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Conclusive evidence of order by disorder is scarce in real materials. Perhaps one of the strongest cases presented has been for the pyrochlore XY antiferromagnet Er2Ti2O7, with the ground state selection proceeding by order by disorder…

强关联电子 · 物理学 2016-05-11 Jeffrey G. Rau , Sylvain Petit , Michel J. P. Gingras

Geometric frustration usually arises in systems that comprise magnetic moments (spins) which reside on the sites of a lattice made up of elementary triangular or tetrahedral units and which interact via antiferromagnetic nearest-neighbor…

统计力学 · 物理学 2009-03-17 Michel J. P. Gingras

Neutron scattering, a.c. magnetic susceptibility and specific heat studies have been carried out on polycrystalline Dy2Zr2O7. Unlike the pyrochlore spin ice Dy2Ti2O7, Dy2Zr2O7 crystallizes into the fluorite structure and the magnetic Dy3+…

无序系统与神经网络 · 物理学 2019-07-01 J. G. A. Ramon , C. W. Wang , L. Ishida , P. L. Bernardo , M. M. Leite , F. M. Vichi , J. S. Gardner , R. S. Freitas

We present here magnetization, specific heat and Raman studies on single-crystalline specimens of the first pyrochlore member $Sm_2Ti_2O_7$ of the rare-earth titanate series. Its analogous compound $Sm_2Zr_2O_7$ in the rare-earth zirconate…

材料科学 · 物理学 2009-11-13 Surjeet Singh , Surajit Saha , S. K. Dhar , R. Suryanarayanan , A. K. Sood , A. Revcolevschi

Among the frustrated magnetic materials, spin-ice stands out as a particularly interesting system. Residual entropy, freezing and glassiness, Kasteleyn transitions and fractionalisation of excitations in three dimensions all stem from a…

The field-induced dynamics of artificial spin ice are determined in part by interactions between magnetic islands, and the switching characteristics of each island. Disorder in either of these affects the response to applied fields.…

介观与纳米尺度物理 · 物理学 2012-02-15 Zoe Budrikis , Paolo Politi , R. L. Stamps

The disordered pyrochlore oxide Dy$_{2}$Zr$_{2}$O$_{7}$ shows the signatures of field-induced spin freezing with remnant zero-point spin-ice entropy at 5 kOe magnetic field. We have performed zero-field and longitudinal field Muon spin…

强关联电子 · 物理学 2023-03-28 Sheetal , Pabitra K. Biswas , K. Yokoyama , D. T. Adroja , C. S. Yadav

We report a combined muon spin relaxation/rotation, bulk magnetization, neutron scattering, and transport study of the electronic properties of the pyrochlore iridate Nd2Ir2O7. We observe the onset of strongly hysteretic behavior in the…

The standard approach to realize a spin liquid state is through magnetically frustrated states, relying on ingredients such as the lattice geometry, dimensionality, and magnetic interaction type of the spins. While Heisenberg spins on a…

强关联电子 · 物理学 2025-04-10 Margarita G. Dronova , Vaclav Petricek , Zachary Morgan , Feng Ye , Daniel M. Silevitch , Yejun Feng

While the spin liquid state in the frustrated pyrochlore Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ has been studied both experimentally and theoretically for more than two decades, no definite description of this unconventional state has been achieved.…

Effect of structural disorder is investigated for an $XY$ pyrochlore antiferromagnet with continuous degeneracy of classical ground states. Two types of disorder, vacancies and weakly fluctuating exchange bonds, lift degeneracy selecting…

强关联电子 · 物理学 2014-09-26 V. S. Maryasin , M. E. Zhitomirsky

Examples of materials where an "order by disorder" mechanism is at play to select a particular ground state are scarce. It has recently been proposed, however, that the antiferromagnetic XY pyrochlore Er2Ti2O7, reveals a most convincing…

强关联电子 · 物理学 2015-06-23 S. Petit , J. Robert , S. Guitteny , P. Bonville , C. Decorse , J. Ollivier , H. Mutka , M. J. P. Gingras , I. Mirebeau

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

强关联电子 · 物理学 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

We present a comprehensive experimental and theoretical study of the pyrochlore Tb$_2$Ge$_2$O$_7$, an exemplary realization of a material whose properties are dominated by competition between magnetic dipolar and electric quadrupolar…

The dipolar-octupolar (DO) pyrochlores, R$_2$M$_2$O$_7$ (R = Ce, Sm, Nd), are key players in the search for realizable novel quantum spin liquid (QSL) states as a large parameter space within the DO pyrochlore phase diagram is theorized to…

Disorder in materials may be used to tune their functionalities, but much more strikingly, its presence can entail entirely new behavior. This happens in charge-ice where structural disorder is not weak and local, but strong and long-range…

统计力学 · 物理学 2023-11-10 A. Hemmatzade , K. Essafi , M. Taillefumier , M. Müller , T. Fennell , P. M. Derlet

Magnetization and susceptibility studies on single crystals of the pyrochlore Ho$_{2}$Ti$_{2}$O$_{7}$ are reported for the first time. Magnetization isotherms are shown to be qualitatively similar to that predicted by the nearest neighbor…

无序系统与神经网络 · 物理学 2009-11-07 A. L. Cornelius , J. S. Gardner

We investigate partially disordered antiferromagnetism in CoCl$_2$-2SC(NH$_2$)$_2$, in which a-b plane hexagonal layers are staggered along the c-axis, rather than stacked. A robust 1/3 state forms in applied magnetic fields which the spins…

We study the pyrochlore Heisenberg antiferromagnet with additional positive biquadratic interaction in the semiclassical limit. The classical ground state manifold of the model contains an extensively large family of non-coplanar spin…

强关联电子 · 物理学 2016-11-15 Yuan Wan , Michel J. P. Gingras

We investigate the structural, magnetic, and thermodynamic properties of \BSCO\ ($x$ = 0.04, $\delta$ = 0.54), a hexagonal perovskite featuring face-sharing CoO$_6$ octahedra that forms Co dimers. DC and AC magnetization measurements reveal…

强关联电子 · 物理学 2025-08-15 Anzar Ali , Guratinder Kaur , Lukas Keller , Masahiko Isobe