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Nd-based pyrochlore oxides of the form Nd$_{2}B_{2}$O$_{7}$ have garnered a significant amount of interest owing to the moment fragmentation physics observed in Nd$_{2}$Zr$_{2}$O$_{7}$ and speculated in Nd$_{2}$Hf$_{2}$O$_{7}$. Notably this…

The pyrochlore compounds Ho2Ti2O7 and Dy2Ti2O7 show an exotic form of magnetism called the spin ice state, resulting from the interplay between geometrical frustration and ferromagnetic coupling. A fascinating feature of this state is the…

材料科学 · 物理学 2013-09-11 D. P. Leusink , F. Coneri , M. Hoek , S. Turner , H. Idrissi , G. Van Tendeloo , H. Hilgenkamp

Motivated by several claims of spin-orbit driven spin-liquid physics in hexagonal Ba$_3$Ti$_{3-x}$Ir$_x$O$_9$ hosting Ir2O9 dimers, we report on resonant inelastic x-ray scattering (RIXS) at the Ir L3 edge for different x. We demonstrate…

We study the ground state and thermodynamic properties of the spin-half XXZ model, with an Ising interaction $J_z$ and a transverse exchange interaction $J_{x}$, on a pyrochlore tube obtained by joining together elementary cubes in a…

强关联电子 · 物理学 2022-08-31 Chunhan Feng , Alexander Wietek , E. Miles Stoudenmire , Rajiv R. P. Singh

The recent discoveries of proximate quantum spin-liquid compounds and their potential application in quantum computing informs the search for new candidate materials for quantum spin-ice and spin-liquid physics. While the majority of such…

强关联电子 · 物理学 2019-01-16 K. M. Taddei , L. Sanjeewa , J. W. Kolis , A. S. Sefat , C. de la Cruz , D. M. Pajerowski

We investigate a phenomenological model for the spin glass phase of La_{2-x}Sr_xCuO_4, in which it is assumed that holes doped into the CuO_2 planes localize near their Sr dopant, where they cause a dipolar frustration of the…

无序系统与神经网络 · 物理学 2009-11-10 N. Hasselmann , A. H. Castro Neto , C. Morais Smith

Ho2Ti2O7 and Dy2Ti2O7 spin ices exhibit elementary excitations akin to magnetic monopoles. Here we focus on Tb2Ti2O7 spin liquid, where correlated magnetic moments keep fluctuating down to very low temperatures. Using a monopole picture, we…

强关联电子 · 物理学 2015-06-05 A. P. Sazonov , A. Gukasov , I. Mirebeau , P. Bonville

We report on the origin of spin freezing in the disordered fluorite Ho$_2$Zr$_2$O$_7$. The system is investigated by low-temperature heat capacity as well as by DC and AC magnetization. While the system does not show a long-range magnetic…

强关联电子 · 物理学 2024-07-19 A. Elghandour , Sheeta , C. S. Yadav , R. Klingeler

We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an "all-in-all-out" magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation…

材料科学 · 物理学 2016-09-07 J. Xu , C. Balz , C. Baines , H. Luetkens , B. Lake

Materials with coupled or competing order parameters display highly tunable ground states, where subtle perturbations reveal distinct electronic and magnetic phases. These phases generally are underpinned by complex crystal structures, but…

强关联电子 · 物理学 2019-11-25 Elizabeth A. Nowadnick , Jiangang He , Craig J. Fennie

We report high-frequency/high-field electron spin resonance (ESR) and high-field magnetization studies on single crystals of the bond-disordered pyrochlore NaCaCo$_2$F$_7$. Frequency- and temperature-dependent ESR investigations above the…

The spin ice materials Ho$_{2}$Ti$_{2}$O$_{7}$ and Dy$_{2}$Ti$_{2}$O$_{7}$ are by now perhaps the best-studied classical frustrated magnets. A crucial step towards the understanding of their low temperature behaviour -- both regarding their…

强关联电子 · 物理学 2019-08-14 Bruno Tomasello , Claudio Castelnovo , Roderich Moessner , Jorge Quintanilla

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

强关联电子 · 物理学 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

Frustrated magnets provide a platform for exploring exotic phases beyond conventional ordering, with potential relevance to functional materials and information technologies. In this work, we use Monte Carlo simulations to map the…

强关联电子 · 物理学 2025-12-16 Prakash Timsina , Andres Chappa , Deema Alyones , Igor Vasiliev , Ludi Miao

Recent experiments on Mn doped multiferroic $CoCr_{2}O_{4}$ indicate that a possible distribution of Mn atoms among tetrahedrally and octahedrally coordinated sites in the spinel lattice give rise to different variations in the structural…

材料科学 · 物理学 2017-01-04 Debashish Das , Subhradip Ghosh

Transport and magnetic properties along with high resolution valence band photoemission study of disordered double perovskite Sr$_{2}$TiIrO$_{6}$ has been investigated. Insulator to insulator transition along with a magnetic transition…

强关联电子 · 物理学 2023-01-18 B. H. Reddy , Asif Ali , Ravi Shankar Singh

$\gamma$-triclinic and $\alpha$-monoclinic polymorphs of CoV$_{2}$O$_{6}$ are two of the few known transition metal ion based materials that display stepped $1/3$ magnetization plateaus at low temperatures. Neutron diffraction [M. Markkula…

Pyrochlore iridates A2Ir2O7 (A = rare earth elements, Y or Bi) hold great promise for realizing novel electronic and magnetic states owing to the interplay of spin-orbit coupling, electron correlation and geometrical frustration. A…

强关联电子 · 物理学 2017-10-04 W. C. Yang , W. K. Zhu , H. D. Zhou , L. Ling , E. S. Choi , M. Lee , Y. Losovyj , Chi-Ken Lu , S. X. Zhang

Pyrochlore $\rm Pr^{3+}_{2+x}Zr^{4+}_{2-x}O_{7-x/2}$ samples in the form of both powders $(-0.02 \le x \le 0.02)$ and bulk single crystals have been studied to elucidate the dependence of their magnetic, compositional and structural…

材料科学 · 物理学 2014-07-08 S. M. Koohpayeh , J. -J. Wen , B. A. Trump , C. L. Broholm , T. M. McQueen

We report the anisotropic magnetic properties of Ho2Ge2O7 determined from dc and ac magnetization, specific heat and powder neutron diffraction experiments. The magnetic lanthanide sublattice, seen in our refinement of the tetragonal…

其他凝聚态物理 · 物理学 2009-11-13 E. Morosan , J. A. Fleitman , Q. Huang , J. W. Lynn , Y. Chen , X. Ke , M. L. Dahlberg , P. Schiffer , C. R. Craley , R. J. Cava