相关论文: How systems of single-molecule magnets magnetize a…

We show that correlations established before quenching to very low temperatures, later drive the magnetization process of systems of single molecule magnets, after a magnetic field is applied at t=0. We also show that in SC lattices, m…

Precise magnetic hysteresis measurements of small single crystals of Mn$_{12}$ acetate of spin 10 have been conducted down to 0.4 K using a high sensitivity Hall magnetometer. At higher temperature (>1.6K) step-like changes in magnetization…

We have studied the crossover between thermally assisted and pure quantum tunneling in single crystals of high spin (S=10) uniaxial single molecule magnet Mn12-acetate using micro-Hall effect magnetometry. Magnetic hysteresis experiments…

Single molecule magnets straddle the classical and quantum mechanical worlds, displaying many fascinating phenomena. They may have important technological applications in information storage and quantum computation. We review the physical…

We use neutron diffraction to probe the magnetization components of a crystal of Mn12 single-molecule magnets. Each of these molecules behaves, at low temperatures, as a nanomagnet with spin S = 10 and strong anisotropy along the…

We report results from Monte Carlo simulations of systems of magnetic dipoles that relax through quantum tunneling, much as Fe_8 crystals at very low temperature.For short times, a hole develops in suitably defined magnetic field…

In this paper, we combine thermal effects with Landau-Zener (LZ) quantum tunneling effects in a dynamical Monte Carlo (DMC) framework to produce satisfactory magnetization curves of single-molecule magnet (SMM) systems. We use the giant…

We study the magnetic relaxation of a system of localized spins interacting through weak dipole interactions, at a temperature large with respect to the ordering temperature but low with respect to the crystal field level splitting. The…

The low temperature spin dynamics of a Fe8 Single-Molecule Magnet was studied under circularly polarized electromagnetic radiation allowing us to establish clearly photon-assisted tunneling. This effect, while linear at low power, becomes…

We study the relaxation of interacting single--molecule magnets (SMMs) in both spatially ordered and disordered systems. The tunneling window is assumed to be, as in Fe8, much narrower than the dipolar field spread. We show that relaxation…

The low temperature relaxation of the magnetization in magnetic molecular solids such as Fe$_8$ is studied using Monte Carlo simulations. A set of rate equations is developed to understand the simulations, and the results are compared. The…

The magnetic behavior of the Ca3Co2O6 spin chain compound is characterized by a large Ising-like character of its ferromagnetic chains, set on triangular lattice, that are antiferromagnetically coupled. At low temperature, T < 7K, the 3D…

We examine the quantum tunneling of magnetization in molecular spin in weak interaction with a bath subject to Redfield master equation. By designing a microscopic model for a multilevel spin system using only a generic Hamiltonian and…

Here, a dynamical Monte-Carlo (DMC) method is used to study temperature-dependent dynamical magnetization of famous Mn2Ni system as typical example of single-chain magnets with strong magnetic anisotropy. Simulated magnetization curves are…

Tunneling of the spins in the Fe$_8$ molecular magnet from a metastable ground state to an excited state is accompanied by a decay of these spins to the global ground state, and an increase of the crystal temperature. We measured this…

The field sweep rate (v=dH/dt) and temperature (T) dependence of the magnetization reversal of a single-chain magnet (SCM) is studied at low temperatures. As expected for a thermally activated process, the nucleation field (H_n) increases…

We present a quantum interpretation of the heights in hysteresis of $Fe_{8}$ molecule at lower temperatures by treating the crystal as an Ising spin system with the dipolar interaction between spins. Then we apply it to two limit cases :…

We argue that to explain recent resonant tunneling experiments on crystals of Mn$_{12}$ and Fe$_8$, particularly in the low-T limit, one must invoke dynamic nuclear spin and dipolar interactions. We show the low-$T$, short-time relaxation…

We study low temperature resonant spin tunneling in molecular magnets induced by a field sweep with account of dipole-dipole interactions. Numerical simulations uncovered formation of self-organized patterns of the magnetization and of the…

We present high-frequency angle-dependent EPR data for crystals of [NixZn1-x(hmp)(t-BuEtOH)Cl]4 (x = 1 and 0.02). The x = 1 complex behaves as a single-molecule magnet at low temperatures, displaying hysteresis and exceptionally fast…