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The core issue for the implementation of the diamond NV centre qubits technology is the sensitive readout of NV spin state. We have recently demonstrated the photoelectric detection of NV magnetic resonances (PDMR), anticipated to be faster…

介观与纳米尺度物理 · 物理学 2017-01-25 E. Bourgeois , E. Londero , K. Buczak , Y. Balasubramaniam , G. Wachter , J. Stursa , K. Dobes , F. Aumayr , M. Trupke , A. Gali , M. Nesladek

Although 19F has high potential to serve as a background-free molecular marker in bioimaging, the molar amount of marker substance is often too small to enable 19F MR imaging or 19F NMR spectroscopy with a sufficiently high signal-to-noise…

化学物理 · 物理学 2022-05-24 Johannes Bernarding , Christian Bruns , Isabell Prediger , Markus Plaumann

Due to their large coherent scattering cross section, diamond nanoparticles (DNPs) are considered as a promising candidate material for a new neutron reflector. For investigation of scattering cross sections of packed samples, we have…

仪器与探测器 · 物理学 2020-07-17 Kenji Mishima , Toshiya Otomoa , Kazutaka Ikeda , Hidetoshi Ohshita

Scanning-probe and wide-field magnetic microscopes based on Nitrogen-Vacancy (NV) centers in diamond have enabled remarkable advances in the study of biology and materials, but each method has drawbacks. Here, we implement an alternative…

Quantum sensors have attracted broad interest in the quest towards sub-micronscale NMR spectroscopy. Such sensors predominantly operate at low magnetic fields. Instead, however, for high resolution spectroscopy, the high-field regime is…

We report a versatile method to efficiently polarize single nuclear spins in diamond, which is based on optical pumping of a single NV color center and mediated by a level-anti crossing in its excited state. A nuclear spin polarization…

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

The ability to optically initialize the electronic spin of the nitrogen-vacancy (NV) center in diamond has long been considered a valuable resource to enhance the polarization of neighboring nuclei, but efficient polarization transfer to…

介观与纳米尺度物理 · 物理学 2018-08-01 F. Shagieva , S. Zaiser , P. Neumann , D. B. R. Dasari , R. Stöhr , A. Denisenko , R. Reuter , C. A. Meriles , J. Wrachtrup

Nanomagnetometry using the nitrogen-vacancy (NV) centre in diamond has attracted a great deal of interest because of the combined features of room temperature operation, nanoscale resolution and high sensitivity. One of the important goals…

We introduce an alternate route to dynamically polarize the nuclear spin host of nitrogen-vacancy (NV) centers in diamond. Our approach articulates optical, microwave and radio-frequency pulses to recursively transfer spin polarization from…

量子物理 · 物理学 2014-12-18 Daniela Pagliero , Abdelghani Laraoui , Jacob D. Henshaw , Carlos A. Meriles

Dynamic Nuclear Polarization (DNP) is transforming NMR and MRI by significantly enhancing sensitivity through the transfer of polarization from electron spins to nuclear spins via microwave irradiation. However, the use of monochromatic…

量子物理 · 物理学 2024-10-28 Mayur Jhamnani , Sajith V Sadasivan , Sheetal Kumar Jain , Asif Equbal

Diamond-based quantum sensors have enabled high-resolution NMR spectroscopy at the microscale in scenarios where fast molecular motion averages out dipolar interactions among target nuclei. However, in samples with low-diffusion, ubiquitous…

量子物理 · 物理学 2025-08-26 Carlos Munuera-Javaloy , Ander Tobalina , Jorge Casanova

The boron-doped single crystal diamond films were grown homoepitaxially on synthetic (100) oriented Type Ib diamond substrates using a Microwave Plasma Chemical Vapor Deposition (MPCVD) technique. Raman spectrum showed a few additional…

材料科学 · 物理学 2013-02-01 Sunil K. Karna , Yogesh. K. Vohra , Samuel T. Weir

Si nanoparticles (NPs) have been actively developed as a hyperpolarized magnetic resonance imaging (MRI) contrast agent with an imaging window close to one hour. However, the progress in the development of NPs has been hampered by the…

Dynamic nuclear polarization (DNP) is an attractive method for initializing nuclear spins that are strongly coupled to optically active electron spins because it functions at room temperature and does not require strong magnetic fields. In…

Optomechanical devices sensitively transduce and actuate motion of nanomechanical structures using light. Single--crystal diamond promises to improve the performance of optomechanical devices, while also providing opportunities to interface…

Nitrogen Vacancy diamond nanoparticles (NVNPs) are increasingly integrated with methods for optical detection of magnetic resonance (ODMR), providing new opportunities in magnetic characterization that span the visualization of magnetic…

We present theoretical proposals for two-dimensional nuclear magnetic resonance spectroscopy protocols based on Nitrogen-vacancy (NV) centers in diamond that are strongly coupled to the target nuclei. Continuous microwave and…

量子物理 · 物理学 2024-10-31 Matthias Kost , Jianming Cai , Martin B. Plenio

Color centers in diamond nanocrystals are a new class of fluorescence markers that attract significant interest due to matchless brightness, photostability and biochemical inertness. Fluorescing diamond nanocrystals containing defects can…

生物大分子 · 定量生物学 2009-11-13 M. Boersch , R. Reuter , G. Balasubramanian , R. Erdmann , F. Jelezko , J. Wrachtrup

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…