相关论文: Efficient high-harmonic generation in van der Waal…
High-efficiency second-harmonic generation (SHG) in compact integrated photonic systems is crucial for advancing nonlinear optical technologies. However, achieving exceptional conversion efficiencies while maintaining stable performance…
Recent experiments in the topological Weyl semimetal TaAs have observed record-breaking second-harmonic generation, a non-linear optical response at $2\omega$ generated by an incoming light source at $\omega$. However, whether…
Although second harmonic generation (SHG) is a promising and widely used method recently for studying 2D magnetic materials, the quantitative analysis of the full SHG tensor is currently challenging. In this letter, we describe a…
The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…
Controlling light at subwavelength scales is one of the main challenges of nanophotonics. Leveraging hyperbolic polaritons supporting arbitrarily large wavevectors can lead to extreme light confinement, effectively overcoming the…
High-order frequency mixing in graphene using a two-color radiation field consisting of the fundamental and the second harmonic fields of an ultrashort linearly polarized laser pulse is studied. It is shown that the harmonics originated…
Infrared laser systems are vital for applications in spectroscopy, communications, and biomedical devices, where infrared nonlinear optical (NLO) crystals are required for broadband frequency down-conversion. Such crystals need to have high…
High-order harmonic generation is investigated for H$_2^+$ and D$_2^+$ with and without Born-Oppenheimer approximation by numerical solution of full dimensional electronic time-dependent Schr\"{o}dinger equation under 4-cycle intense laser…
We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…
Emission of high-order harmonics from solids provides a new avenue in attosecond science. On one hand, it allows to investigate fundamental processes of the non-linear response of electrons driven by a strong laser pulse in a periodic…
We explore with ab-initio theory high harmonic generation (HHG) from a series of gas-phase fullerenes (from C$_{20}$ to C$_{60}$, including isomers) under varying laser conditions (different ellipticities, angular orientations, intensities…
We employ the two-band density-matrix equations and time-dependent density functional theory to calculate high-order harmonic generation (HOHG) in graphene under a femtosecond laser irradiation. Our investigation uncovers a striking…
Low-dimensional ferroelectricity and polar materials have attracted considerable attentions for their fascinating physics and potential applications. Based on first-principles calculations, here we investigate the stacking modes and polar…
The controlled assembly of twisted 2D structures requires precise determination of the crystal orientation of their component layers. In the established procedure, the second-harmonic generation (SHG) intensity of a noncentrosymmetric layer…
While all media can exhibit first-order conductivity describing current linearly proportional to electric field, $E$, the second-order conductivity, $\sigma^{(2)}$ , relating current to $E^2$, is nonzero only when inversion symmetry is…
High harmonic generation (HHG) from crystals in strong laser fields has been understood by the band theory of solid, which is based on the periodic boundary condition (PBC) of translational invariant. For systems having PBC of rotational…
Understanding how low-dimensional ferroelectrics respond to ultrafast excitation at nanoscales is essential for controlling energy flow and mechanical functionality in next-generation polar devices, yet the nanoscopic structural response to…
True phase-matched second-harmonic generation in a waveguide of crosslinkable ferroelectric liquid crystals is demonstrated. These materials allow the formation of macroscopically polar structures whose order can be frozen by…
High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…
High-harmonic generation (HHG) is a strong-field phenomenon that is sensitive to the attosecond dynamics of tunnel ionization and coherent transport of electron-hole pairs in solids. While the foundations of solid HHG have been established,…