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The interrelations between short range structural and elastic aspects in glasses and glass forming liquids pose important and yet unresolved questions. In this paper these relations are analyzed for mono-atomic glasses and stressed liquids…

无序系统与神经网络 · 物理学 2009-10-31 Tamar Kustanovich , Zeev Olami

In a recent paper [S. Mandal et al., Phys. Rev. E 88, 022129 (2013)] the nature of spatial correlations of plasticity in hard sphere glasses was addressed both via computer simulations and in experiments. It was found that the…

Glasses behave as solids on experimental time scales due to their slow relaxation. Growing dynamic length scales due to cooperative motion of particles are believed to be central to this slow response. For quiescent glasses, however, the…

软凝聚态物质 · 物理学 2015-05-30 Vijayakumar Chikkadi , Gerard Wegdam , Daniel Bonn , Bernard Nienhuis , Peter Schall

One of the central problems of the liquid-glass transition is whether there is a structural signature that can qualitatively distinguish different dynamic behaviors at different degrees of supercooling. Here, we propose a novel structural…

软凝聚态物质 · 物理学 2015-09-24 Yan-Wei Li , You-Liang Zhu , Zhao-Yan Sun

There is growing evidence that the flow of driven amorphous solids is not homogeneous, even if the macroscopic stress is constant across the system. Via event driven molecular dynamics simulations of a hard sphere glass, we provide the…

软凝聚态物质 · 物理学 2015-06-04 Suvendu Mandal , Markus Gross , Dierk Raabe , Fathollah Varnik

Glasses at low temperature fluctuate around their inherent states; glassy anomalies reflect the structure of these states. Recently there have been numerous observations of long-range stress correlations in glassy materials, from…

无序系统与神经网络 · 物理学 2018-09-12 E. DeGiuli

The structural description for the intriguing link between the fast vibrational dynamics and slow diffusive dynamics in glass-forming systems is one of the most challenging issues in physical science. Here, in a model of metallic…

无序系统与神经网络 · 物理学 2017-08-09 Z. W. Wu , W. H. Wang , Limei Xu

We rigorously establish that, in disordered three-dimensional (3D) isotropic solids, the stress autocorrelation function presents anisotropic terms that decay as $1/r^3$ at long-range, with $r$ the distance, as soon as either pressure or…

软凝聚态物质 · 物理学 2018-08-06 Anaël Lemaître

We study theoretically and numerically a family of multi-point dynamic susceptibilities that quantify the strength and characteristic lengthscales of dynamic heterogeneities in glass-forming materials. We use general theoretical arguments…

Identifying heterogeneous structures in glasses --- such as localized soft spots --- and understanding structure-dynamics relations in these systems remain major scientific challenges. Here we derive an exact expression for the local…

软凝聚态物质 · 物理学 2017-08-16 Jacques Zylberg , Edan Lerner , Yohai Bar-Sinai , Eran Bouchbinder

Simulation studies of the atomic shear stress in the local potential energy minima (inherent structures) are reported for binary liquid mixtures in 2D and 3D. These inherent structure stresses are fundamental to slow stress relaxation and…

软凝聚态物质 · 物理学 2016-04-20 Sadrul Chowdhury , Sneha Abraham , Toby Hudson , Peter Harrowell

Dynamic heterogeneity as one of the most important properties in supercooled liquids has been found for several decades. However, its structural origin remains open for many systems. Here, we propose a new structural parameter to…

无序系统与神经网络 · 物理学 2015-10-16 S. P. Pan , S. D. Feng , J. W. Qiao , W. M. Wang , J. Y. Qin

We show that a number of model liquids at fixed volume exhibit strong correlations between equilibrium fluctuations of the configurational parts of (instantaneous) pressure and energy. We present detailed results for thirteen systems,…

软凝聚态物质 · 物理学 2009-11-13 Nicholas P. Bailey , Ulf R. Pedersen , Nicoletta Gnan , Thomas B. Schrøder , Jeppe C. Dyre

We image local structural rearrangements in soft colloidal glasses under small periodic perturbations induced by thermal cycling. Local structural entropy $S_{2}$ positively correlates with observed rearrangements in colloidal glasses. The…

软凝聚态物质 · 物理学 2016-06-13 Xiunan Yang , Rui Liu , Mingcheng Yang , Wei-Hua Wang , Ke Chen

Glass-forming liquids grow dramatically sluggish upon cooling. This slowdown has long been thought to be accompanied by a growing correlation length. Characteristic dynamical and static length scales, however, have been observed to grow at…

无序系统与神经网络 · 物理学 2016-08-22 Patrick Charbonneau , Ethan Dyer , Jaehoon Lee , Sho Yaida

If a liquid is cooled rapidly to form a glass, its structural relaxation becomes retarded, producing a drastic increase in viscosity. In two dimensions, strong long-wavelength fluctuations persist, even at low temperature, making it…

软凝聚态物质 · 物理学 2019-12-25 Hayato Shiba , Takeshi Kawasaki , Kang Kim

The existence of a generalized fluctuation-dissipation theorem observed in simulations and experiments performed in various glassy materials is related to the concepts of local equilibration and heterogeneity in space. Assuming the…

统计力学 · 物理学 2009-11-10 Ludovic Berthier

We use a confocal microscope to examine the motion of individual particles in a dense colloidal suspension. Close to the glass transition, particle motion is strongly spatially correlated. The correlations decay exponentially with particle…

无序系统与神经网络 · 物理学 2007-08-09 Eric R. Weeks , John C. Crocker , David A. Weitz

We report a detailed experimental study of the structure and dynamics of glassy states in hard spheres with short-range attraction. The system is a suspension of nearly-hard-sphere colloidal particles and non-adsorbing linear polymer which…

软凝聚态物质 · 物理学 2009-11-10 K. N. Pham , S. U. Egelhaaf , P. N. Pusey , W. C. K. Poon

We use Photon Correlation Imaging, a recently introduced space-resolved dynamic light scattering method, to investigate the spatial correlation of the dynamics of a variety of jammed and glassy soft materials. Strikingly, we find that in…

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