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Weak bond disorder disrupts the expected spin-liquid ground-state of the ideal $S$ = 1/2 Heisenberg pyrochlore antiferromagnet. Here we introduce a single crystal study of the structural and magnetic properties of the bond-disordered…

强关联电子 · 物理学 2023-07-12 Andrej Kancko , Gerald Giester , Ross H. Colman

Being motivated by recent experimental studies, we investigate magnetic structures of the Mo pyrochlores $A_2$Mo$_2$O$_7$ ($A$= Y, Nd, and Gd) and their impact on the electronic properties. The latter are closely related with the behavior…

强关联电子 · 物理学 2009-11-07 I. V. Solovyev

We have studied the hidden long-range order (LRO) of the frustrated pyrochlore magnet Tb$_2$Ti$_2$O$_7$ by means of specific-heat experiments and Monte-Carlo (MC) simulations, which has been discussed as the LRO of quadrupole moments…

强关联电子 · 物理学 2016-02-09 H. Takatsu , T. Taniguchi , S. Kittaka , T. Sakakibara , H. Kadowaki

Neutron diffraction studies have been carried out in the applied magnetic field H(//[011]) on a single crystal of pyrochlore ferromagnet Nd2Mo2O7, whose Hall resistivity(r_H) has been reported to have quite unusual magnetic field (H)- and…

We report the crystal structures, magnetic and thermodynamic properties of two magnetically frustrated $A$'$A$"$M_2$F$_7$-type antiferromagnets, NaCdNi$_2$F$_7$ and NaCdMn$_2$F$_7$. While NaCdNi$_2$F$_7$ forms a stable pyrochlore structure…

强关联电子 · 物理学 2025-04-10 Andrej Kancko , Cinthia Antunes Corrêa , Ross Harvey Colman

In this work, we report on the thermomagnetic characterization and crystalline-electric field (CEF) energy scheme of the disordered defect-fluorite Ho2Zr2O7. This structural phase is distinguished by the coexistence of magnetic frustration…

The lanthanide pyrochlore oxides Ln$_2$B$_2$O$_7$ are one of the most intensely studied classes of materials within condensed matter physics, firmly centered as one of the pillars of frustrated magnetism. The extensive chemical diversity of…

The pyrochlore magnet $\rm Yb_2Ti_2O_7$ has been proposed as a quantum spin ice candidate, a spin liquid state expected to display emergent quantum electrodynamics with gauge photons among its elementary excitations. However, $\rm…

强关联电子 · 物理学 2018-06-20 Gabriele Sala , Dalini D. Maharaj , Matthew B. Stone , Hanna A. Dabkowska , Bruce D. Gaulin

Dipolar-octupolar (DO) pyrochlore systems Ce$_2$(Zr,Sn,Hf)$_2$O$_7$ have garnered much attention as recent investigations suggest that they may stabilize a novel quantum spin ice (QSI), a quantum spin liquid (QSL) with an emergent $U(1)$…

强关联电子 · 物理学 2025-12-10 Zhengbang Zhou , Félix Desrochers , Yong Baek Kim

Pressure-induced ordering close to a $z=1$ quantum critical point is studied in the presence of bond disorder in the quantum spin system (C$_4$H$_{12}$N$_2$)Cu$_2$(Cl$_{1-x}$Br$_{x}$)$_6$ (PHCX) by means of muon-spin rotation and…

The pyrochlore lattice involves corner sharing tetrahedra and the resulting geometric frustration is believed to suppress any antiferromagnetic order for Mott insulators on this structure. There are nevertheless short-range correlations…

强关联电子 · 物理学 2016-10-19 Nyayabanta Swain , Rajarshi Tiwari , Pinaki Majumdar

We investigated the electronic and magnetic properties of the pyrochlore oxide Cd$_2$Os$_2$O$_7$ using the density-functional theory plus on-site repulsion ($U$) method, and depict the ground-state phase diagram with respect to $U$. We…

强关联电子 · 物理学 2012-06-15 Hiroshi Shinaoka , Takashi Miyake , Shoji Ishibashi

We report that the local Ising anisotropy in pyrochlore oxides - the crucial requirement for realizing the spin-ice state - can be broken by means of high magnetic fields. For the case of the well-established classical spin-ice compound…

We report the low temperature magnetic properties of Nd$^{3+}$ pyrochlore $\rm Nd_2ScNbO_7$. Susceptibility and magnetization show an easy-axis moment, and heat capacity reveals a phase transition to long range order at $T_N=371(2)$ mK with…

强关联电子 · 物理学 2022-08-11 A. Scheie , M. Sanders , Yiming Qiu , T. R. Prisk , R. J. Cava , C. Broholm

We report on the study of unusual spin glass properties in the geometrically frustrated pyrochlore Tb$_{2}$Mo$_{2}$O$_{7}$, $T$$_{g}$$\simeq$24 K. The analysis of the nonlinear part of dc and complex susceptibilities, near the glass…

强关联电子 · 物理学 2013-09-17 D. K. Singh , Y. S. Lee

The crystal structures of the A2B2O7-x Niobium-based pyrochlores Y2(Nb0.86Y0.14)2O6.91, CaYNb2O7, and Y2NbTiO7 are reported, determined by powder neutron diffraction. These compounds represent the first observation of B-site displacements…

强关联电子 · 物理学 2009-02-02 T. M. McQueen , B. Muegge , Q. Huang , K. Noble , H. W. Zandbergen , R. J. Cava

In this work, polycrystalline NiCrGa half Heusler alloy, which is predicted to be half-metallic ferromagnet from first principles calculations, has been synthesized by arc meting technique and its structural, magnetic as well as the…

材料科学 · 物理学 2018-12-26 Madhusmita Baral , M. K. Chattopadhyay , Aparna Chakrabarti , Tapas Ganguli

We report an analysis of neutron diffraction from single crystals of the spin-liquid pyrochlore Tb2Ti2O7 under the application of magnetic fields along the crystallographic $[110]$ direction. Such a perturbation has been shown to destroy…

强关联电子 · 物理学 2009-11-17 J. P. C. Ruff , B. D. Gaulin , K. C. Rule , J. S. Gardner

In spin ice research, small variations in structure or interactions drive a multitude of different behaviors, yet the collection of known materials relies heavily on the `227' pyrochlore structure. Here, we present thermodynamic, structural…

无序系统与神经网络 · 物理学 2019-04-30 D. Reig-i-Plessis , S. V. Geldern , A. A. Aczel , D. Kochkov , B. K. Clark , G. J. MacDougall

The complex structure and magnetism of Pr$_{2-x}$Bi$_x$Ru$_2$O$_7$ was investigated by neutron scattering and EXAFS. Pr has an approximate doublet ground-state and the first excited state is a singlet. This overall crystal field level…