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Nanoscale structural and electronic heterogeneities are prevalent in condensed matter physics. Investigating these heterogeneities in three dimensions (3D) has become an important task for understanding their material properties. To provide…

Magneto-optical microscopies, including optical measurements of magnetic circular dichroism, are increasingly ubiquitous tools for probing spin-orbit coupling, charge-carrier g-factors, and chiral excitations in matter, but the minimum…

Recent x-ray absorption experiments have demonstrated the possibility to accurately monitor the magnetism of metallic hetero-structures controlled via a time-independent perturbation caused for example by a static electric field. Using a…

材料科学 · 物理学 2020-09-16 Alberto Marmodoro , Sebastian Wimmer , Ondrej Sipr , Masako Ogura , Hubert Ebert

DNA and proteins are chiral: their three-dimensional structure cannot be superimposed with its mirror image. Circular dichroism spectroscopy is widely used to characterize chiral compounds, but data interpretation is difficult in the case…

生物大分子 · 定量生物学 2020-09-09 Steven Daly , Frederic Rosu , Valerie Gabelica

We report measurements of the electron transport through atomic-scale constrictions and tunnel junctions between ferromagnetic electrodes. Structures are fabricated using a combination of e-beam lithography and controlled electromigration.…

介观与纳米尺度物理 · 物理学 2007-05-23 Z. K. Keane , L. H. Yu , D. Natelson

The occurrence of a noncollinear magnetic structure at a Mn monolayer grown epitaxially on Fe(100) is predicted theoretically, using spinor density-functional theory, and observed experimentally, using x-ray magnetic circular dichroism…

Polarization-dependent photon spectroscopy (dichroism) using signal-enhancing superchiral beams is shown to be sensitive to magnetic properties of the sample, whereas previous investigations explored charge-like electronic properties of…

材料科学 · 物理学 2019-03-06 S. W. Lovesey , J. T. Collins , S. P. Collins

This work reports the measurement of magnetic dichroism in angular-resolved photoemission from in-plane magnetized buried thin films. The high bulk sensitivity of hard X-ray photoelectron spectroscopy (HAXPES) in combination with circularly…

We propose a new microscopy simulation system that can depict atomistic models in a micrograph visual style, similar to results of physical electron microscopy imaging. This system is scalable, able to represent simulation of electron…

定量方法 · 定量生物学 2026-03-27 Ngan Nguyen , Feng Liang , Dominik Engel , Ciril Bohak , Peter Wonka , Timo Ropinski , Ivan Viola

Magnetic circular dichroism (MCD) is a widely used spectroscopic technique which reveals valuable information about molecular geometry and electronic structure. However, the weak signal and the necessary strong magnets impose major…

化学物理 · 物理学 2022-11-16 Jiaan Cao , Lyuzhou Ye , Dawei He , Xiao Zheng , Shaul Mukamel

We propose a novel paradigm to vector magnetometry based on machine learning. Unlike conventional schemes where one measured signal explicitly connects to one parameter, here we encode the three-dimensional magnetic-field information in the…

Chiroptical effects using circularly polarized light produce signals that change sign when switching either molecular handedness (enantiosensitivity) or the light helicity (circular dichroism). Here, we break this…

A microscopic model for the room-temperature multiferroic BiFeO$_3$ that includes two Dzyaloshinskii-Moriya interactions and single-ion anisotropy along the ferroelectric polarization predicts both the zero-field spectroscopic modes as well…

Investigation of magnetic materials using the first-order magneto-optical Kerr effects (MOKE) is well established and is frequently used in the literature. On the other hand, the utilization of the second-order (or quadratic)…

材料科学 · 物理学 2015-06-12 N. Tesarova , J. Subrt , P. Maly , P. Nemec , C. T. Ellis , A. Mukherjee , J. Cerne

We present the classical electromagnetic theory framework of reflection of a light beam carrying Orbital Angular Momentum (OAM) by an in-plane magnetic structure with generic symmetry. Depending on the magnetization symmetry, we find a…

Atomic-scale characterization of spin textures in solids is essential for understanding and tuning properties of magnetic materials and devices. While high-energy electrons are employed for atomic-scale imaging of materials, they are…

材料科学 · 物理学 2023-12-29 Jizhe Cui , Haozhi Sha , Wenfeng Yang , Rong Yu

We propose that X-ray absorption and emission magnetic circular dichroism (XAS-MCD and XES-MCD) are promising measurements to directly detect ferroic higher-rank multipoles as candidate order parameters in altermagnets. Using the sum rules…

强关联电子 · 物理学 2025-09-19 Masaichiro Mizumaki , Norimasa Sasabe , Takayuki Uozumi , Rikuto Oiwa , Hiroaki Kusunose

We demonstrate a combination of computational tools and experimental 4D-STEM methods to image the local magnetic moment in antiferromagnetic Fe$_2$As with 6 angstrom spatial resolution. Our techniques utilize magnetic diffraction peaks,…

Dependence of x-ray magnetic circular dichroism on the experimental geometry is described by a frequency-dependent Hall vector. Using group theory, we derive a general relationship between the Hall vector and the orientation of the N\'eel…

材料科学 · 物理学 2025-11-12 Jan Kuneš

In this work we derive sum rules for orbital angular momentum(OAM) resolved electron magnetic chiral dichroism (EMCD) which enable the evaluation of the strength of spin and orbital components of the atomic magnetic moments in a crystalline…