相关论文: Proton Spin Relaxation Induced by Quantum Tunnelin…
The proton nuclear spin-lattice relaxation rate 1/T1 has been measured as a function of temperature and magnetic field (up to 15 T) in the molecular magnetic ring Fe10. Striking enhancement of 1/T1 is observed around magnetic field values…
$^{57}$Fe and $^1$H relaxation measurements have been performed in single crystal and oriented powder of enriched $^{57}$Fe8 molecular cluster in the temperature range 0.05--1.7 K in zero external field and with small perturbing…
Measurements of proton NMR and the spin lattice relaxation rate 1/T1 in the octanuclear iron (III) cluster [Fe8(N3C6H15)6O2(OH)12][Br8 9H2O], in short Fe8, have been performed at 1.5 K in a powder sample aligned along the main anisotropy z…
A theoretical interpretation is given to recent proton spin relaxation-time (T_1) measurements on NiCu(C_7H_6N_2O_6)(H_2O)_3$\cdot$2H_2O, which is an ideal one-dimensional ferrimagnetic Heisenberg model system of alternating spins 1 and…
We argue that to explain recent resonant tunneling experiments on crystals of Mn$_{12}$ and Fe$_8$, particularly in the low-T limit, one must invoke dynamic nuclear spin and dipolar interactions. We show the low-$T$, short-time relaxation…
We report measurements of 19F nuclear spin-lattice relaxation 1/T1 as a function of temperature and external magnetic field in LiY0.998Ho0.002F4 single crystal, a single-ion magnet exhibiting interesting quantum effects. The 19F 1/T1 is…
We present an ultra-low temperature study (down to T = 20 mK) of the nuclear spin-lattice relaxation (SLR) in the 55Mn nuclei of the molecular magnet Mn12-ac. The nuclear spins act as local probes for the electronic spin fluctuations, due…
Using X-band pulsed electron spin resonance, we report the intrinsic spin-lattice ($T_1$) and phase coherence ($T_2$) relaxation times in molecular nanomagnets for the first time. In Cr$_7M$ heterometallic wheels, with $M$ = Ni and Mn,…
We investigate the effect of dynamic nuclear spin fluctuation on quantum tunneling of the magnetization (QTM) in the molecular magnet Fe8 by increasing the nuclei temperature using radio frequency (RF) pulses before the hysteresis loop…
We derive a simple system of equations to describe the magnetization relaxation of a molecular spin in weak interaction with a thermal bath for the whole temperature domain. Using this for the intermediate temperature domain where the…
Measurements of proton Nuclear Magnetic Resonance (1H NMR) spectra and relaxation and of Muon Spin Relaxation ($\mu^{+}$SR) have been performed as a function of temperature and external magnetic field on two isostructural lanthanide…
$^{235}$U nuclear spin-lattice ($T_1^{-1}$) and spin-spin ($T_2^{-1}$) relaxation rates in the itinerant antiferromagnet USb$_2$ are reported as a function of temperature in zero field. The heating effect from the intense rf pulses that are…
In response to recent proton spin relaxation-time measurements on NiCu(pba)(H$_2$O)$_3$$\cdot$2H$_2$O with ${pba}=1,3{-propylenebis(oxamato)}$, which is an excellent one-dimensional ferrimagnetic Heisenberg model system of spin-$(1,{1/2})$,…
We present the results of a ^{1}H NMR study of the single-component molecular conductor, [Au(tmdt)_{2}]. A steep increase in the NMR line width and a peak formation of the nuclear spin-lattice relaxation rate, 1/T_{1}, were observed at…
The magnetic state of the single-component molecular compound, [Cu(tmdt)$_{2}$], is investigated by means of $^{1}$H-NMR. An abrupt spectral broadening below 13 K and a sharp peak in nuclear spin-lattice relaxation rate, $T_{1}^{-1}$, at 13…
We present muon spin lattice relaxation measurements in the V15 spin 1/2 molecular nano-magnet. We find that the relaxation rate in low magnetic fields (<5 kG) is temperature independent below ~10 K, implying that the molecular spin is…
The magnetic properties of dilute Li$_2$(Li$_{1-x}$Fe$_x$)N with $x \sim 0.001$ are dominated by the spin of single, isolated Fe atoms. Below $T = 10$ K the spin-relaxation times become temperature-independent indicating a crossover from…
We conducted $^{77}$Se-nuclear magnetic resonance studies of the iron-based superconductor FeSe in magnetic fields of 0.6 to 19 T to investigate the superconducting and normal-state properties. The nuclear spin-lattice relaxation rate…
We study the nuclear magnetic resonance (NMR) spin-lattice relaxation rate $1/T_1$ in random one-dimensional spin chains as function of the temperature and disorder strength. In the zero temperature limit, the system displays a…
A new mechanism is proposed for the magnetization reversal of molecular nanomagnets such as \Fe8. In this process the spin tunnels from the lowest state near one easy direction to the first excited state near the opposite easy direction,…