相关论文: Dynamic Lattice Disorder and Collective Dipole Cou…

We study Dicke superradiance as collective and coherent absorption and (time-delayed) emission of photons from an ensemble of ultracold atoms in an optical lattice. Since this process depends on the coherence properties of the atoms (e.g.,…

In recent years there have been significant advances in the study of many-body interactions between atoms and light confined to optical cavities. One model which has received widespread attention of late is the Dicke model, which under…

Resonant dipole-dipole interaction modifies the energy and decay rate of electronic excitations for finite one dimensional chains of ultracold atoms in an optical lattice. We show that collective excited states of the atomic chain can be…

Lead-free halide double perovskites provide a promising solution for the long-standing issues of lead-containing halide perovskites, i.e., the toxicity of Pb and the low stability under ambient conditions and high-intensity illumination.…

All inorganic halide perovskites offer promising optoelectronic properties at low cost, but their structural softness and thermal instability limit applications. Density functional theory using the FP-LAPW method (WIEN2k) was used to study…

A cloud of cold N two-level atoms driven by a resonant laser beam shows cooperative effects both in the scattered radiation field and in the radiation pressure force acting on the cloud center-of-mass. The induced dipoles synchronize and…

Lead-free vacancy-ordered perovskites (VOHPs) such as Cs2SnCl6 have emerged as promising materials for optoelectronic applications but typically suffer from wide band gaps and low photoluminescence quantum yields (PLQY). In this work, the…

2D Ruddlesden-Popper perovskites are compelling platforms for quantum-confined optoelectronics. However, polar order in iodide composition remains rare under ambient conditions, and the mechanistic origin of anomalous photoluminescence in…

We consider quantum droplets in dipolar Bose-Einstein condensates (BECs) embedded in optical lattices within the framework of Gross-Pitaevskii equations. In dipolar BECs, the long-range and anistropic dipole-dipole interaction provides an…

The derivative discontinuity of the exchange-correlation (xc) energy at integer particle number is a property of the exact, unknown xc functional of density functional theory (DFT) which is absent in many popular local and semilocal…

We discuss the emergence and growth of the cooperativity accompanying vitrification based on the density fluctuation dynamics for fragile glass-forming liquids. (i) The relaxation of density fluctuations proceeds by the particle (density)…

In two-dimensional hybrid organic-inorganic metal-halide perovskites, the intrinsic optical lineshape reflects multiple excitons with distinct binding energies, each dressed differently by the hybrid lattice. Given this complexity, a…

The Dicke model describes the collective behavior of a sub-wavelength--size ensemble of two-level atoms (i.e., spin-1/2) interacting identically with a single quantized radiation field of a cavity. Across a critical coupling strength it…

Superfluorescence, the cooperative burst of spontaneous emission from an ensemble of dipoles, arises when microscopic oscillators spontaneously synchronize their phases. Here we show that this process can be reversed in time within quantum…

Hybrid organic-inorganic semiconductors feature complex lattice dynamics due to the ionic character of the crystal and the softness arising from non-covalent bonds between molecular moieties and the inorganic network. Here we establish that…

Metal halide perovskites have emerged as an exciting class of materials for applications in solar energy harvesting, optical devices, catalysis, and other photophysical applications. Many of the exciting properties of halide perovskites are…

Lead halide perovskites have been extensively studied as a class of materials with unique optoelectronic properties. A fundamental aspect that governs optical and electronic behaviors within these materials is the intricate coupling between…

The microscopic origin of slow carrier cooling in lead-halide perovskites remains debated, and has direct implications for applications. Slow carrier cooling has been attributed to either polaron formation or a hot-phonon bottleneck effect…

Recent experiments suggest that atomic disordering dynamics are more universal than conventional coherent processes in photoinduced phase transitions (PIPTs), yet its mechanism remains unclear. Using real-time time-dependent density…

Hybrid halide perovskite semiconductors exhibit complex, dynamical disorder while also harboring properties ideal for optoelectronic applications that include photovoltaics. However, these materials are structurally and compositionally…