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相关论文: Real-time exciton dynamics in two-dimensional mate…

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Phosphorene is a two-dimensional (2D) material exhibiting strong in-plane structural anisotropy. In this work, we investigate the influence of structural anisotropy on the optics, dynamics, and transport of excitons in phosphorene by…

介观与纳米尺度物理 · 物理学 2025-09-04 Kai-Wei Chang , Joshua J. P. Thompson , Bartomeu Monserrat

Quantum simulations of photoexcited low-dimensional systems are pivotal for understanding how to functionalize and integrate novel two-dimensional (2D) materials in next-generation optoelectronic devices. First principles predictions are…

介观与纳米尺度物理 · 物理学 2023-05-15 Enrico Perfetto , Gianluca Stefanucci

Microcavity exciton-polaritons are two-dimensional bosonic quasiparticles composed by excitons and photons. Using model Hamiltonian with parameters generated from ab initio density-functional theory and Bathe-Salpeter Equation calculations,…

材料科学 · 物理学 2021-12-01 Huaiyuan Yang , Xinqiang Wang , Xin-Zheng Li

Optical responses of atomically thin 2D materials are greatly influenced by electron-hole interactions. It is by far established that exciton signatures can be well-identified in the optical absorption spectrum of quasi-2D materials.…

介观与纳米尺度物理 · 物理学 2023-10-30 Yu-Tzu Chang , Yang-Hao Chan

Excitons, quasi particles composed of an electron and a hole, play an important role in optical responses in low-dimensional nanostructures. In this work, we have investigated exciton diffusion in a monolayer MoSe2 encapsulated between…

介观与纳米尺度物理 · 物理学 2020-09-30 T. Hotta , S. Higuchi , A. Ueda , K. Shinokita , Y. Miyauchi , K. Matsuda , K. Ueno , T. Taniguchi , K. Watanabe , R. Kitaura

We perform coherent nonlinear spectroscopy of excitons in single-layers of MoSe$_2$ and WSe$_2$ encapsulated between thin films of hexagonal boron nitride. Employing four-wave mixing microscopy we identify virtually disorder free areas,…

Two-dimensional semiconductors have emerged as a new class of materials for nanophotonics for their strong exciton-photon interaction and flexibility for engineering and integration. Taking advantage of these properties, we engineer an…

介观与纳米尺度物理 · 物理学 2020-01-08 Eunice Y. Paik , Long Zhang , G. William Burg , Rahul Gogna , Emanuel Tutuc , Hui Deng

In recent years the physics of two-dimensional semiconductors was revived by the discovery of the class of transition metal dichalcogenides. In these systems excitons dominate the optical response in the visible range and open many…

介观与纳米尺度物理 · 物理学 2021-02-26 Thilo Hahn , Jacek Kasprzak , Paweł Machnikowski , Tilmann Kuhn , Daniel Wigger

We study the binding energies and optical properties of direct and indirect excitons in monolayers and double layer heterostructures of Xenes: silicene, germanene, and stanene. It is demonstrated that an external electric field can be used…

介观与纳米尺度物理 · 物理学 2018-09-19 Matthew N Brunetti , Oleg L. Berman , Roman Ya. Kezerashvili

While polarons --- charges bound to a lattice deformation induced by electron-phonon coupling --- are primary photoexcitations at room temperature in bulk metal-halide hybrid organic-inorganic perovskites (HOIP), excitons --- Coulomb-bound…

材料科学 · 物理学 2020-04-14 Ajay Ram Srimath Kandada , Carlos Silva

Excitons -- bound electron-hole pairs -- play a central role in light-matter interaction phenomena, and are crucial for wide-ranging applications from light harvesting and generation to quantum information processing. A long-standing…

介观与纳米尺度物理 · 物理学 2023-08-15 Jenny Hu , Etienne Lorchat , Xueqi Chen , Kenji Watanabe , Takashi Taniguchi , Tony F. Heinz , Puneet A. Murthy , Thibault Chervy

Tightly bound excitons in monolayer semiconductors represent a versatile platform to study two-dimensional propagation of neutral quasiparticles. Their intrinsic properties, however, can be severely obscured by spatial energy fluctuations…

We demonstrate the feasibility of the time-linear scaling formulation of the $GW$ method [Phys. Rev. Lett. {\bf 124}, 076601 (2020)] for {\it ab initio} simulations of optically driven two-dimensional materials. The time-dependent $GW$…

介观与纳米尺度物理 · 物理学 2022-01-19 E. Perfetto , Y. Pavlyukh , G. Stefanucci

Excitons, Coulomb-bound electron-hole pairs, are the fundamental excitations governing the optoelectronic properties of semiconductors. While optical signatures of excitons have been studied extensively, experimental access to the excitonic…

The attraction between electrons and holes in semiconductors forms excitons, which largely determine the optical properties of the hosting material, and hence the device performance, especially for low-dimensional systems. Mono- and…

介观与纳米尺度物理 · 物理学 2018-03-20 Guowei Zhang , Andrey Chaves , Shenyang Huang , Fanjie Wang , Qiaoxia Xing , Tony Low , Hugen Yan

Atomically thin semi-conductors are characterized by strongly bound excitons which govern the optical properties of the materials below and near the band edge. Efficient conversion of photons into electrical current requires, as a first…

介观与纳米尺度物理 · 物理学 2016-02-15 Sten Haastrup , Simone Latini , Kirill Bolotin , Kristian Sommer Thygesen

Exciton-polariton modes arising from interaction between bound excitons in monolayer thin semiconductor sheets and photons in a Fabry-Perot microcavity are considered theoretically. We calculate the dispersion curves, mode lifetimes, Rabi…

介观与纳米尺度物理 · 物理学 2015-12-30 Mikhail I. Vasilevskiy , Darío G. Santiago-Pérez , Carlos Trallero-Giner , Nuno M. R. Peres , Alexey Kavokin

Excitons are key quasiparticles determining the optical properties of solids. As such, they can be utilized to coherently control the electronic structure of materials using optical femtosecond pulses. Identifying the decoherence mechanism…

Time-dependent density functional theory (TDDFT) has been applied to the calculation of absorption spectra for two-dimensional atomic layer materials. We reveal that the character of the first bright exciton state of bi-layer hexagonal…

材料科学 · 物理学 2020-01-08 Yasumitsu Suzuki , Kazuyuki Watanabe

Atomically thin semiconductors such as transition metal dichalcogenide (TMD) monolayers exhibit a very strong Coulomb interaction, giving rise to a rich exciton landscape. This makes these materials highly attractive for efficient and…