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We report on the systematic characterization of the optical properties of diamond color centers based on Pb impurities. An ensemble photoluminescence analysis of their spectral emission was performed at different excitation wavelengths in…

Research on diamond has intensified due to its exceptional thermal, optical, and mechanical properties, making it a key material in quantum technologies and high-power applications. Diamonds with engineered nitrogen-vacancy (NV) centers…

Solid state defects such as nitrogen vacancy (NV) centers in diamond have been utilized for NMR sensing at ambient temperatures for samples at the nano-scale and up to the micro-scale. Similar to standard NMR, NV-sensitivities can be…

量子物理 · 物理学 2026-01-28 Oliver T. Whaites , Jaime García Oliván , Jorge Casanova

The development of materials processing techniques for optical diamond nanostructures containing a single color center is an important problem in quantum science and technology. In this work, we present the combination of ion implantation…

We reveal an interplay between temperature and radical concentration necessary to establish thermal mixing (TM) as an efficient dynamic nuclear polarization (DNP) mechanism. We conducted DNP experiments by hyperpolarizing widely used DNP…

量子物理 · 物理学 2024-04-12 Ludovica M. Epasto , Thibaud Maimbourg , Alberto Rosso , Dennis Kurzbach

Two-dimensional ferromagnetic nanodot structures exhibit intriguing magnetization dynamics and hold promise for future magnonic devices. In this study, we present a comparative experimental investigation into the reconfigurable…

介观与纳米尺度物理 · 物理学 2024-07-15 Swapnil Barman , Rajib Kumar Mitra

Arrays of NV centers in the diamond have the potential in the fields of chip-scale quantum information processing and nanoscale quantum sensing. However, determining their orientations one by one is resource intensive and time consuming.…

应用物理 · 物理学 2019-12-18 Xuerui Song , Fupan Feng , Chunxiao Cai , Guanzhong Wang , Wei Zhu , Wenting Diao , Chongdi Duan

One of the most remarkable properties of the nitrogen-vacancy (NV) center in diamond is that optical illumination initializes its electronic spin almost completely, a feature that can be exploited to polarize other spin species in their…

Nanodiamonds containing nitrogen vacancy (NV-) centers show promise for a number of emerging applications including targeted in vivo imaging and generating nuclear spin hyperpolarization for enhanced NMR spectroscopy and imaging. Here, we…

Polarization transfers are crucial building blocks in magnetic resonance experiments, i.e., they can be used to polarize insensitive nuclei and correlate nuclear spins in multidimensional NMR spectroscopy. The polarization can be…

化学物理 · 物理学 2022-08-24 Zhenfeng Pang , Sheetal Jain , Chen Yang , Xueqian Kong , Kong Ooi Tan

We report on a planar microwave resonator providing arbitrarily polarized oscillating magnetic fields that enable selective excitation of the electronic spins of nitrogen-vacancy (NV) centers in diamond. The polarization plane is parallel…

介观与纳米尺度物理 · 物理学 2016-11-07 Johannes Herrmann , Marc A. Appleton , Kento Sasaki , Yasuaki Monnai , Tokuyuki Teraji , Kohei M. Itoh , Eisuke Abe

Nuclear spin hyperpolarization techniques, such as dynamic nuclear polarization (DNP) and parahydrogen-induced polarization (PHIP), have revolutionized nuclear magnetic resonance and magnetic resonance imaging. In these methods, a readily…

In pulsed dynamic nuclear polarization (DNP), enhancement of the polarization of bulk nuclei requires the repeated application of a microwave pulse sequence. So far, analysis of a one-time transfer of electron spin polarization to a…

Nitrogen vacancy (NV) centers in diamond have been used as ultrasensitive magnetometers to perform nuclear magnetic resonance (NMR) spectroscopy of statistically polarized samples at 1 - 100 nm length scales. However, the spectral linewidth…

We study a mechanism by which nuclear hyperpolarization due to the polarization transfer from a microwave-pulse-controlled electron spin is suppressed. From analytical and numerical calculations of the unitary dynamics of multiple nuclear…

量子物理 · 物理学 2024-03-12 Kento Sasaki , Eisuke Abe

In the present work we report about the investigation of the conduction mechanism of sp2 carbon micro-channels buried in single crystal diamond. The structures are fabricated with a novel technique which employs a MeV focused ion-beam to…

材料科学 · 物理学 2016-08-29 P. Olivero , G. Amato , F. Bellotti , S. Borini , A. Lo Giudice , F. Picollo , E. Vittone

Highly sensitive nuclear spin detection is crucial in many scientific areas including nuclear magnetic resonance spectroscopy (NMR), imaging (MRI) and quantum computing. The tiny thermal nuclear spin polarization represents a major obstacle…

The nitrogen vacancy (NV) color center in diamond is an enormously important platform for the development of quantum sensors, including for single spin and single molecule NMR. Detection of weak single-spin signals is greatly enhanced by…

量子物理 · 物理学 2017-05-29 J. E. Lang , J. Casanova , Z. -Y. Wang , M. B. Plenio , T. S. Monteiro

Efficient, low noise conversion between different colors of light is a necessary tool for interfacing quantum optical technologies that have different operating wavelengths. Optomechanically mediated wavelength conversion and amplification…

光学 · 物理学 2019-12-16 Matthew Mitchell , David P. Lake , Paul E. Barclay

The nitrogen-vacancy (N-V) center in diamond is promising as an electron spin qubit due to its long-lived coherence and optical addressability. The ground state is a spin triplet with two levels ($m_s = \pm 1$) degenerate at zero magnetic…

其他凝聚态物理 · 物理学 2007-10-15 T. P. Mayer Alegre , C. Santori , G. Medeiros-Ribeiro , R. G. Beausoleil