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There is compelling evidence that charge carriers in organic semiconductors (OSs) self-localize in nano-scale space because of dynamic disorder. Yet, some OSs, in particular recently emerged high-mobility organic molecular crystals, feature…

One of the basic assumptions in organic field-effect transistors, the most fundamental device unit in organic electronics, is that charge transport occurs two-dimensionally in the first few molecular layers near the dielectric interface.…

The anisotropic charge carrier mobilities of two phenancene series compounds such as dibenzo[a,c]picene (DBP) and tribenzo[a,c,k]tetraphene (TBT) is investigated based on the first-principle calculations and Marcus-Hush theory. The…

化学物理 · 物理学 2019-10-28 Smruti R. Sahoo , Rudranarayan Khatua , Suryakanti Debata , Sagar Sharma , Sridha Sahu

We report density-functional theory (DFT), atomistic simulations of the non-equilibrium transport properties of carbon nanotube (CNT) field-effect transistors (FETs). Results have been obtained within a self-consistent approach based on the…

介观与纳米尺度物理 · 物理学 2007-05-23 L. Latessa , A. Pecchia , A. Di Carlo

The one-dimensional confinement of quasiparticles in individual carbon nanotubes (CNTs) leads to extremely anisotropic electronic and optical properties. In a macroscopic ensemble of randomly oriented CNTs, this anisotropy disappears…

The electronic structures of boron nitride nanotubes (BNNTs) doped by organic molecules are investigated with density functional theory. Electrophilic molecule introduces acceptor states in the wide gap of BNNT close to the valence band…

材料科学 · 物理学 2009-11-13 Wei He , Zhenyu Li , Jinlong Yang , J. G. Hou

Single-crystal organic field-effect transistors (OFETs) based on p-channel molecular semiconductors have led to breakthrough carrier mobilities and to the observation of band-like transport. These results represent the limit in our quest…

材料科学 · 物理学 2012-02-10 Nikolas A. Minder , Shimpei Ono , Zhihua Chen , Antonio Facchetti , Alberto F. Morpurgo

The electronic transport of electrons and holes through stacks of $\alpha$,$\ome ga$-dicyano-$\beta$,$\beta$'-dibutyl- quaterthiophene (DCNDBQT) as part of a nov el organic ferroic field-effect transistor (OFFET) is investigated. The novel…

材料科学 · 物理学 2015-05-14 T. Kunze , S. Gemming , V. Pankoke , K. Morawetz , R. Luschtinetz , G. Seifert

Rapid progress in organic electronics demands new highly efficient organic semiconducting materials. Nevertheless, only few materials have been created so far that show reliable band-like transport with high charge mobilities, which…

Organic semiconductors are indispensable for today's display technologies in form of organic light emitting diodes (OLEDs) and further optoelectronic applications. However, organic materials do not reach the same charge carrier mobility as…

软凝聚态物质 · 物理学 2023-10-12 Patrick Reiser , Manuel Konrad , Artem Fediai , Salvador Léon , Wolfgang Wenzel , Pascal Friederich

Solution-processed networks of semiconducting, single-walled carbon nanotubes (SWCNTs) have attracted considerable attention as materials for next-generation electronic devices and circuits. However, the impact of the SWCNT network…

Atomistic modeling of energetic disorder in organic semiconductors (OSCs) and its effects on the optoelectronic properties of OSCs requires a large number of excited-state electronic-structure calculations, a computationally daunting task…

化学物理 · 物理学 2021-05-10 Chengqiang Lu , Qi Liu , Qiming Sun , Chang-Yu Hsieh , Shengyu Zhang , Liang Shi , Chee-Kong Lee

We report charge transport measurements in nanoscale vertical pillar structures incorporating ultrathin layers of the organic semiconductor poly(3-hexylthiophene)(P3HT). P3HT layers with thickness down to 5 nm are gently top-contacted using…

介观与纳米尺度物理 · 物理学 2017-01-16 Janine G. E. Wilbers , Bojian Xu , Peter A. Bobbert , Michel P. de Jong , Wilfred G. van der Wiel

This paper presents a symmetric unified transport (UT) compact model for metal-oxide-semiconductor field-effect transistors (MOSFETs) that bridges drift-diffusion (DD) and ballistic transport (BT) regimes. The proposed model self…

介观与纳米尺度物理 · 物理学 2026-05-27 Chien-Ting Tung

Charge transport in organic semiconductors is notoriously extremely sensitive to the presence of disorder, both internal and external (i.e. related to the interactions with the dielectric layer), especially for n-type materials. Internal…

We investigate the electronic transport properties of semiconducting ($m$,$n$) carbon nanotubes (CNTs) on the mesoscopic length scale with arbitrarily distributed realistic defects. The study is done by performing quantum transport…

介观与纳米尺度物理 · 物理学 2018-11-26 Fabian Teichert , Andreas Zienert , Jörg Schuster , Michael Schreiber

Miniaturized electronics require lightweight conductors that maintain high conductance under demanding conditions. CNT networks are promising candidates, but their transport is governed by inter-nanotube junctions where electron waves…

Organic electrochemical transistors (OECTs) have the potential to revolutionize the field of organic bioelectronics. To date, most of the reported OECTs include p-type (semi-)conducting polymers as the channel material, while n-type OECTs…

This study investigates the impact of exchange-correlation functional choices on the predictive accuracy of multiscale models for charge transport in organic semiconductors (OSCs). A hybrid functional approach is applied to analyze…

材料科学 · 物理学 2025-03-31 Zhongquan Chen , Pim van der Hoorn , Bjoern Baumeier

Curved polycyclic aromatic hydrocarbons (PAHs) exhibit distinctive geometric and electronic structures, rendering them highly promising in addressing issues of solubility and air stability, which are faced for large linear arene…

化学物理 · 物理学 2025-05-27 Hengyu Jin , Xiaoqi Sun , Guiya Qin , Zhipeng Tong , Rui Wang , Qi Zhao , Ai-Min Ren , Jingfu Guo
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