相关论文: Influence of controlled disorder on the dipolar sp…
Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…
Cu$_2$IrO$_3$ is a honeycomb iridate which has been studied recently as a candidate Kitaev quantum spin liquid. Its magnetic ground state however, has been reported to be quantum disordered, spin glassy, or magnetically ordered depending on…
Despite a well-ordered pyrochlore crystal structure and strong magnetic interactions between the Dy$^{3+}$ or Ho$^{3+}$ ions, no long range magnetic order has been detected in the pyrochlore titanates Ho$_2$Ti$_2$O$_7$ and…
Recent experimental results have emphasized two aspects of Tb2Ti2O7 which have not been taken into account in previous attempts to construct theories of Tb2Ti2O7: the role of small levels of structural disorder, which appears to control the…
A study of the modifications of the magnetic properties of Ho$_{2-x}$Y$_x$Sn$_2$O$_7$ upon varying the concentration of diamagnetic Y$^{3+}$ ions is presented. Magnetization and specific heat measurements show that the Spin Ice ground-state…
The third law of thermodynamics dictates that the entropy of a system in thermal equilibrium goes to zero as its temperature approaches absolute zero. In ice, however, a "zero point" or residual entropy can be measured - attributable to a…
The pyrochlore Ho2Ge2O7 is a new highly correlated spin ice material. Physical property measurements including x-ray diffraction, dc susceptibility and ac susceptibility, confirm that it shares the distinctive characteristics of other known…
There are reasons to believe that the ground state of the magnetic rare earth pyrochlore Yb$_2$Ti$_2$O$_7$ is on the boundary between competing ground states. We have carried out $\mathrm{\textit{ab initio}}$ density functional calculations…
We report the magnetic and thermal properties of Dy2Sn2-xSbxO7+x/2, x = 0, 0.25, and 0.5, and Dy2NbScO7. We find evidence for Ising-like single ion ground states in the Dy2Sn2-xSbxO7+x/2 materials. These materials possess nearly the same…
The formation of a spin glass usually requires both structural disorder and frustrated magnetic interactions. Consequently, the origin of spin-glass behaviour in Y$_2$Mo$_2$O$_7$ $-$ in which magnetic Mo$^{4+}$ ions occupy a frustrated…
The layered perovskites $R$Cr(BO$_3$)$_2$ ($R$ = Y and Ho) with magnetic triangular lattices were studied by performing ac/dc susceptibility, specific heat, elastic and inelastic neutron scattering, and dielectric constant measurements. The…
Magnetic-rare-earth pyrochlore iridates exhibit a rich variety of unconventional phases, driven by the complex interactions within and between the rare-earth and the iridium sublattices. In this study, we investigate the peculiar magnetic…
At zero temperature, the classical antiferromagnetic Ising model on the pyrochlore lattice is a spin disorder phase of the critical spin correlation. It is a deconfined phase in that the binding energy of the monopole-anti-monopole pair is…
The singlet ground state magnetism in pyrochlore osmates Y$_2$Os$_2$O$_7$ and Ho$_2$Os$_2$O$_7$ is studied by DC and AC susceptibility, specific heat, and neutron powder diffraction measurements. Despite the expected non-magnetic singlet in…
We describe why Ising spin chains with competing interactions in $\rm SrHo_2O_4$ segregate into ordered and disordered ensembles at low temperatures ($T$). Using elastic neutron scattering, magnetization, and specific heat measurements, the…
We report a random singlet ground state in the $S=\frac{1}{2}$ Heisenberg pyrochlore antiferromagnet NaCdCu$_2$F$_7$. Cationic Na$^+$/Cd$^{2+}$ disorder on the pyrochlore $A$ site generates a broad distribution of…
In this Comment we argue that Ho$_2$Ti$_2$O$_7$ does not exhibit a transition to a partially ordered state unlike what is argued in PRL 83, 1854 (1999), that it exhibits spin ice behavior, and that the experimental specific heat data by…
The delicate balance between spin-orbit coupling, Coulomb repulsion and crystalline electric field interactions observed in Ir-based oxides is usually manifested as exotic magnetic behavior. Here we investigate the evolution of the exchange…
The pyrochlore material $\rm Ho_{2}Ti_{2}O_{7}$ has been suggested to show ``spin ice'' behaviour. We present neutron scattering and specific heat results that establish unambiguously that Ho$_2$Ti$_2$O$_7$ exhibits spin ice correlations at…
Gd2GaSbO7 and Gd2InSbO7 pyrochlore compounds exhibit quantum fluctuations in a spin ice-like state. These compounds have not been adequately studied based on the concept of magnetic frustration. Here, we have synthesised and characterised…