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We propose a framework for designing coherent optical environments that enable versatile and dynamic optical manipulation. In contrast to conventional material-based near-field platforms, our approach employs a structured coherent light…

光学 · 物理学 2025-10-07 Xiaoshu Zhao , Xu Yuan , Hongxia Zheng , Huajin Chen , Zhifang Lin

We report the first experimental observation of non-adiabatic field-free orientation of a heteronuclear diatomic molecule (CO) induced by an intense two-color (800 and 400 nm) femtosecond laser field. We monitor orientation by measuring…

This paper explains some fundamental ideas of {\em feedback} control of quantum systems through the study of a relatively simple two-level system coupled to optical field channels. The model for this system includes both continuous and…

量子物理 · 物理学 2014-06-23 Matthew James

We demonstrate coherent optical control of a single hole spin confined to an InAs/GaAs quantum dot. A superposition of hole spin states is created by fast (10-100 ps) dissociation of a spin-polarized electron-hole pair. Full control of the…

介观与纳米尺度物理 · 物理学 2012-01-09 T. M. Godden , J. H. Quilter , A. J. Ramsay , Yanwen Wu , P. Brereton , S. J. Boyle , I. J. Luxmoore , J. Puebla-Nunez , A. M. Fox , M. S. Skolnick

We apply the quantum optimal control theory based on the Krotov method to implement single-qubit $X$ and $Z$ gates and two-qubit CNOT gates for inductively coupled superconducting flux qubits with fixed qubit transition frequencies and…

量子物理 · 物理学 2014-07-16 Shang-Yu Huang , Hsi-Sheng Goan

Control of multi-level quantum systems is sensitive to implementation errors in the control field and uncertainties associated with system Hamiltonian parameters. A small variation in the control field spectrum or the system Hamiltonian can…

量子物理 · 物理学 2015-06-23 Andy Koswara , Raj Chakrabarti

A quantum fluid dynamic control formulation is presented for optimally manipulating atomic and molecular systems. In quantum fluid dynamic the control quantum system is expressed in terms of the probability density and the quantum current.…

化学物理 · 物理学 2009-11-06 Bijoy K. Dey , Herschel Rabitz , Attila Askar

We consider the coherent control of ultracold molecule-molecule scattering, impacted by a dense set of rovibrational resonances. To characterize the resonance spectrum, a rudimentary model based on multichannel quantum defect theory has…

原子物理 · 物理学 2023-01-18 Adrien Devolder , Timur V. Tscherbul , Paul Brumer

We demonstrate coherent microwave control of rotational and hyperfine states of trapped, ultracold, and chemically stable $^{23}$Na$^{40}$K molecules. Starting with all molecules in the absolute rovibrational and hyperfine ground state, we…

量子气体 · 物理学 2016-06-08 Sebastian A. Will , Jee Woo Park , Zoe Z. Yan , Huanqian Loh , Martin W. Zwierlein

We exploit a novel approximation scheme to obtain a new and compact formula for the parameters underlying coherent-state control of the evolution of a pair of entangled two-level systems. It is appropriate for long times and for relatively…

量子物理 · 物理学 2010-08-24 Muhammed Yonac , Joseph H. Eberly

Conventional information processors freely convert information between different physical carriers to process, store, or transmit information. It seems plausible that quantum information will also be held by different physical carriers in…

量子物理 · 物理学 2020-05-21 Yiheng Lin , David R. Leibrandt , Dietrich Leibfried , Chin-wen Chou

We demonstrate coherent control of both the rotational and hyperfine state of ultracold, chemically stable $^{87}$Rb$^{133}$Cs molecules with external microwave fields. We create a sample of ~2000 molecules in the lowest hyperfine level of…

量子气体 · 物理学 2016-11-02 Philip D. Gregory , Jesus Aldegunde , Jeremy M. Hutson , Simon L. Cornish

Oriented external electric fields are ubiquitous in chemistry; however, the effects of fields applied in different directions on molecular systems remain underexplored. A major challenge is that an applied field exerts a torque on a…

化学物理 · 物理学 2026-05-12 Duc Anh Lai , Devin A. Matthews

Two mechanisms of two-color (\omega + 2\omega) laser-induced field-free molecular orientation, based on the hyperpolarizability and ionization depletion, are explored and compared. The CO molecule is used as a computational example. While…

原子物理 · 物理学 2012-09-14 Michael Spanner , Serguei Patchkovskii , Eugene Frumker , Paul Corkum

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

量子物理 · 物理学 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

Experiments in coherent spectroscopy correspond to control of quantum mechanical ensembles guiding them from initial to final target states by unitary transformations. The control inputs (pulse sequences) that accomplish these unitary…

量子物理 · 物理学 2007-05-23 Navin Khaneja , Steffen Glaser

We consider the problem of time-optimal control of quadrupole nucleus with the spin I=1 by NMR. In contrast to the conventional methods based on selective pulses, the control is implemented using nonselective pulses separated by free…

量子物理 · 物理学 2015-06-05 V. P. Shauro

Control of quantum systems typically relies on the interaction with electromagnetic radiation. In this study, we experimentally show that the electromagnetic near-field of a spatially modulated freespace electron beam can be used to drive…

We present new results on the quantum control of systems with infinitely large Hilbert spaces. A control-theoretic analysis of the control of trapped ion quantum states via optical pulses is performed. We demonstrate how resonant…

量子物理 · 物理学 2007-05-23 C. Rangan , A. M. Bloch , C. Monroe , P. H. Bucksbaum

In many quantum information processing applications, it is important to be able to transfer a quantum state from one location to another - even within a local device. Typical approaches to implement the quantum state transfer rely on…

量子物理 · 物理学 2018-10-09 Yuichiro Matsuzaki , Victor M. Bastidas , Yuki Takeuchi , William J. Munro , Shiro Saito
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