

We present series of first-principles calculations for both pure and hydrogen contaminated gold wire systems in order to investigate how such impurities can be detected. We show how a single H atom or a single H2 molecule in an atomic gold…

介观与纳米尺度物理 · 物理学 2007-05-23 Thomas Frederiksen , Magnus Paulsson , Mads Brandbyge

Ab initio modeling of molecular electronics is nowadays routinely performed by combining the Density Functional Theory (DFT) and Nonequilibrium Green function (NEGF) techniques. This method has its roots in the current formula given by Meir…

介观与纳米尺度物理 · 物理学 2009-11-11 A. P. Jauho

We present a technique to calculate the transport properties through one-dimensional models of molecular wires. The calculations include inelastic electron scattering due to electron-lattice interaction. The coupling between the electron…

凝聚态物理 · 物理学 2009-10-31 H. Ness , S. A. Shevlin , A. J. Fisher

Inelastic light scattering from electrons is a symmetry-selective probe of the charge dynamics within correlated materials. Many measurements have been made on correlated insulators, and recent exact solutions in large dimensions explain a…

强关联电子 · 物理学 2009-11-07 J. K. Freericks , T. P. Devereaux , R. Bulla , Th. Pruschke

We describe how to treat the interaction of travelling electrons with localised vibrational modes in nanojunctions. We present a multichannel scattering technique which can be applied to calculate the transport properties for realistic…

介观与纳米尺度物理 · 物理学 2007-05-23 H. Ness , A. J. Fisher

We calculate the inelastic scattering probabilities in the wide band limit of a local polaron model with quadratic coupling to bosons. The central object is a two-particle Green function which is calculated exactly using a purely algebraic…

材料科学 · 物理学 2010-03-25 Thomas Olsen

We present here a theoretical method to determine the phononic contribution to the thermal conductance of nanoscale systems in the phase-coherent regime. Our approach makes use of classical molecular dynamics (MD) simulations to calculate…

介观与纳米尺度物理 · 物理学 2022-11-09 Fabian Müller , Peter Nielaba , Juan Carlos Cuevas , Fabian Pauly

Detailed understanding of vibrational heat transfer mechanisms between solids is essential for the efficient thermal engineering and control of nanomaterials. We investigate the frequency dependence of anharmonic scattering and interfacial…

材料科学 · 物理学 2014-10-31 K. Sääskilahti , J. Oksanen , J. Tulkki , S. Volz

A method is proposed for studying wave and particle transport in disordered waveguide systems of dimension higher than unity by means of exact one-dimensionalization of the dynamic equations in the mode representation. As a particular case,…

无序系统与神经网络 · 物理学 2013-01-31 Yu. V. Tarasov

Using first-principles approaches we investigate local heating and the inelastic contribution to the current for various alkanethiols sandwiched between metal electrodes. In the absence of good heat dissipation into the bulk electrodes, we…

介观与纳米尺度物理 · 物理学 2015-06-24 Yu-Chang Chen , Michael Zwolak , Massimiliano Di Ventra

We report a theoretical study on the inelastic Coulomb scattering rate of an injected electron in two coupled quantum wires in quasi-one-dimensional doped semiconductors. Two peaks appear in the scattering spectrum due to the optical and…

强关联电子 · 物理学 2009-10-31 Marcos R. S. Tavares , Guo-Qiang Hai
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