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Redox molecular junctions are molecular conduction junctions that involve more than one oxidation state of the molecular bridge. This property is derived from the ability of the molecule to transiently localize transmitting electrons,…

介观与纳米尺度物理 · 物理学 2013-06-21 Agostino Migliore , Abraham Nitzan

A kinetic equation for a dilute gas of hard spheres confined between two parallel plates separated a distance smaller than two particle dimeters is derived. It is a Boltzmann-like equation, which incorporates the effect of the confinement…

统计力学 · 物理学 2016-11-23 J. Javier Brey , P. Maynar , M. I. García de Soria

A new kinetic instability which results in formation of charge density waves is proposed. The instability is of a purely classical nature. A spatial period of arising space-charge and field configuration is inversely proportional to…

软凝聚态物质 · 物理学 2009-11-07 V. Yu. Kachorovskii , I. S. Lioublinskii , L. D. Tsendin

These are notes for lectures delivered at the NATO ASI on Dynamics in Leiden, The Netherlands, in July 1998. The quantum kinetic theory for noninteracting electrons in a disordered solid is introduced and discussed. We first use many-body…

统计力学 · 物理学 2007-05-23 T. R. Kirkpatrick , D. Belitz

Inelastic effects in electron transport through nano-sized devices are addressed with a method based on nonequilibrium Green's functions (NEGF) and perturbation theory to infinite order in the electron-vibration coupling. We discuss the…

介观与纳米尺度物理 · 物理学 2007-05-23 Thomas Frederiksen , Mads Brandbyge , Nicolas Lorente , Antti-Pekka Jauho

We present a new way of quantum kinetic equation derivation. This method appears as a natural generalization of the many-particle quantum hydrodynamic method. Kinetic equations are derived for different system of particles. First of all we…

等离子体物理 · 物理学 2012-12-04 Pavel A. Andreev

Electrokinetic flows of an aqueous NaCl solution in nanochannels with negatively charged surfaces are studied using molecular dynamics (MD) simulations. The four transport coefficients that characterise the response to weak electric and…

化学物理 · 物理学 2014-06-05 Hiroaki Yoshida , Hideyuki Mizuno , Tomoyuki Kinjo , Hitoshi Washizu , Jean-Louis Barrat

Geometric symmetries cause orbital degeneracies in a molecule's spectrum. In a single-molecule junction, these degeneracies are lifted by various symmetry-breaking effects. We study quantum transport through such nanostructures with an…

介观与纳米尺度物理 · 物理学 2013-05-29 Maximilian G. Schultz , Felix von Oppen

Understanding electron energy dynamics in low-temperature plasmas such as capacitively coupled plasmas (CCPs), including energy absorption, conversion, transport, and dissipation, is essential for interpreting discharge physics and process…

等离子体物理 · 物理学 2026-01-23 Jianxiong Yao , Zeduan Zhang , Feng He , Jinsong Miao , Jiting Ouyang , Bocong Zheng

Recent studies have utilized AC fields and electrochemical reactions in multicomponent electrolyte solutions to control colloidal assembly. However, theoretical investigations have thus far been limited to binary electrolytes and have…

软凝聚态物质 · 物理学 2023-08-15 Nathan Jarvey , Filipe Henrique , Ankur Gupta

We present an ab initio inelastic quantum transport approach based on maximally localized Wannier functions. Electronic-structure properties are calculated with density-functional theory in a planewave basis, and electron-vibration coupling…

介观与纳米尺度物理 · 物理学 2013-06-12 Sejoong Kim , Nicola Marzari

The thermoelectric transport properties of nanostructured devices continue to attract attention from theorists and experimentalist alike as the spatial confinement allows for a controlled approach to transport properties of correlated…

强关联电子 · 物理学 2015-06-12 Stefan Kirchner , Farzaneh Zamani , Enrique Muñoz

Vibrationally inelastic electron transport through a molecular bridge that is connected to two leads is investigated. The study is based on a generic model of vibrational excitation in resonant transmission of electrons through a molecular…

介观与纳米尺度物理 · 物理学 2009-11-10 Martin Cizek , Michael Thoss , Wolfgang Domcke

Exposing a molecule to intense light pulses may bring this molecule to a nonstationary quantum state, thus launching correlated dynamics of electronic and nuclear subsystems. Although much had been achieved in the understanding of…

化学物理 · 物理学 2024-04-11 Nikolay V. Golubev , Jiří Vaníček

A method for increasing the accuracy of configuration interaction (CI) calculations of molecules and other electronic systems is proposed. The energy defect of a given calculation is associated with the electron pair origin of…

化学物理 · 物理学 2025-11-18 Jerry L. Whitten

Electric, thermal and thermoelectric transport in correlated electron systems probe different aspects of the many-body dynamics, and thus provide complementary information. These are well studied in the low- and high-temperature limits,…

强关联电子 · 物理学 2020-02-19 Woo-Ram Lee , Alexander M. Finkel'stein , Karen Michaeli , Georg Schwiete

The ultimate goal of electronic structure calculations is to make the left and right hand sides of the titled ``equation'' as close as possible. This requires high-precision treatment of relativistic, correlation, and quantum…

化学物理 · 物理学 2022-10-10 Wenjian Liu

In many situations, one can approximate the behavior of a quantum system, i.e. a wave function subject to a partial differential equation, by effective classical equations which are ordinary differential equations. A general method and…

数学物理 · 物理学 2007-05-23 Martin Bojowald , Aureliano Skirzewski

The electron transport in a 1D conductor with an isolated local defect such as an impurity or a non-adiabatic contact is studied theoretically. New regime of conduction in correlated 1D systems is predicted beyond the well-known regime of…

强关联电子 · 物理学 2015-10-01 S. N. Artemenko , P. P. Aseev , D. S. Shapiro , R. R. Vakhitov

We study the Kondo effect in the electron transport through a quantum dot coupled to ferromagnetic leads, using a real-time diagrammatic technique which provides a systematic description of the nonequilibrium dynamics of a system with…

介观与纳米尺度物理 · 物理学 2007-05-23 Yasuhiro Utsumi , Jan Martinek , Gerd Schön , Hiroshi Imamura , Sadamichi Maekawa