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A new relaxation mechanism is shown to arise from overdamped two-level systems above a critical temperature $T^*\approx 5$ K, thus yielding an explanation for experimental observations in dielectric glasses in the temperature range between…

凝聚态物理 · 物理学 2009-10-22 Peter Neu , Alois Würger

The relaxation dynamics and thermodynamic properties of supercooled and glassy gambogic acid are investigated using both theory and experiment. We measure the temperature dependence of the relaxation times in three polymorphs (alpha-,…

Within the mode-coupling theory (MCT) for the evolution of structural relaxation in glass-forming liquids, correlation functions and susceptibility spectra are calculated characterizing the rotational dynamics of a top-down symmetric…

软凝聚态物质 · 物理学 2015-06-24 W. Gotze , A. P. Singh , Th. Voigtmann

The shear flow and the dielectric alpha-process in molecular glass formers is modeled in terms of local structural rearrangements which reverse a strong local shear. Using Eshelby's solution of the corresponding elasticity theory problem…

无序系统与神经网络 · 物理学 2009-09-24 U. Buchenau

We study the relaxation dynamics of a compressible bilayer vesicle with an asymmetry in the viscosity of the inner and outer fluid medium. First we explore the stability of the vesicle free energy which includes a coupling between the…

软凝聚态物质 · 物理学 2017-01-03 T. V. Sachin Krishnan , Ryuichi Okamoto , Shigeyuki Komura

We address the relaxation dynamics in hydrogen-bonded super-cooled liquids near the glass transition, measured via Broad-Band Dielectric Spectroscopy (BDS). We propose a theory based on decomposing the relaxation of the macroscopic dipole…

软凝聚态物质 · 物理学 2009-11-13 H. G. E. Hentschel , Itamar Procaccia

Glass-forming liquids display strong fluctuations -- dynamical heterogeneities -- near their glass transition. By numerically simulating a binary Weeks-Chandler-Andersen liquid and varying both temperature and timescale, we investigate the…

无序系统与神经网络 · 物理学 2011-08-15 Azita Parsaeian , Horacio E. Castillo

Studying the primary {\alpha}- and secondary {\beta}-relaxation process has contributed significantly to the understanding of the structure and rheology of metallic glasses. In this letter, we report on a third relaxation mechanism…

材料科学 · 物理学 2017-03-28 Stefan Küchemann , Robert Maaß

An analytically tractable model is introduced which exhibits both, a glass--like freezing transition, and a collection of double--well configurations in its zero--temperature potential energy landscape. The latter are generally believed to…

凝聚态物理 · 物理学 2009-10-28 Reimer Kuehn

The recently developed pragmatical model of asymmetric double-well potentials with a finite lifetime is applied to nonlinear dielectric data in polar undercooled liquids. The viscous effects from the finite lifetime provide a crossover from…

无序系统与神经网络 · 物理学 2017-05-23 U. Buchenau

While deeply supercooled liquids exhibit divergent viscosity and increasingly heterogeneous dynamics as the temperature drops, their structure shows only seemingly marginal changes. Understanding the nature of relaxation processes in this…

材料科学 · 物理学 2022-11-03 Matthias Lerbinger , Armand Barbot , Damien Vandembroucq , Sylvain Patinet

We study the solid-to-liquid transition in a two-dimensional fully periodic soft-glassy model with an imposed spatially heterogeneous stress. The model we consider consists of droplets of a dispersed phase jammed together in a continuous…

软凝聚态物质 · 物理学 2018-06-06 Matteo Lulli , Roberto Benzi , Mauro Sbragaglia

The dynamical glass transition is typically taken to be the temperature at which a glassy liquid is no longer able to equilibrate on experimental timescales. Consequently, the physical properties of these systems just above or below the…

软凝聚态物质 · 物理学 2017-03-08 Samuel S. Schoenholz , Ekin D. Cubuk , Efthimios Kaxiras , Andrea J. Liu

We analyze a simple dynamical model of glasses, based on the idea that each particle is trapped in a local potential well, which itself evolves due to hopping of neighbouring particles. The glass transition is signalled by the fact that the…

凝聚态物理 · 物理学 2009-10-28 Jean-Philippe Bouchaud , Alain Comtet , Cécile Monthus

The incoherent dynamic structure factor of ortho-terphenyl has been measured by neutron time-of-flight and backscattering technique in the pressure range from 0.1 MPa to 240 MPa for temperatures between 301 K and 335 K. Tagged-particle…

统计力学 · 物理学 2011-04-05 A. Toelle , H. Schober , J. Wuttke , F. Fujara

It is shown that the dynamics of a two-dimensional crystal with a finite concentration of dislocations, as well as vacancy and interstitial defects, is governed by the hydrodynamic equations of a viscoelastic medium. At the longest length…

软凝聚态物质 · 物理学 2009-11-07 M. Cristina Marchetti , Karl Saunders

Glasses are out-of-equilibrium systems aging under the crystallization threat. During ordinary glass formation, the atomic diffusion slows down rendering its experimental investigation impractically long, to the extent that a timescale…

无序系统与神经网络 · 物理学 2015-08-28 E. A. A. Pogna , C. Rodríguez-Tinoco , G. Cerullo , C. Ferrante , J. Rodríguez-Viejo , T. Scopigno

We investigate the heterogeneous dynamics in a model, where chemical gelation and glass transition interplay, focusing on the dynamical susceptibility. Two independent mechanisms give raise to the correlations, which are manifested in the…

软凝聚态物质 · 物理学 2017-05-09 Antonio de Candia , Annalisa Fierro , Raffaele Pastore , Massimo Pica Ciamarra , Antonio Coniglio

The stability to dislocations of the elastic phase, or ``Bragg glass'', of a randomly pinned elastic medium in two dimensions is studied using the minimum-cost-flow algorithm for a disordered fully-packed loop model. The elastic phase is…

无序系统与神经网络 · 物理学 2009-10-31 Chen Zeng , Paul L. Leath , Daniel S. Fisher

We report a molecular dynamics simulation study of a model gel whose interaction potential is obtained by modifying the three body Stillinger-Weber model potential for silicon. The modification reduces the average coordination number, and…

软凝聚态物质 · 物理学 2015-05-14 Shibu Saw , Niels L. Ellegaard , Walter Kob , Srikanth Sastry