相关论文: Non-Equilibrium Dynamics of the Time-Dependent Exc…
Strong excitonic coupling and photon antibunching (AB) have been observed together in Venus yellow fluorescent protein dimers and currently lack a cohesive theoretical explanation. In 2019, Kim et al. demonstrated Davydov splitting in…
The non-hermitian quantum dynamics of excitonic energy transfer in photosynthetic systems is investigated using a dissipative two-level dimer model. The approach is based on the Green's function formalism which permits consideration of…
Understanding the nature of molecular excitons in low-dimensional molecular solids is of paramount importance in fundamental photophysics and various applications such as energy harvesting, switching electronics and display devices. Despite…
The optical properties of molecular crystals are largely determined by the excitonic coupling of neighboring molecules. This coupling is extremely sensitive to the arrangement of adjacent molecular units, as their electronic interaction is…
Material systems with Dirac electrons on a bipartite planar lattice and possessing superconducting and excitonic interactions are investigated both in the half-filling and doped regimes at zero temperature. Excitonic pairing is the analog…
In this article, we explore the dynamical decoherence of the chromophores within a green fluorescent protein when coupled to a finite-temperature dielectric environment. Such systems are of significant interest due to their anomalously long…
The quantum-dynamical mechanism of photoinduced subpicosecond exciton dissociation and the concomitant formation of a charge-separated state at a TFB:F8BT polymer heterojunction is elucidated. The analysis is based upon a two-state vibronic…
We investigate the description of excitonic effects within time-dependent density-functional theory (TDDFT). The exchange-correlation kernel f_xc introduced in TDDFT allows a clear separation of quasiparticle and excitonic effects. Using a…
Starting from the many-body Bethe-Salpeter equation we derive an exchange-correlation kernel $f_{xc}$ that reproduces excitonic effects in bulk materials within time-dependent density functional theory. The resulting $f_{xc}$ accounts for…
We study excitonic pairing in nodal fermion systems characterized by a vanishing quasiparticle density of states at the pointlike Fermi surface and a concomitant lack of screening for long-range interactions. By solving the gap equation for…
Inter- or intramolecular coupling processes between chromophores such as excimer formation or H- and J-aggregation are crucial to describing the photophysics of closely packed films of conjugated polymers. Such coupling is highly distance…
Deterministic control of excitonic properties is key to advancing nanoscale optoelectronic and quantum technologies and to understanding diverse physical, optical, chemical, and biological phenomena. At the molecular scale, these properties…
We study critical properties of the relaxation time at a threshold point in switching processes between bistable states under change of external fields. In particular, we investigate the relaxation processes near the spinodal point of the…
We present a rigorous theoretical description of excitonic dynamics in molecular light-harvesting aggregates photoexcited by weak-intensity radiation of arbitrary properties. While the interaction with light is included up to the second…
We analyze the many-particle correlations that affect the optical properties of two-dimensional semiconductors. These correlations manifest themselves through the specific optical resonances such as excitons, trions, etc. Starting from the…
An excitonic insulator phase is expected to arise from the spontaneous formation of electron-hole pairs (excitons) in semiconductors where the exciton binding energy exceeds the size of the electronic band gap. At low temperature, these…
Coupled many-body quantum systems give rise to rich emergent physics and abundance of both stationary and dynamical behaviours. Designing platforms with tunable and distinct forms of coupling gives new insight into the collective behaviour…
We analyze possible nonlinear exciton-exciton correlation effects in the optical response of semiconductors by using a time-dependent density-functional theory (TDDFT) approach. For this purpose, we derive the nonlinear (third-order) TDDFT…
We investigate the temporal fluctuations characteristic of the formation of molecular dimers from ultracold fermionic atoms via Raman photoassociation. The quantum fluctuations inherent to the initial atomic state result in large…
Excitonic couplings between (bacterio)chlorophyll molecules are necessary for simulating energy transport in photosynthetic complexes. Many techniques for calculating the couplings are in use, from the simple (but inaccurate) point-dipole…